用于调谐太赫兹波的ti2o3薄膜的优异光热转换

Yu Cai, Hongfu Zhu, Qiwu Shi, Ye Cheng, Lei Chang, Wanxia Huang
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摘要

太赫兹(THz)波的动态调谐对于下一代太赫兹器件的开发至关重要。利用太阳能来调谐太赫兹波是解决长期能源危机的一种有前途的、环保的、可持续的方法。Ti 2o3具有0.1eV的超窄带隙,表现出令人感兴趣的热致金属-绝缘体转变(MIT),并具有优异的光热转换效率。本文采用两步磁控溅射法制备了Ti 2o3薄膜,该薄膜具有90.45%的光热转换效率,且具有0.1-1 THz宽带的温度依赖太赫兹传输特性。我们希望将ti2o3薄膜的光热转换特性与温度相关的太赫兹透射特性结合起来,从而引入太阳能作为调谐太赫兹波的能量源。我们的工作将为研究ti2o3在太赫兹波段的MIT特性提供新的视角,并在未来户外场景中调谐太赫兹波的应用中显示出巨大的潜力。
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Excellent Photothermal Conversion of Ti 2O 3 Film for Tuning Terahertz Waves
Dynamic tuning of terahertz (THz) wave is vital for the development of next generation THz devices. Utilization of solar energy for tuning THz waves is a promising, eco-friendly, and sustainable way to solve the long-standing energy crisis. Ti 2 O 3 with an ultra-narrow bandgap of 0.1eV exhibits intriguing thermal-induced metal-insulator transition(MIT), and possesses excellent photothermal conversion efficiency. Herein, Ti 2 O 3 film was fabricated by a two-step magnetron sputtering method, and exhibited excellent photothermal conversion efficiency of 90.45% and demonstrated temperature-dependent THz transmission characteristics with a wide-band at 0.1-1 THz. We supposed to combine photothermal conversion characteristics with temperature-dependent THz transmission properties of Ti 2 O 3 film, which could introduce solar light as the energy source for tuning THz waves. Our work will provide new sight for investigating MIT characteristics of Ti 2 O 3 at THz regime and exhibit huge potential in the application of tuning terahertz waves in outdoor scenarios in the future.
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