Zizhan Sun, Qianmin Cong, Xiaoyu Wang, Jiayi Cui, Z. Cai, C. Fan, L. Pei
{"title":"一种可见光敏感的氧化银/铝酸钙纳米复合光催化剂","authors":"Zizhan Sun, Qianmin Cong, Xiaoyu Wang, Jiayi Cui, Z. Cai, C. Fan, L. Pei","doi":"10.1080/02670836.2023.2237273","DOIUrl":null,"url":null,"abstract":"A photo-deposition method was developed to synthesise argentous oxide/calcium aluminate nanocomposites (Ag2O-CAONCS) with orthorhombic Ca5Al6O14 and cubic Ag2O phases. Micro-morphology, micro-structure, optical, and visible-light catalytic properties were investigated via different techniques. Ag2O enhances visible-light absorption performance and decreases the band gap of the Ag2O-CAONCS. About 20 mL crystal violet (CV) dye (10 mgL–1) is totally degraded using 20 mg Ag2O-CAONCS under sunlight irradiation for 20 min. The enhanced photocatalytic activity of the Ag2O-CAONCS towards CV under sunlight irradiation is ascribed to the reduction of the band gap, improvement in visible-light absorption and inhibitation role of carriers recombination by Ag2O. The high, stable visible-light catalytic activity makes Ag2O-CAONCS promising photocatalysts for removing organic pollutants.","PeriodicalId":18232,"journal":{"name":"Materials Science and Technology","volume":null,"pages":null},"PeriodicalIF":1.7000,"publicationDate":"2023-07-21","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"A visible light-sensitive argentous oxide/calcium aluminate nanocomposite photocatalyst\",\"authors\":\"Zizhan Sun, Qianmin Cong, Xiaoyu Wang, Jiayi Cui, Z. Cai, C. Fan, L. Pei\",\"doi\":\"10.1080/02670836.2023.2237273\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"A photo-deposition method was developed to synthesise argentous oxide/calcium aluminate nanocomposites (Ag2O-CAONCS) with orthorhombic Ca5Al6O14 and cubic Ag2O phases. Micro-morphology, micro-structure, optical, and visible-light catalytic properties were investigated via different techniques. Ag2O enhances visible-light absorption performance and decreases the band gap of the Ag2O-CAONCS. About 20 mL crystal violet (CV) dye (10 mgL–1) is totally degraded using 20 mg Ag2O-CAONCS under sunlight irradiation for 20 min. The enhanced photocatalytic activity of the Ag2O-CAONCS towards CV under sunlight irradiation is ascribed to the reduction of the band gap, improvement in visible-light absorption and inhibitation role of carriers recombination by Ag2O. The high, stable visible-light catalytic activity makes Ag2O-CAONCS promising photocatalysts for removing organic pollutants.\",\"PeriodicalId\":18232,\"journal\":{\"name\":\"Materials Science and Technology\",\"volume\":null,\"pages\":null},\"PeriodicalIF\":1.7000,\"publicationDate\":\"2023-07-21\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Materials Science and Technology\",\"FirstCategoryId\":\"88\",\"ListUrlMain\":\"https://doi.org/10.1080/02670836.2023.2237273\",\"RegionNum\":4,\"RegionCategory\":\"材料科学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q3\",\"JCRName\":\"MATERIALS SCIENCE, MULTIDISCIPLINARY\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Materials Science and Technology","FirstCategoryId":"88","ListUrlMain":"https://doi.org/10.1080/02670836.2023.2237273","RegionNum":4,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q3","JCRName":"MATERIALS SCIENCE, MULTIDISCIPLINARY","Score":null,"Total":0}
A visible light-sensitive argentous oxide/calcium aluminate nanocomposite photocatalyst
A photo-deposition method was developed to synthesise argentous oxide/calcium aluminate nanocomposites (Ag2O-CAONCS) with orthorhombic Ca5Al6O14 and cubic Ag2O phases. Micro-morphology, micro-structure, optical, and visible-light catalytic properties were investigated via different techniques. Ag2O enhances visible-light absorption performance and decreases the band gap of the Ag2O-CAONCS. About 20 mL crystal violet (CV) dye (10 mgL–1) is totally degraded using 20 mg Ag2O-CAONCS under sunlight irradiation for 20 min. The enhanced photocatalytic activity of the Ag2O-CAONCS towards CV under sunlight irradiation is ascribed to the reduction of the band gap, improvement in visible-light absorption and inhibitation role of carriers recombination by Ag2O. The high, stable visible-light catalytic activity makes Ag2O-CAONCS promising photocatalysts for removing organic pollutants.
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