{"title":"湍流均匀燃料-空气混合物中燃料Lewis数对最小点火能量及其跃迁的影响","authors":"V. Papapostolou, N. Chakraborty","doi":"10.1177/17568277231187494","DOIUrl":null,"url":null,"abstract":"The effects of fuel Lewis number on the minimum ignition energy (MIE) requirements for ensuring successful thermal runaway, and self-sustained flame propagation have been analysed for forced ignition of homogeneous fuel–air mixtures under decaying turbulence for a wide range of initial turbulence intensities using three-dimensional direct numerical simulations. The minimum energy demand for ensuring self-sustained flame propagation has been found to be greater than that for ensuring only thermal runaway irrespective of its outcome for large turbulence intensities, and the minimum ignition energy increases with increasing rms turbulent velocity irrespective of the fuel Lewis number. The MIE values have been found to increase more sharply with increasing turbulence intensity beyond a critical value for all fuel Lewis numbers considered here. The variations of the normalised MIE (MIE normalised by its laminar value) with increasing turbulence intensity beyond the critical point follow a power-law and the power-law exponent has been found to increase with an increase in fuel Lewis number. This behaviour has been explained using a scaling analysis. The stochasticity associated with forced ignition has been demonstrated by using different realisations of statistically similar turbulent flow fields for the energy inputs corresponding to the MIE and successful outcomes are obtained in most instances, justifying the evaluation of the MIE values in this analysis.","PeriodicalId":1,"journal":{"name":"Accounts of Chemical Research","volume":null,"pages":null},"PeriodicalIF":16.4000,"publicationDate":"2023-07-19","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Effects of fuel Lewis number on the minimum ignition energy and its transition for turbulent homogeneous fuel–air mixtures\",\"authors\":\"V. Papapostolou, N. Chakraborty\",\"doi\":\"10.1177/17568277231187494\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"The effects of fuel Lewis number on the minimum ignition energy (MIE) requirements for ensuring successful thermal runaway, and self-sustained flame propagation have been analysed for forced ignition of homogeneous fuel–air mixtures under decaying turbulence for a wide range of initial turbulence intensities using three-dimensional direct numerical simulations. The minimum energy demand for ensuring self-sustained flame propagation has been found to be greater than that for ensuring only thermal runaway irrespective of its outcome for large turbulence intensities, and the minimum ignition energy increases with increasing rms turbulent velocity irrespective of the fuel Lewis number. The MIE values have been found to increase more sharply with increasing turbulence intensity beyond a critical value for all fuel Lewis numbers considered here. The variations of the normalised MIE (MIE normalised by its laminar value) with increasing turbulence intensity beyond the critical point follow a power-law and the power-law exponent has been found to increase with an increase in fuel Lewis number. This behaviour has been explained using a scaling analysis. The stochasticity associated with forced ignition has been demonstrated by using different realisations of statistically similar turbulent flow fields for the energy inputs corresponding to the MIE and successful outcomes are obtained in most instances, justifying the evaluation of the MIE values in this analysis.\",\"PeriodicalId\":1,\"journal\":{\"name\":\"Accounts of Chemical Research\",\"volume\":null,\"pages\":null},\"PeriodicalIF\":16.4000,\"publicationDate\":\"2023-07-19\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Accounts of Chemical Research\",\"FirstCategoryId\":\"5\",\"ListUrlMain\":\"https://doi.org/10.1177/17568277231187494\",\"RegionNum\":1,\"RegionCategory\":\"化学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q1\",\"JCRName\":\"CHEMISTRY, MULTIDISCIPLINARY\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Accounts of Chemical Research","FirstCategoryId":"5","ListUrlMain":"https://doi.org/10.1177/17568277231187494","RegionNum":1,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"CHEMISTRY, MULTIDISCIPLINARY","Score":null,"Total":0}
Effects of fuel Lewis number on the minimum ignition energy and its transition for turbulent homogeneous fuel–air mixtures
The effects of fuel Lewis number on the minimum ignition energy (MIE) requirements for ensuring successful thermal runaway, and self-sustained flame propagation have been analysed for forced ignition of homogeneous fuel–air mixtures under decaying turbulence for a wide range of initial turbulence intensities using three-dimensional direct numerical simulations. The minimum energy demand for ensuring self-sustained flame propagation has been found to be greater than that for ensuring only thermal runaway irrespective of its outcome for large turbulence intensities, and the minimum ignition energy increases with increasing rms turbulent velocity irrespective of the fuel Lewis number. The MIE values have been found to increase more sharply with increasing turbulence intensity beyond a critical value for all fuel Lewis numbers considered here. The variations of the normalised MIE (MIE normalised by its laminar value) with increasing turbulence intensity beyond the critical point follow a power-law and the power-law exponent has been found to increase with an increase in fuel Lewis number. This behaviour has been explained using a scaling analysis. The stochasticity associated with forced ignition has been demonstrated by using different realisations of statistically similar turbulent flow fields for the energy inputs corresponding to the MIE and successful outcomes are obtained in most instances, justifying the evaluation of the MIE values in this analysis.
期刊介绍:
Accounts of Chemical Research presents short, concise and critical articles offering easy-to-read overviews of basic research and applications in all areas of chemistry and biochemistry. These short reviews focus on research from the author’s own laboratory and are designed to teach the reader about a research project. In addition, Accounts of Chemical Research publishes commentaries that give an informed opinion on a current research problem. Special Issues online are devoted to a single topic of unusual activity and significance.
Accounts of Chemical Research replaces the traditional article abstract with an article "Conspectus." These entries synopsize the research affording the reader a closer look at the content and significance of an article. Through this provision of a more detailed description of the article contents, the Conspectus enhances the article's discoverability by search engines and the exposure for the research.