ii型InAs/GaAsSb量子点中空间间接激子的辐射寿命

IF 2.4 4区 物理与天体物理 Q3 PHYSICS, CONDENSED MATTER Solid State Communications Pub Date : 2025-03-01 Epub Date: 2024-12-10 DOI:10.1016/j.ssc.2024.115794
I. Saïdi, K. Boujdaria
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引用次数: 0

摘要

InAs/GaAsSb量子点(QDs)在近红外光谱中具有特殊的发射特性,通常在1.28 ~ 1.6 μm范围内。这些纳米结构在光纤通信、医学成像和环境传感系统中有着重要的应用前景。在这项工作中,我们从理论上研究了锑成分对嵌入在GaAsSb势垒中的ii型InAs量子点发射特性的影响。首先,我们重点研究了InAs/GaAs1−xSbx/GaAs异质结构中晶格失配引起的应变对载流子约束谱的依赖关系(x=0.18, 0.24和0.28)。其次,讨论了约束势对载流子空间分布的影响。然后,我们用精确的数值对角化方法计算了电子态作为锑组成的函数。ii型量子点的基态激子结合能较低,约为(≃4 meV)。最后,空间间接激子结构的基态激子跃迁能和相应的辐射寿命的预测值与实验结果基本一致。
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Radiative lifetimes of spatially indirect excitons in type-II InAs/GaAsSb quantum dots
InAs/GaAsSb quantum dots (QDs) are recognized for their exceptional emission in the near-infrared spectrum, typically ranging from 1.28 to 1.6 μm. These nanostructures hold significant promise for applications in fiber-optic communication, medical imaging, and environmental sensing systems. In this work, we theoretically investigated the effect of antimony composition on the emission properties of type-II InAs QDs embedded in GaAsSb barriers. First, we focus on the dependence of strain induced by lattice mismatch on charge carrier confinement profiles in InAs/GaAs1xSbx/GaAs heterostructures ( x=0.18, 0.24, and 0.28). Second, we discuss the influence of confinement potentials on the spatial distribution of charge carriers. We then calculate the electronic states as a function of antimony composition using an exact numerical diagonalization method. The ground-state exciton binding energy is estimated to be low, around ( 4 meV), for type-II QDs. Finally, the predicted values of the ground-state excitonic transition energy and the corresponding radiative lifetime of spatially indirect excitons structures are generally consistent with experimental results.
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来源期刊
Solid State Communications
Solid State Communications 物理-物理:凝聚态物理
CiteScore
3.40
自引率
4.80%
发文量
287
审稿时长
51 days
期刊介绍: Solid State Communications is an international medium for the publication of short communications and original research articles on significant developments in condensed matter science, giving scientists immediate access to important, recently completed work. The journal publishes original experimental and theoretical research on the physical and chemical properties of solids and other condensed systems and also on their preparation. The submission of manuscripts reporting research on the basic physics of materials science and devices, as well as of state-of-the-art microstructures and nanostructures, is encouraged. A coherent quantitative treatment emphasizing new physics is expected rather than a simple accumulation of experimental data. Consistent with these aims, the short communications should be kept concise and short, usually not longer than six printed pages. The number of figures and tables should also be kept to a minimum. Solid State Communications now also welcomes original research articles without length restrictions. The Fast-Track section of Solid State Communications is the venue for very rapid publication of short communications on significant developments in condensed matter science. The goal is to offer the broad condensed matter community quick and immediate access to publish recently completed papers in research areas that are rapidly evolving and in which there are developments with great potential impact.
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