{"title":"一种灵活、高效、低成本的太阳能界面水蒸发水凝胶膜FeS2@CTS","authors":"Yunsong Xu, Yanran Gu, Zhongping Yao, Songtao Lu, Xiaohong Wu, Zhaohua Jiang","doi":"10.1139/cjc-2022-0174","DOIUrl":null,"url":null,"abstract":"Solar interfacial water evaporation to obtain pure water has attracted extensive attention in recent years. In this work, based on the excellent optical property of FeS2 and the cross-linking nanostructure of chitosan (CTS), a FeS2@CTS hydrogel composite film for solar interfacial water evaporation was developed by hydrothermal synthesis and the following composite coating technology. The prepared FeS2@CTS presented high solar absorptivity of 95.27% and fast optical response capability. Under the optimized condition, the evaporation rate of pure water reached 3.34 kg m−2 h−1 and the photothermal conversion efficiency was 103.06% under one sun irradiation. In five runs, the evaporation rate of the FeS2@CTS was stable, indicating the excellent cycle stability. Also, in the desalination test, the stable evaporation rate of 1.74 kg m−2 h−1 was obtained in five runs. Due to the simple preparation method, low cost, and outstanding interfacial evaporation property, this FeS2@CTS indicates great potential for the seawater desalination or other photothermal conversion applications.","PeriodicalId":9420,"journal":{"name":"Canadian Journal of Chemistry","volume":"28 1","pages":""},"PeriodicalIF":1.1000,"publicationDate":"2023-01-17","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"A flexible, high-efficiency, and low-cost FeS2@CTS hydrogel film for solar interface water evaporation\",\"authors\":\"Yunsong Xu, Yanran Gu, Zhongping Yao, Songtao Lu, Xiaohong Wu, Zhaohua Jiang\",\"doi\":\"10.1139/cjc-2022-0174\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"Solar interfacial water evaporation to obtain pure water has attracted extensive attention in recent years. In this work, based on the excellent optical property of FeS2 and the cross-linking nanostructure of chitosan (CTS), a FeS2@CTS hydrogel composite film for solar interfacial water evaporation was developed by hydrothermal synthesis and the following composite coating technology. The prepared FeS2@CTS presented high solar absorptivity of 95.27% and fast optical response capability. Under the optimized condition, the evaporation rate of pure water reached 3.34 kg m−2 h−1 and the photothermal conversion efficiency was 103.06% under one sun irradiation. In five runs, the evaporation rate of the FeS2@CTS was stable, indicating the excellent cycle stability. Also, in the desalination test, the stable evaporation rate of 1.74 kg m−2 h−1 was obtained in five runs. Due to the simple preparation method, low cost, and outstanding interfacial evaporation property, this FeS2@CTS indicates great potential for the seawater desalination or other photothermal conversion applications.\",\"PeriodicalId\":9420,\"journal\":{\"name\":\"Canadian Journal of Chemistry\",\"volume\":\"28 1\",\"pages\":\"\"},\"PeriodicalIF\":1.1000,\"publicationDate\":\"2023-01-17\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Canadian Journal of Chemistry\",\"FirstCategoryId\":\"92\",\"ListUrlMain\":\"https://doi.org/10.1139/cjc-2022-0174\",\"RegionNum\":4,\"RegionCategory\":\"化学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q3\",\"JCRName\":\"CHEMISTRY, MULTIDISCIPLINARY\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Canadian Journal of Chemistry","FirstCategoryId":"92","ListUrlMain":"https://doi.org/10.1139/cjc-2022-0174","RegionNum":4,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q3","JCRName":"CHEMISTRY, MULTIDISCIPLINARY","Score":null,"Total":0}
引用次数: 0
摘要
近年来,利用太阳界面蒸发获得纯水的研究受到了广泛的关注。本文基于FeS2优异的光学性能和壳聚糖(CTS)的交联纳米结构,采用水热合成和复合涂层技术制备了一种用于太阳界面水蒸发的FeS2@CTS水凝胶复合膜。制备的FeS2@CTS具有95.27%的太阳吸收率和快速的光响应能力。在优化条件下,单次照射下,纯水蒸发速率可达3.34 kg m−2 h−1,光热转换效率为103.06%。在5次运行中,FeS2@CTS的蒸发速率稳定,表明循环稳定性好。在脱盐试验中,5次运行获得了1.74 kg m−2 h−1的稳定蒸发速率。由于制备方法简单,成本低,界面蒸发性能优异,该FeS2@CTS在海水淡化或其他光热转换应用中具有很大的潜力。
A flexible, high-efficiency, and low-cost FeS2@CTS hydrogel film for solar interface water evaporation
Solar interfacial water evaporation to obtain pure water has attracted extensive attention in recent years. In this work, based on the excellent optical property of FeS2 and the cross-linking nanostructure of chitosan (CTS), a FeS2@CTS hydrogel composite film for solar interfacial water evaporation was developed by hydrothermal synthesis and the following composite coating technology. The prepared FeS2@CTS presented high solar absorptivity of 95.27% and fast optical response capability. Under the optimized condition, the evaporation rate of pure water reached 3.34 kg m−2 h−1 and the photothermal conversion efficiency was 103.06% under one sun irradiation. In five runs, the evaporation rate of the FeS2@CTS was stable, indicating the excellent cycle stability. Also, in the desalination test, the stable evaporation rate of 1.74 kg m−2 h−1 was obtained in five runs. Due to the simple preparation method, low cost, and outstanding interfacial evaporation property, this FeS2@CTS indicates great potential for the seawater desalination or other photothermal conversion applications.
期刊介绍:
Published since 1929, the Canadian Journal of Chemistry reports current research findings in all branches of chemistry. It includes the traditional areas of analytical, inorganic, organic, and physical-theoretical chemistry and newer interdisciplinary areas such as materials science, spectroscopy, chemical physics, and biological, medicinal and environmental chemistry. Articles describing original research are welcomed.