Jing Niu , Yu-Ting Miao , Wei David Wang , Meng-Tong Ruan , Zhi-Peng Wang , Hua-Dong Xue , Si-Min Yu , Chong Liu , Jian-Feng Wu , Wei Wang
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Observation of reactive intermediates in the initial stage during ethene conversion over acidic zeolites†
The key intermediates, i.e., surface ethoxy species, were observed upon the adsorption of ethene on zeolite H-Y for the first time. By combining a selective 13C-labeling protocol with a multitechnique approach, we confirmed the critical role of surface ethoxy species, that is, equilibrium with ethene in the primary step and further alkylation to form the C–C bond.
期刊介绍:
A multidisciplinary journal focusing on cutting edge research across all fundamental science and technological aspects of catalysis.
Editor-in-chief: Bert Weckhuysen
Impact factor: 5.0
Time to first decision (peer reviewed only): 31 days