快堆压力容器包覆用低活化改性高锰氮奥氏体不锈钢

A. Saeed, Raed Mohmed El-Shazly, S. Ghali, S. El-Khamisy, S. El-fiki, M. Eissa
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引用次数: 7

摘要

研制成功了低镍和游离镍奥氏体不锈钢合金,并提出将其用作快堆压力容器包壳的液态钠冷却剂。制作了标准奥氏体不锈钢SS316L (AISI 316L)作为参考样品。镍含量部分或全部被锰和氮所取代。采用舍弗勒图、光学显微镜和x射线衍射图(XRD)对制备的不锈钢合金的显微组织进行了研究。采用维氏硬度、冲击和室温拉伸试验研究了所研制的不锈钢梯度的力学性能。采用开路电位法,用氯化钠对合金的腐蚀速率进行了研究。利用241 Am-Be中子源和高度校准的He-3探测器测量了慢中子和总慢中子去除截面。利用60 Co和232 Th放射源发射的8条伽马射线线和HPGe探测器研究了所制备合金的衰减参数。金相、舍弗勒图和XRD结果表明,所制备的不锈钢以奥氏体相为主,铁素体相较少。所研制的锰氮不锈钢的硬度、屈服强度和极限抗拉强度均高于SS316L。开发的不锈钢的延伸率相对低于标准的SS316L。Mn取代Ni后,合金的冲击韧性降低。开发的锰不锈钢具有比SS316L更高的总缓慢去除截面。另一方面,慢中子和伽马射线对所有被研究的不锈钢具有几乎相同的行为。
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Low Activation-Modified High Manganese-Nitrogen Austenitic Stainless Steel for Fast Reactor Pressure Vessel Cladding
Low and free nickel austenitic stainless steel alloys were developed successfully and proposed to be used as a liquid sodium coolant fast reactor pressure vessel cladding. A standard austenitic stainless steel SS316L (AISI 316L) was produced as a reference sample. The nickel content was partially or totally replaced by manganese and nitrogen. The microstructure of the produced stainless steel alloys was investigated using Schaeffler diagram, optical microscopy and X-ray diffraction patterns (XRD). Mechanical properties of the developed stainless steel grads were investigated using Vickers hardness, impact and tensile tests at room temperature. Sodium chloride was used to study the corrosion rate of the investigated alloys by open circuit potential technique. Slow and total slow neutrons removal cross sections were measured using 241 Am-Be neutron source and highly calibrated He-3 detector. Eight gamma ray lines which emitted from 60 Co and 232 Th radioactive sources and HPGe detector were used to study the attenuation parameters of the produced alloys. Metallography, Schaeffler diagram and XRD results showed that all the produced stainless steels are mainly of austenite phase with a small ferrite phase. The developed manganese-nitrogen stainless steels showed higher hardness, yield and ultimate tensile strength than SS316L. The elongation of developed stainless steels is relatively lower than the standard SS316L. The impact toughness was reduced with replacement of Ni by Mn. The developed manganese stainless steels have a higher total slow removal cross section than SS316L. On the other hand, the slow neutron and gamma rays have nearly the same behavior for all studied stainless steels.
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