Dmitrii Kolupaev , Michail Logunov , Alexader Mashkin , Konstantin Bugrov , Konstanin Korchenkin , Andrei Shadrin , Konstanin Dvoeglazov
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引用次数: 5
摘要
2012年和2014年,RT-1工厂对BN-600反应堆的混合铀钚乏燃料进行了两次后处理。总共有8个燃料组件进行了再处理,燃耗从73到89 GW /t,冷却时间从17到21年不等。后处理包括溶解、澄清、从裂变产物中提纯U和Pu的提取分离、在相应的精炼循环中精炼铀和钚等阶段。在氟离子存在的情况下,硝酸溶液中MOX UNF燃料成分的溶解是随着锕系元素完全转移到溶液中而发生的。在高浓铀乏燃料后处理和铀精炼的核安全设备上进行了铀和铀的分离。锕系元素的提取、分离和精炼的工艺过程没有偏离正常模式。提取口的输出流量在其组成中符合管制规范,并保持在RT-1厂典型燃料类型后处理所产生的流的组成水平。在BN-600 MOX UNF后处理过程中,与VVER-440铀UNF后处理相比,没有记录到Pu在废物中的损失增加。
Reprocessing of the mixed uranium-plutonium spent nuclear fuel of the BN-600 reactor was performed at the RT-1 plant twice, in 2012 and 2014. In total, 8 fuel assemblies with a burn-up from 73 to 89 GW day/t and the cooling time from 17 to 21 years were reprocessed. The reprocessing included the stages of dissolution, clarification, extraction separation of U and Pu with purification from the fission products, refining of uranium and plutonium at the relevant refining cycles. Dissolution of the fuel composition of MOX UNF in nitric acid solutions in the presence of fluoride ion has occurred with the full transfer of actinides into solution. Due to the high content of Pu extraction separation of U and Pu was carried out on a nuclear-safe equipment designed for the reprocessing of highly enriched U spent nuclear fuel and Pu refining. Technological processes of extraction, separation and refining of actinides proceeded without deviations from the normal mode. The output flow of the extraction outlets in their compositions corresponded to the regulatory norms and remained at the level of the compositions of the streams resulting from the reprocessing of fuel types typical for the RT-1 plant. No increased losses of Pu into waste have been registered during the reprocessing of BN-600 MOX UNF an compare with VVER-440 uranium UNF reprocessing.