非晶纳米催化剂的中短期有序

Geng Wu, Xiao Han, Xun Hong
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引用次数: 0

摘要

非晶态纳米催化剂由于其优异的催化性能而引起了人们的极大关注。最近的研究表明,非晶态纳米催化剂的性能与中短程有序度密切相关。这一观点旨在全面总结在理解无定形纳米催化剂中短程到中程有序的重要性及其与催化性能的相关性方面的最新进展。这一观点首先介绍了用于表征非晶纳米催化剂中短程有序的先进方法,包括纳米束电子衍射、扫描透射电子显微镜、原子电子断层扫描、对分布函数和X射线吸收精细结构光谱。接下来,讨论了中短程有序度对非晶纳米催化剂性能的影响。最后总结了无定形纳米催化剂目前面临的挑战,并提出了几个有前景的研究方向。通过确定进一步探索的障碍和潜在途径,这一观点旨在提供有价值的见解,推动高效无定形纳米催化剂的发展。
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Short-to-medium-range order in amorphous nanocatalysts

Amorphous nanocatalysts have attracted significant attention due to their outstanding catalytic performance. Recent research has indicated that the performance of amorphous nanocatalysts is closely related to the short-to-medium-range order. This perspective aims to provide a comprehensive summary of the latest advances in understanding the significance of short-to-medium-range order in amorphous nanocatalysts and its correlation with catalytic performance. This perspective commences by presenting advanced methods employed for characterizing the short-to-medium-range order of amorphous nanocatalysts, including nanobeam electron diffraction, scanning transmission electron microscopy, atomic electron tomography, pair distribution function, and X-ray absorption fine structure spectroscopy. Next, the effect of short-to-medium-range order in determining the properties of amorphous nanocatalysts is discussed. Current challenges faced in amorphous nanocatalysts are eventually summarized with several prospective research directions. By identifying the obstacles and potential avenues for further exploration, this perspective aims to contribute valuable insights that will propel the development of high-efficient amorphous nanocatalysts.

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