WRF-Chem模式对利马地区颗粒物的模拟研究:以2016年4月为例

O. Sánchez-Ccoyllo, C. G. Ordoñez-Aquino, Á. Muñoz, Alan Llacza, M. Andrade, Yang Liu, Warren Réategui-Romero, G. Brasseur
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引用次数: 14

摘要

气象研究和预报化学(WRF-Chem)模型用于开发秘鲁利马-卡亚奥大都市区(MALC)的可操作空气质量预报系统,该地区受到高颗粒物浓度事件的影响。在这项工作中,我们描述了一个可操作的空气质量预测平台的实施,该平台将用于决策者制定公共政策,并作为评估MALC空气污染物形成和运输的研究工具。为了检验这一新系统的能力,模拟了2016年4月的一次空气污染事件,该事件显示PM2.5浓度异常升高,并与现场空气质量测量结果进行了比较。此外,还开发了一种模型输出统计(MOS)算法,以改善WRF-Chem模型的可吸入颗粒物(PM10)和细颗粒物(PM2.5)的输出。结果表明,MOS将PM10和PM2.5的平均归一化偏差精度分别从-43.1%和71.3%提高到3.1%和7.3%。PM10和PM2.5的平均归一化总误差分别从48%和92.3%降低到13.4%和10.1%。WRF-Chem模式结果显示,气温和相对湿度与2016年4月观测值之间存在较好的相关关系。温度和相对湿度的平均归一化偏差分别约为- 0.6%和1.1%。此外,温度和相对湿度的平均归一化总误差分别约为4.0%和0.1%。结果表明,该模型系统可作为分析MALC地区空气质量的有效工具。
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Modeling Study of the Particulate Matter in Lima with the WRF-Chem Model: Case Study of April 2016.
The Weather Research and Forecasting-Chemistry (WRF-Chem) model was used to develop an operational air quality forecast system for the Metropolitan Area of Lima-Callao (MALC), Peru, that is affected by high particulate matter concentrations episodes. In this work, we describe the implementation of an operational air quality-forecasting platform to be used in the elaboration of public policies by decision makers, and as a research tool to evaluate the formation and transport of air pollutants in the MALC. To examine the skills of this new system, an air pollution event in April 2016 exhibiting unusually elevated PM2.5 concentrations was simulated and compared against in situ air quality measurements. In addition, a Model Output Statistic (MOS) algorithm has been developed to improve outputs of inhalable particulate matter (PM10) and fine particulate matter (PM2.5) from the WRF-Chem model. The obtained results showed that MOS increased the accuracy in terms of mean normalized bias for PM10 and PM2.5 from -43.1% and 71.3% to 3.1%, 7.3%, respectively. In addition, the mean normalized gross error for PM10 and PM2.5 were reduced from 48% and 92.3% to 13.4% and 10.1%, respectively. The WRF-Chem Model results showed an appropriate relationship between of temperature and relative humidity with observations during April 2016. Mean normalized bias for temperature and relative humidity were approximately - 0.6% and 1.1% respectively. In addition, the mean normalized gross error for temperature and relative humidity were approximately 4.0% and 0.1% respectively. The results showed that this modelling system can be a useful tool for the analysis of air quality in MALC.
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Modeling Study of the Particulate Matter in Lima with the WRF-Chem Model: Case Study of April 2016. Modeling Study of the Particulate Matter in Lima with the WRF-Chem Model: Case Study of April 2016.
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