{"title":"粘弹性溶液中非布朗颗粒悬浮液的流变学。第一部分:聚合物浓度的影响","authors":"Anni Zhang, E. Shaqfeh","doi":"10.1122/8.0000540","DOIUrl":null,"url":null,"abstract":"We study the effect of varying polymer concentration, measured by the dimensionless polymer viscosity partition function [Formula: see text], on the steady shear rheology of rigid particle suspensions using direct numerical simulation of the Oldroyd-B model. We compare the bulk rheology using immersed boundary simulations at [Formula: see text] and [Formula: see text] to body-fitted single-particle simulations and find that the per-particle viscosity and first normal stress difference coefficient are always shear-thickening at all values of [Formula: see text] considered. However, as [Formula: see text] decreases, the polymer stress transforms the flow field near each particle from closed concentric streamlines to helical streamlines that advect stretched polymers away from the particle surface. At low [Formula: see text], the polymer stress is diffuse, where the distribution of the particle induced fluid stress (PIFS) caused by the stretched polymers is spread out in the simulation domain rather than concentrated near the particle surface. Therefore in multiparticle simulations, the polymer stress can be significantly affected by particle-particle interactions. The stress generated by a given particle is disrupted by the presence of particles in its vicinity, leading to a significantly lower PIFS than that of the single-particle simulation. In addition, at increased volume fractions and low values of [Formula: see text], the polymer stress distribution on the particle surface shifts so as to increase the magnitude of the polymer stress moments, resulting in a shear-thickening stresslet contribution to the viscosity that is not seen in single particle or high [Formula: see text] simulations. This result indicates that for suspensions in highly viscoelastic suspending fluids that are characterized by a low [Formula: see text] parameter, hydrodynamic interactions are significant even at modest particle concentrations and fully resolved multiparticle simulations are necessary to understand the rheological behavior.","PeriodicalId":16991,"journal":{"name":"Journal of Rheology","volume":" ","pages":""},"PeriodicalIF":3.0000,"publicationDate":"2023-03-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"3","resultStr":"{\"title\":\"Rheology of non-Brownian particle suspensions in viscoelastic solutions. Part 1: Effect of the polymer concentration\",\"authors\":\"Anni Zhang, E. Shaqfeh\",\"doi\":\"10.1122/8.0000540\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"We study the effect of varying polymer concentration, measured by the dimensionless polymer viscosity partition function [Formula: see text], on the steady shear rheology of rigid particle suspensions using direct numerical simulation of the Oldroyd-B model. We compare the bulk rheology using immersed boundary simulations at [Formula: see text] and [Formula: see text] to body-fitted single-particle simulations and find that the per-particle viscosity and first normal stress difference coefficient are always shear-thickening at all values of [Formula: see text] considered. However, as [Formula: see text] decreases, the polymer stress transforms the flow field near each particle from closed concentric streamlines to helical streamlines that advect stretched polymers away from the particle surface. At low [Formula: see text], the polymer stress is diffuse, where the distribution of the particle induced fluid stress (PIFS) caused by the stretched polymers is spread out in the simulation domain rather than concentrated near the particle surface. Therefore in multiparticle simulations, the polymer stress can be significantly affected by particle-particle interactions. The stress generated by a given particle is disrupted by the presence of particles in its vicinity, leading to a significantly lower PIFS than that of the single-particle simulation. In addition, at increased volume fractions and low values of [Formula: see text], the polymer stress distribution on the particle surface shifts so as to increase the magnitude of the polymer stress moments, resulting in a shear-thickening stresslet contribution to the viscosity that is not seen in single particle or high [Formula: see text] simulations. This result indicates that for suspensions in highly viscoelastic suspending fluids that are characterized by a low [Formula: see text] parameter, hydrodynamic interactions are significant even at modest particle concentrations and fully resolved multiparticle simulations are necessary to understand the rheological behavior.\",\"PeriodicalId\":16991,\"journal\":{\"name\":\"Journal of Rheology\",\"volume\":\" \",\"pages\":\"\"},\"PeriodicalIF\":3.0000,\"publicationDate\":\"2023-03-01\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"3\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Journal of Rheology\",\"FirstCategoryId\":\"5\",\"ListUrlMain\":\"https://doi.org/10.1122/8.0000540\",\"RegionNum\":2,\"RegionCategory\":\"工程技术\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q2\",\"JCRName\":\"MECHANICS\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Journal of Rheology","FirstCategoryId":"5","ListUrlMain":"https://doi.org/10.1122/8.0000540","RegionNum":2,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q2","JCRName":"MECHANICS","Score":null,"Total":0}
Rheology of non-Brownian particle suspensions in viscoelastic solutions. Part 1: Effect of the polymer concentration
We study the effect of varying polymer concentration, measured by the dimensionless polymer viscosity partition function [Formula: see text], on the steady shear rheology of rigid particle suspensions using direct numerical simulation of the Oldroyd-B model. We compare the bulk rheology using immersed boundary simulations at [Formula: see text] and [Formula: see text] to body-fitted single-particle simulations and find that the per-particle viscosity and first normal stress difference coefficient are always shear-thickening at all values of [Formula: see text] considered. However, as [Formula: see text] decreases, the polymer stress transforms the flow field near each particle from closed concentric streamlines to helical streamlines that advect stretched polymers away from the particle surface. At low [Formula: see text], the polymer stress is diffuse, where the distribution of the particle induced fluid stress (PIFS) caused by the stretched polymers is spread out in the simulation domain rather than concentrated near the particle surface. Therefore in multiparticle simulations, the polymer stress can be significantly affected by particle-particle interactions. The stress generated by a given particle is disrupted by the presence of particles in its vicinity, leading to a significantly lower PIFS than that of the single-particle simulation. In addition, at increased volume fractions and low values of [Formula: see text], the polymer stress distribution on the particle surface shifts so as to increase the magnitude of the polymer stress moments, resulting in a shear-thickening stresslet contribution to the viscosity that is not seen in single particle or high [Formula: see text] simulations. This result indicates that for suspensions in highly viscoelastic suspending fluids that are characterized by a low [Formula: see text] parameter, hydrodynamic interactions are significant even at modest particle concentrations and fully resolved multiparticle simulations are necessary to understand the rheological behavior.
期刊介绍:
The Journal of Rheology, formerly the Transactions of The Society of Rheology, is published six times per year by The Society of Rheology, a member society of the American Institute of Physics, through AIP Publishing. It provides in-depth interdisciplinary coverage of theoretical and experimental issues drawn from industry and academia. The Journal of Rheology is published for professionals and students in chemistry, physics, engineering, material science, and mathematics.