磷灰石密闭裂变径迹的揭示:它是如何工作的以及为什么重要

IF 2.7 Q2 GEOCHEMISTRY & GEOPHYSICS Geochronology Pub Date : 2020-10-20 DOI:10.5194/gchron-2020-31
R. Ketcham, M. Tamer
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引用次数: 4

摘要

摘要我们提出了一个新的蚀刻模型和磷灰石中局限裂变径迹的揭示,基于阶梯蚀刻测量,显示了沿径迹变化的蚀刻速度,vT(x)。我们定义了两种端元模型形式:恒定核心,具有恒定蚀刻速率的中心区域,然后向轨道尖端脱落;线性,其中蚀刻速率从中点到尖端呈线性下降。在此基础上,我们构建了包含所有相关过程的受限轨道揭示特征,包括从抛光颗粒表面穿透和增厚半轨道,受限轨道的相交,以及分析选择测量哪些轨道和绕过哪些轨道。这两种模型形式都能够拟合来自化石足迹和未退火和退火诱导足迹的五组配对实验的阶梯蚀刻数据,支持了我们方法的正确性,并为裂变足迹热年代学的理论和实践提供了一系列见解。退火诱导磁道的蚀刻速率比未退火诱导磁道和自发磁道快得多,这影响了受限磁道长度和密度测量的相对效率,并表明高温实验室退火可能导致磁道芯的转变,而这种转变在局部退火的地质条件下不会发生。该模型量化了分析人员选择标准的变化,总结为轨迹尖端沿轨迹与整体蚀刻速度的比率(vT/vB),可能在受限长度测量的可重复性中发挥一级作用。这也表明,大部分相交的轨道没有被测量,这表明长度偏差是一个不充分的统计模型,以预测不同轨道种群的相对检测概率。vT(x)模型提供了一种优化蚀刻条件和跨蚀刻协议连接轨迹长度测量的方法。
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Confined fission track revelation in apatite: how it works and why it matters
Abstract. We present a new model for the etching and revelation of confined fission tracks in apatite, based on step etching measurements that demonstrate variable along-track etching velocity, vT(x). We define two end-member model forms: Constant-core, with a central zone of constant etching rate that then falls off toward track tips; and Linear, in which etching rates fall linearly from the midpoint to the tips. Based on these, we construct a characterization of confined track revelation that encompasses all of the relevant processes, including penetration and thickening of semi-tracks from the polished grain surface, intersection of confined tracks, and analyst selection of which tracks to measure and which to bypass. Both model forms are able to fit step-etching data from five sets of paired experiments of fossil tracks and unannealed and annealed induced tracks, supporting the correctness of our approach and providing a series of insights into the theory and practice of fission-track thermochronology. Etching rates for annealed induced tracks are much faster than those for unannealed induced and spontaneous tracks, impacting the relative efficiency of both confined track length and density measurements, and suggesting that high-temperature laboratory annealing may induce a transformation in track cores that does not occur at geological conditions of partial annealing. The model quantifies how variation in analyst selection criteria, summarized as the ratio of along-track to bulk etching velocity at the track tip (vT/vB), likely plays a first-order role in the reproducibility of confined length measurements. It also shows that a large proportion of tracks that are intersected are not measured, indicating that length biasing is an insufficient statistical model for predicting the relative probability of detection of different track populations. The vT(x) model provides an approach to both optimizing etching conditions and linking track length measurements across etching protocols.
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来源期刊
Geochronology
Geochronology Earth and Planetary Sciences-Paleontology
CiteScore
6.60
自引率
0.00%
发文量
35
审稿时长
19 weeks
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