环境辐射监测中空气中剂量当量率和活度浓度同时测定方法的研究

M. Kowatari, 古渡意彦, Y. Tanimura, 谷村嘉彦, P. Kessler, S. Neumaier, A. Röttger
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引用次数: 0

摘要

为了进行环境辐射监测,研究了利用新研制的cebr3闪烁光谱仪同时测定环境剂量当量率和空气中放射性浓度的方法。根据欧洲辐射剂量测定组(EURADOS)进行的早期预警网络探测器比对程序,通过一系列测量验证了所提出方法的性能,包括能量依赖性、角度依赖性和光谱仪的线性度(即其响应的剂量率依赖性)。实测结果表明,该方法适用于环境辐射监测。经过充分的试验,在实验室中利用一个点状密封的133ba源模拟了由于含有133i和133xe的放射性云造成的环境剂量当量率的人工增加,证明了从γ射线脉冲高度谱中获得空气中活度浓度的研究。利用展开法从脉冲高度谱得到了光子通量率,利用蒙特卡罗计算得到的转换系数,可以从得到的光子通量率估计出空气中放射性核素的活度浓度。
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Study on Method for Simultaneous Determination of Ambient Dose Equivalent Rates and Activity Concentration in Air for Environmental Radiation Monitoring
For proper environmental radiation monitoring, a method to simultaneously determine ambient dose equivalent rate and radioactivity concentration in the air by using a newly developed scintillation spectrometer, namely a CeBr 3 spectrometer was investigated. The performance of the proposed method, including energy dependence, angular dependence and the linearity of the spectrometer (i.e. the dose rate dependence of its re-sponse), was verified by a series of measurements, conducted according to the procedure of inter-comparison of detectors used for early warning network performed by the European Radiation Dosimetry Group (EURADOS). Measurement results show that the proposed method is suitable for environmental radiation monitoring pur-poses. After thorough tests, the investigation on obtaining activity concentration in air from the pulse height spectrum of γ-ray was demonstrated in the laboratory by using a point-like sealed 133 Ba source to simulate an artificial increase of ambient dose equivalent rate due to a radioactive cloud containing 131 I and 133 Xe. The photon fluence rate was obtained from the pulse height spectrum by using the unfolding method, and the activ ity concentration in air for radionuclides of interest could be estimated from the obtained photon fluence rate by applying the conversion coefficient evaluated via a Monte Carlo calculation.
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