Spin–Charge Conversion in Hybrid Structure PbZrO3/Y3Fe5O12/Pt

Multifunctional oxide heterostructures exhibiting magnetoelectric properties show great potential in advanced applications which are attracting a number of recent investigations. Herein, hybrid structures are presented including the antiferroelectricity film PbZrO3 (PZO) and the ferrimagnetic insulator (FMI) yttrium iron garnet (Y3Fe5O12, (YIG)) film by means of pulse laser deposition and magnetron sputtering, respectively. A visible double ferroelectricity hysteresis loop for PZO at low electrical field and the distinct X‐ray magnetic circular dichroism (XMCD) spectra for YIG are obtained. To study the spin current transfer processes between platinum (Pt) and the PZO/YIG system, the Pt film is deposited on the PZO/YIG bilayers as the conversion detector and the spin–charge conversion voltage can be obtained via inverse spin Hall effect (ISHE) under thermal gradient excitation. These results indicate that the hybrid structure PZO/YIG/Pt provides a potential route to realize an electric field control of spin–charge conversion and is instructive for future low‐power multiferroic heterostructures‐based spintronic devices.