新鲜有机食品中荧光锗检测仪在光谱分析中减少计数时间的研究

IF 1.8 3区 工程技术 Q3 CHEMISTRY, INORGANIC & NUCLEAR Applied Radiation and Isotopes Pub Date : 2025-06-01 Epub Date: 2025-02-18 DOI:10.1016/j.apradiso.2025.111744
Nadia Rodrigues dos Santos , Alessandro Mariano Domingues , Izabella Soares de Souza , Carlos Omar Pastrana Orejuela , Ademir Xavier da Silva , Edmilson Monteiro de Souza , Inayá Corrêa Barbosa Lima
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引用次数: 0

摘要

环境基质中天然放射性核素的定量通常采用伽马能谱法,采用HPGe探测器。计数时间的可变性在文献中有报道,通常基于经验知识。本研究旨在通过减少环境保护单位种植的一些新鲜和冷冻有机蔬菜中40K放射性核素活性浓度的不确定性百分比变化,估计在分析40K放射性核素活性浓度过程中计数时间的减少。对于每个样品,使用HPGe检测器和Genie 2000数据采集软件,在36,000 s的周期内,以3600 s的定期间隔进行10次计数测量。在相同的时间间隔和相同的样品几何形状下获得背景光谱。利用LabSOCS软件进行效率曲线和自衰减校正。考虑计数次数25,200 s和36,000 s,测定的红萝卜、大白菜和红枣的40K活性浓度(Bq.kg−1)为(107±16.49);109±16.35),(79±12.77);81±12.62)和(100±15.44);102±15.36)。活动集中度的不确定性开始略有变化,并从2005年开始趋于稳定。结果表明,考虑到所采用的方法,延长新鲜和冷冻有机食品的计数时间不会比减少检测器操作时间产生显著的优势。
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Study of the reduction in the time of counting in spectrometric analysis using HPGe detector for samples of fresh organic foods
The quantification of natural radionuclides within environmental matrices is commonly executed via gamma spectrometry, employing HPGe detector. Variability in counting times is reported in the literature, often predicated on empirical knowledge. This study aims to estimate a reduction in counting time in the process of analyzing activity concentration of 40K radionuclide, based on reducing the percentage variation of their uncertainties, in some fresh and frozen organic vegetables, grown in an environmental conservation unit. For each sample, 10 count measurements were taken at regular intervals of 3600 s over a period of 36,000 s using the HPGe detector and the Genie 2000 data acquisition software. The background spectrum was obtained at the same time intervals and with the same sample geometry. Efficiency curves and self-attenuation corrections were performed using the LabSOCS software. Considering the counting times 25,200 s and 36,000 s, the determined 40K activity concentration (Bq.kg−1) for lady's finger banana, cabbage and carrot were (107 ± 16.49; 109 ± 16.35), (79 ± 12.77; 81 ± 12.62) and (100 ± 15.44; 102 ± 15.36), respectively. The activity concentrate uncertainty starts to vary slightly and began to stabilize from 25,200s onwards. The results indicate that considering the employed methodology, extending the counting time for fresh and frozen organic foods would not yield a significant advantage over reducing the detector operation time.
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来源期刊
Applied Radiation and Isotopes
Applied Radiation and Isotopes 工程技术-核科学技术
CiteScore
3.00
自引率
12.50%
发文量
406
审稿时长
13.5 months
期刊介绍: Applied Radiation and Isotopes provides a high quality medium for the publication of substantial, original and scientific and technological papers on the development and peaceful application of nuclear, radiation and radionuclide techniques in chemistry, physics, biochemistry, biology, medicine, security, engineering and in the earth, planetary and environmental sciences, all including dosimetry. Nuclear techniques are defined in the broadest sense and both experimental and theoretical papers are welcome. They include the development and use of α- and β-particles, X-rays and γ-rays, neutrons and other nuclear particles and radiations from all sources, including radionuclides, synchrotron sources, cyclotrons and reactors and from the natural environment. The journal aims to publish papers with significance to an international audience, containing substantial novelty and scientific impact. The Editors reserve the rights to reject, with or without external review, papers that do not meet these criteria. Papers dealing with radiation processing, i.e., where radiation is used to bring about a biological, chemical or physical change in a material, should be directed to our sister journal Radiation Physics and Chemistry.
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