脉冲热流点燃多分散喷雾火焰

IF 16.4 1区 化学 Q1 CHEMISTRY, MULTIDISCIPLINARY Accounts of Chemical Research Pub Date : 2021-05-31 DOI:10.1177/17568277211014105
G. Kats, J. Greenberg
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引用次数: 0

摘要

提出了一种多分散喷雾/空气混合物在脉冲加热的无限表面下点火的数学分析方法。与以往的文献工作不同,本文叙述了整个点火过程的历史,从火焰胚祖阶段开始,经过热失控阶段,最后到火焰传播阶段。在当前阶段,化学动力学被认为是一个单一的全局反应的动力学。采用截面法对喷雾进行建模,确定了燃油喷射特性对点火的影响。在理论预测和完整的数值模拟之间发现了很好的一致性。在某些操作条件下,由于燃料液滴的蒸汽积聚以及液滴蒸发的热量损失而导致的点火延迟被发现起着重要的作用。临界能量通量与初始喷雾多分散性的比较表明,脉冲持续时间较大时差异较小,而脉冲持续时间较小时差异较大。尽管这些看似微小的差异,但研究表明,即使对于具有相同初始SMD的喷雾,初始喷雾的多分散性也会对火焰点燃是否发生或失败产生关键影响。
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Polydisperse spray flame ignition by a pulsed heat flux
A mathematical analysis of the ignition of a polydisperse spray/air mixture by an infinite surface heated in a pulsed manner is presented. In contrast to previous work in the literature, the entire history of the ignition process is accounted for starting from the flame-embryo progenitor stage, through the thermal runaway stage to the final flame propagation stage. For tractability at the current stage, the chemical kinetics is taken to be that of a single global reaction. The spray is modeled using the sectional approach and the influence of fuel spray characteristics on ignition is determined. Good agreement was found between the theoretical predictions and full numerical simulations. Delay in ignition due to the build-up of vapor from the fuel droplets as well as heat loss to the droplets for evaporation are found to play a significant role under certain operating conditions. Comparison between the critical energy flux and the initial spray polydispersity revealed small differences for larger values of the pulse duration but more significant minor differences for smaller pulse durations. Despite these seemingly minor differences, it was shown that the initial spray polydispersity can have a critical influence on whether flame ignition will occur or fail, even for sprays having the same initial SMD.
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来源期刊
Accounts of Chemical Research
Accounts of Chemical Research 化学-化学综合
CiteScore
31.40
自引率
1.10%
发文量
312
审稿时长
2 months
期刊介绍: Accounts of Chemical Research presents short, concise and critical articles offering easy-to-read overviews of basic research and applications in all areas of chemistry and biochemistry. These short reviews focus on research from the author’s own laboratory and are designed to teach the reader about a research project. In addition, Accounts of Chemical Research publishes commentaries that give an informed opinion on a current research problem. Special Issues online are devoted to a single topic of unusual activity and significance. Accounts of Chemical Research replaces the traditional article abstract with an article "Conspectus." These entries synopsize the research affording the reader a closer look at the content and significance of an article. Through this provision of a more detailed description of the article contents, the Conspectus enhances the article's discoverability by search engines and the exposure for the research.
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