来自农业用水系统的氧化亚氮被高氮污染

Kiyo Hasegawa , Keisuke Hanaki , Tomonori Matsuo , Shin Hidaka
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引用次数: 63

摘要

对日本埼玉县高氮污染农业用水系统进行了调查。化肥、畜禽粪便等人为氮肥导致该地区地下水出现高硝酸盐氮(20 ~ 30 mgN/l)。地下水中溶解态N2O浓度在0 ~ 28.2 μgN/l之间。地下水中N2O的主要来源似乎是畜牧业区的硝化氮。当这些地下水流入水田和一条小河等有机质丰富的地区时,反硝化作用活跃,产生了大量的N2O。这些地方的溶解N2O浓度在10 ~ 400 μgN/l之间,来自小河的N2O气体通量极高(约500 μgN/m2·min)。虽然这些地区可以去除硝酸盐氮,但这些地区往往是N2O的重要来源。探索在保持高脱氮活性的同时降低N2O排放比的有效可行方法。为验证土壤中硫作为反硝化电子供体的有效性,进行了柱状实验和批状实验。当反硝化作用充分进行时,含单质硫的土壤柱中N2O的形成保持在较低水平。在添加CaCO3调节pH和添加单质硫或硫化铁的情况下,N2O的生成受到抑制。这表明通过向土壤中添加硫并进行硫反硝化可以减少N2O的排放。
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Nitrous oxide from the agricultural water system contaminated with high nitrogen

The agricultural water system especially contaminated with high nitrogen was surveyed in Saitama Prefecture, Japan. The anthropogenic nitrogen, such as fertilizer, livestock wastes, etc., caused the occurrence of high nitrate-nitrogen (20–30 mgN/l) in the groundwater in this area. The concentration of dissolved N2O in the groundwater ranged from 0 to 28.2 μgN/l. The main source of N2O in the groundwater seemed to be nitrified N from the stockbreeding areas. As this groundwater flowed into the organic matter rich areas, such as paddy fields and a small river, denitrification actively occurred and much N2O was produced there. Dissolved N2O concentration in these places ranged from 10 to 400 μgN/l and N2O gas flux from the small river was extremely high (about 500 μgN/m2 · min). While nitrate-nitrogen could be removed in these areas, these areas often served as significant N2O sources. The effective and feasible method to decrease the N2O emission ratio while keeping the denitrification activity high should be explored.

To demonstrate the efficiency of putting sulfur into soil as a denitrification electron donor, the column and the batch experiments were carried out. When denitrification proceeded sufficiently, N2O formation in the soil column packed with elemental sulfur was kept low. In the case of adding CaCO3 for pH adjustment and adding elemental sulfur or iron sulfide, N2O production was suppressed. This indicated the possibility to decrease N2O emission by adding sulfur into the soil and proceeding sulfur denitrification.

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