运输部门对大气气溶胶的全球影响以及由此产生的共同社会经济途径下的气候影响

M. Righi, J. Hendricks, S. Brinkop
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引用次数: 0

摘要

摘要应用全球气溶胶-气候模型来量化运输部门(陆路运输、航运和航空)对气溶胶和气候的影响。基于气候模型相互比较项目第6阶段(CMIP6)的排放清单,以及共享社会经济路径(SSP)下的近期(2030年)和中期(2050年)未来预测,对当前(2015年)进行了全球模拟。目前的结果表明,在全球人口最多的地区,陆地运输排放对黑碳和气溶胶硝酸盐的近地表浓度有很大影响,但发达国家和发展中国家之间的相对贡献模式截然不同。尽管最近出台了限制航运部门燃料硫含量的法规,但航运排放仍然对气溶胶硫酸盐近地表浓度产生了相当大的影响,约为0.5至1 µg m−3,对大陆空气污染和北极地区也有显著影响。航空对气溶胶质量的影响很小,约为每立方米几纳克,而这一部门对粒子数浓度的影响很大,高达20 %–30 % 北中纬度对流层上层粒子数浓度。传输对气溶胶质量和数量浓度的影响导致了今天−164、−145和−64的辐射强迫 mW m−2,分别用于陆地运输、航运和航空,气溶胶-云相互作用起主要作用。这些强迫作用明显抵消了运输部门的二氧化碳变暖,因此与气候政策非常相关。SSPs下的预测表明,运输部门对气溶胶和气候的影响通常与这些情景下的叙述一致:运输对气溶胶和天气的最低影响是在SSP1下模拟的,尤其是对陆地运输部门,而SSP3通常具有最大影响的特征。然而,这一情况也存在明显的例外,因为其他人为部门的排放也有助于总体气溶胶浓度,从而调节了运输部门在不同情景下的相关性,并不总是与其基本故事情节一致。在质量层面上,目前的结果大多证实了我们之前对2000年的评估结果,该评估使用了同一模型的前身版本和CMIP5排放数据。发现了一些重要的定量差异,这主要归因于本研究中气溶胶背景浓度的改善。
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The global impact of the transport sectors on the atmospheric aerosol and the resulting climate effects under the Shared Socioeconomic Pathways (SSPs)
Abstract. A global aerosol–climate model is applied to quantify the impact of the transport sectors (land transport, shipping, and aviation) on aerosol and climate. Global simulations are performed for the present day (2015), based on the emission inventory of the Climate Model Intercomparison Project Phase 6 (CMIP6), and for near-term (2030) and mid-term (2050) future projections, under the Shared Socioeconomic Pathways (SSPs). The results for the present day show that land transport emissions have a large impact on near-surface concentrations of black carbon and aerosol nitrate over the most populated areas of the globe, but with contrasting patterns in terms of relative contributions between developed and developing countries. In spite of the recently introduced regulations to limit the fuel sulfur content in the shipping sector, shipping emissions are still responsible for a considerable impact on aerosol sulfate near-surface concentrations, about 0.5 to 1 µg m−3 in the most travelled regions, with significant effects on continental air pollution and in the northern polar regions as well. Aviation impacts on aerosol mass are found to be quite small, of the order of a few nanograms per cubic metre, while this sector considerably affects particle number concentrations, contributing up to 20 %–30 % of the upper-tropospheric particle number concentration at the northern mid-latitudes. The transport-induced impacts on aerosol mass and number concentrations result in a present-day radiative forcing of −164, −145, and −64 mW m−2 for land transport, shipping, and aviation, respectively, with a dominating contribution by aerosol–cloud interactions. These forcings represent a marked offset to the CO2 warming from the transport sectors and are therefore very relevant for climate policy. The projections under the SSPs show that the impact of the transport sectors on aerosol and climate are generally consistent with the narratives underlying these scenarios: the lowest impacts of transport on both aerosol and climate are simulated under SSP1, especially for the land transport sector, while SSP3 is generally characterized by the largest effects. Notable exceptions to this picture, however, exist, as the emissions of other anthropogenic sectors also contribute to the overall aerosol concentrations and thus modulate the relevance of the transport sectors in the different scenarios, not always consistently with their underlying storyline. On a qualitative level, the results for the present day mostly confirm the findings of our previous assessment for the year 2000, which used a predecessor version of the same model and the CMIP5 emission data. Some important quantitative differences are found, which can mostly be ascribed to the improved representation of aerosol background concentrations in the present study.
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