甲醇制烯烃流化床反应器混合模型的人工神经网络校正

IF 4.3 2区 工程技术 Q2 ENGINEERING, CHEMICAL Chemical Engineering Science Pub Date : 2025-03-15 Epub Date: 2025-02-12 DOI:10.1016/j.ces.2025.121323
Chengyu Wang , Wei Wang , Yanji Sun , Yanqiu Pan , Chuanzhi Jia
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引用次数: 0

摘要

流化床反应器(FBR)的混合建模一直是一个具有挑战性的问题。建立了用于甲醇制烯烃(MTO)快堆过程实时优化与控制的混合模型。具体而言,提出了一种拟均匀移动床反应器(PHMBR)模型作为FBR的近似,然后采用基于人工神经网络(ANN)的校正模型进行误差补偿。采用基于自举算法的数据扩展方法,对训练数据不足的神经网络进行了补充。为了获得更好的预测效果,对偏差校正和因子校正两种混合模型进行了比较。结果表明,经因子校正的MTO-FBR混合模型能够预测出溶出时间小于0.03 s、RMSE小于2.85、MRE小于7.63 %的FBR出口参数。所提出的建模方法有望为其他反应过程提供一种新的策略。
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Hybrid modeling of methanol to olefin fluidized bed reactor corrected by artificial neural network
Hybrid modeling of fluidized bed reactor (FBR) remains as a challenging issue. A novel hybrid model was developed for the real-time optimization and control of FBR in the methanol to olefin (MTO) process. Specifically, a pseudo-homogeneous moving bed reactor (PHMBR) model was proposed as an approximation of the FBR, and then a correction model based on the artificial neural network (ANN) was adopted to compensate errors. A data expansion method based on the bootstrap algorithm was used to supplement insufficient training data for the ANN. Two hybrid models with deviation correction and factor correction were compared in order to attain the better predictive performance. The results showed that the hybrid model of MTO-FBR with factor correction could predict FBR outlet parameters with solution time below 0.03 s, RMSE below 2.85, and MRE below 7.63 %. The proposed modeling approach is expected to provide a new strategy for other reaction processes.
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来源期刊
Chemical Engineering Science
Chemical Engineering Science 工程技术-工程:化工
CiteScore
7.50
自引率
8.50%
发文量
1025
审稿时长
50 days
期刊介绍: Chemical engineering enables the transformation of natural resources and energy into useful products for society. It draws on and applies natural sciences, mathematics and economics, and has developed fundamental engineering science that underpins the discipline. Chemical Engineering Science (CES) has been publishing papers on the fundamentals of chemical engineering since 1951. CES is the platform where the most significant advances in the discipline have ever since been published. Chemical Engineering Science has accompanied and sustained chemical engineering through its development into the vibrant and broad scientific discipline it is today.
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