IF 10.4 1区 化学 Q1 CHEMISTRY, MULTIDISCIPLINARY Science China Chemistry Pub Date : 2024-10-09 DOI:10.1007/s11426-024-2223-0
Shuang Ben, Han Ma, Rui Liu, Yuzhen Ning, Zhihong Zhao, Xudong Zhang, Qiang Li, Kesong Liu
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引用次数: 0

摘要

表面活性剂或水溶液中气泡的可控输送在日用化工、食品发酵、矿物浮选等领域非常重要。然而,气泡主要受浮力影响,在溶液中向上运动,这给气泡的操控带来了困难。尽管在控制水下气泡方面已经取得了一些进展,但不依靠外力实现水下气泡的持续运输和收集仍然是一个巨大的挑战。为此,我们仿生设计了一种具有双破冰特性的柔性聚二甲基硅氧烷(PDMS)多孔表面。也就是说,集结构梯度和润湿性梯度于一体的多孔 PDMS 膜在无外力输入的情况下实现了气泡的水下反浮力单向输送,具备了水下气体反浮力输送和储存的能力。这项工作为水下气体输送与封存装置的开发与设计提供了启示和方向,为海底二氧化碳封存技术的实现提供了创新思维。
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Flexible dual-Janus porous membrane for underwater gas bubbles anti-buoyancy unidirectional transportation

Controllable transportation of bubbles in surfactant or aqueous is very important in daily chemical products, food fermentation, mineral flotation and other fields. However, bubbles are mainly dominated by buoyancy and move upward in solution, which makes the manipulation of bubbles difficult. Although some progress has been made in controlling underwater bubbles, achieving continuous transportation and collection of underwater bubbles without relying on external forces is still a great challenge. To this end, we bionically designed a flexible polydimethylsiloxane (PDMS) porous surface with dual-Janus characteristics. Namely, a porous PDMS membrane integrating structural gradient and wettability gradient realizes the underwater anti-buoyancy unidirectional transportation of bubbles without external force input, and possesses the capability of underwater gas anti-buoyancy transportation and storage. This work provides inspiration and direction for the development and design of underwater gas transportation and storage devices and provides innovative thinking for the implementation of seabed carbon dioxide storage technology.

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来源期刊
Science China Chemistry
Science China Chemistry CHEMISTRY, MULTIDISCIPLINARY-
CiteScore
14.40
自引率
7.30%
发文量
3787
审稿时长
2.2 months
期刊介绍: Science China Chemistry, co-sponsored by the Chinese Academy of Sciences and the National Natural Science Foundation of China and published by Science China Press, publishes high-quality original research in both basic and applied chemistry. Indexed by Science Citation Index, it is a premier academic journal in the field. Categories of articles include: Highlights. Brief summaries and scholarly comments on recent research achievements in any field of chemistry. Perspectives. Concise reports on thelatest chemistry trends of interest to scientists worldwide, including discussions of research breakthroughs and interpretations of important science and funding policies. Reviews. In-depth summaries of representative results and achievements of the past 5–10 years in selected topics based on or closely related to the research expertise of the authors, providing a thorough assessment of the significance, current status, and future research directions of the field.
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