东印度城市大气中黑碳气溶胶的来源解析和健康风险评估

IF 3 4区 地球科学 Q2 ENVIRONMENTAL SCIENCES Journal of Atmospheric Chemistry Pub Date : 2021-04-05 DOI:10.1007/s10874-021-09418-9
Balram Ambade, Tapan Kumar Sankar
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引用次数: 22

摘要

黑碳(BC)与PM2.5(细颗粒物)在评价人类健康影响中起着重要作用。在印度东部贾姆谢德布尔国立理工学院(NIT J)和贾姆谢德布尔Sakchi (SAK J)两个不同地点,通过使用7种不同波长(如370、470、520、590、660、880和950 nm)的便携式酒精计(AE-33, Magee Scientific,美国),对BC浓度进行了冬季运动测量。研究期间,BC的质量浓度变化范围为4.19 ~ 15.36µgm - 3, NIT J和SAK J的平均浓度为8.88±2.40µgm - 3; BC的质量浓度变化范围为6.3 ~ 13.48µgm - 3,平均为10.29±1.58µgm - 3。NIT J区和SAK J区的PM2.5浓度变化范围为102.98 ~ 198.21µgm−3,平均值为155.82±29.98µgm−3;NIT J区PM2.5浓度变化范围为110.83 ~ 207.65µgm−3,平均值为169.14±22.40µgm−3。据报道,与NIT J相比,SAK J的BC浓度更高。这是由于SAK J的交通负荷大,人口密集。根据BC的诊断率分析,在特定地区,BC的质量浓度主要来自化石燃料(69.70%),其次是木材燃烧(30.30%)。研究期间观察到的BC浓度在NIT J的总体健康风险评估为26.70、13.95、24.95和51.32,在SAK J的总体健康风险评估分别为32.07、16.72、29.95和61.87,在CVM、LC、LBW和PLEDSC的风险方面与被动卷烟相当。
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Source apportionment and health risks assessment of black carbon Aerosols in an urban atmosphere in East India

Black carbon (BC) along with PM2.5 (fine particular matters) plays an important role in the assessment health effect of human beings. Winter season campaign measurements carried out for BC concentrations by using 7 different wavelengths such as 370, 470, 520, 590, 660, 880, and 950 nm, handy aethalometer (AE-33, Magee Scientific, USA), at two different locations i.e., National Institute of Technology, Jamshedpur (NIT J) and Sakchi, Jamshedpur (SAK J), in eastern India. During the study period, the mass concentration of BC varies from 4.19 µgm−3 to 15.36 µgm−3, with an average mean of 8.88 ± 2.40 µgm−3 in NIT J and SAK J, the mass concentration of BC varies from 6.3 µgm−3 to 13.48 µgm−3, with an average mean of 10.29 ± 1.58 µgm−3. However, the concentration of PM2.5 varies from 102.98 µgm−3to 198.21 µgm−3, with an average mean of 155.82 ± 29.98 µgm−3 in NIT J and SAK J, the concentration of PM2.5 varies from 110.83 µgm−3 to 207.65 µgm−3, with an average mean of 169.14 ± 22.40 µgm−3. It was reported that SAK J has a higher BC concentration compared to NIT J. This was due to heavy traffic load and dense population in SAK J. Backward Trajectories were seen that the airborne particulate matter came from differerajeshnt directions. According to the diagnostic ratio analysis of BC, it was observed that most of the BC mass concentrations come from fossil-fuel (69.70%) followed by wood-burning (30.30%) in a particular place. The overall health risk assessment of BC concentration observed during the study period was 26.70, 13.95, 24.95 and 51.32 at NIT J as well as 32.07, 16.72, 29.95 and 61.87 at SAK J, the passive cigarettes comparable concerning the risk of CVM, LC, LBW, and PLEDSC, respectively.

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来源期刊
Journal of Atmospheric Chemistry
Journal of Atmospheric Chemistry 地学-环境科学
CiteScore
4.60
自引率
5.00%
发文量
16
审稿时长
7.5 months
期刊介绍: The Journal of Atmospheric Chemistry is devoted to the study of the chemistry of the Earth''s atmosphere, the emphasis being laid on the region below about 100 km. The strongly interdisciplinary nature of atmospheric chemistry means that it embraces a great variety of sciences, but the journal concentrates on the following topics: Observational, interpretative and modelling studies of the composition of air and precipitation and the physiochemical processes in the Earth''s atmosphere, excluding air pollution problems of local importance only. The role of the atmosphere in biogeochemical cycles; the chemical interaction of the oceans, land surface and biosphere with the atmosphere. Laboratory studies of the mechanics in homogeneous and heterogeneous transformation processes in the atmosphere. Descriptions of major advances in instrumentation developed for the measurement of atmospheric composition and chemical properties.
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