基于有效介质理论的金属颗粒掺杂磁光薄膜的非互易光学特性

IF 16.4 1区 化学 Q1 CHEMISTRY, MULTIDISCIPLINARY Accounts of Chemical Research Pub Date : 2023-01-01 DOI:10.1117/1.JNP.17.016001
Jianfei Han, Kaifeng Wei, Han Wang
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引用次数: 1

摘要

摘要在寻找下一代光学信息功能材料的过程中,磁光微结构由于能够打破基尔霍夫定律并产生更高的光电转换效率而引起了人们的极大关注。利用时域有限差分和传递矩阵方法对磁光微结构的光学性质进行了理论研究。然而,这些方法计算密集,并且需要周期性条件,这可能不能满足大多数制造的样品。对等效介质算法进行了改进,使其适用于磁光材料的等效。基于改进的等效介质理论(EMT),设计了一种掺Au颗粒的磁光InSb薄膜结构(D-InSb)。根据Bruggeman近似,得到了D-InSb层对传输矩阵波的有效介电函数。采用包含各向异性波在单轴介质中传播的薄膜光学公式计算了D-InSb薄膜的非互易吸收率。研究了填充率和层数等几何参数的影响。除了对不同入射角下的定向辐射特性进行建模外,还计算了半球形特性以了解光吸收。我们的研究结果可以为太阳能电池、红外吸收剂和光隔离器的设计提供方法和思路。
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Nonreciprocal optical properties of magneto-optical film doped with metal particles based on the effective medium theory
Abstract. In search of next-generation optical information functional materials, magneto-optical microstructures have attracted great attention since they can break Kirchhoff’s law and produce higher photoelectric conversion efficiency. Theoretical studies using finite-difference time-domain and transfer matrix methods have been performed to investigate the optical properties of magneto-optical microstructures. However, these methods are computationally intensive and require periodic conditions, which may not be satisfied with most fabricated samples. The equivalent medium algorithm is improved to make it suitable for the equivalent of magneto-optical materials. Based on the improved equivalent medium theory (EMT), a magneto-optical InSb film structure doped with Au particles (D-InSb) is designed. The effective dielectric functions of the D-InSb layer for transfer matrix waves are obtained from the Bruggeman approximation. Thin-film optics formulas incorporating the anisotropic wave propagation in uniaxial media are employed to calculate the nonreciprocal absorptance of the D-InSb film. The effect of geometric parameters, such as filling ratio and number of layers, is investigated. In addition to modeling the directional radiative properties at various angles of incidence, the hemispherical properties are also calculated to understand the light absorption. The results of our study can provide methods and ideas for the design of solar cells, infrared absorbers, and optical isolators.
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来源期刊
Accounts of Chemical Research
Accounts of Chemical Research 化学-化学综合
CiteScore
31.40
自引率
1.10%
发文量
312
审稿时长
2 months
期刊介绍: Accounts of Chemical Research presents short, concise and critical articles offering easy-to-read overviews of basic research and applications in all areas of chemistry and biochemistry. These short reviews focus on research from the author’s own laboratory and are designed to teach the reader about a research project. In addition, Accounts of Chemical Research publishes commentaries that give an informed opinion on a current research problem. Special Issues online are devoted to a single topic of unusual activity and significance. Accounts of Chemical Research replaces the traditional article abstract with an article "Conspectus." These entries synopsize the research affording the reader a closer look at the content and significance of an article. Through this provision of a more detailed description of the article contents, the Conspectus enhances the article's discoverability by search engines and the exposure for the research.
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