Trung Thanh Nguyen, Ngoc Hanh Nguyen, T. N. Thi, Tri Thich Le, Phuoc Toan Phan, N. Nguyen
{"title":"载体对OMS-2气相氧化甲苯催化活性影响的研究","authors":"Trung Thanh Nguyen, Ngoc Hanh Nguyen, T. N. Thi, Tri Thich Le, Phuoc Toan Phan, N. Nguyen","doi":"10.51316/jst.159.etsd.2022.32.3.2","DOIUrl":null,"url":null,"abstract":"In this study, the complete oxidation of an aromatic hydrocarbon compound such as toluene into carbon dioxide and water was carried out in a continuous fixed bed reactor. OMS-2 material synthesized by the refluxing method was used as the catalyst. To reduce the cost of the catalyst, various support materials were employed for supporting the OMS-2 catalyst. The effects of supports (i.e., bentonite, kaolinite, and alumina) and their contents on the catalytic activity of OMS-2 for the oxidation of toluene were investigated. Among the supports, bentonite with Al:Si ratio of 1:2 was the best material with the lowest temperature that reached 100% of toluene conversion at 260 oC. Therefore, 20%OMS-2/bentonite could be a suitable catalyst with high efficiency but low cost for catalytic oxidation of toluene and other organic compounds in the gas phase.","PeriodicalId":17641,"journal":{"name":"JST: Engineering and Technology for Sustainable Development","volume":"36 1","pages":""},"PeriodicalIF":0.0000,"publicationDate":"2022-07-15","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"A Study on the Effect of Support on the Catalytic Activity of OMS-2 for Oxidation of Toluene in Gas Phase\",\"authors\":\"Trung Thanh Nguyen, Ngoc Hanh Nguyen, T. N. Thi, Tri Thich Le, Phuoc Toan Phan, N. Nguyen\",\"doi\":\"10.51316/jst.159.etsd.2022.32.3.2\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"In this study, the complete oxidation of an aromatic hydrocarbon compound such as toluene into carbon dioxide and water was carried out in a continuous fixed bed reactor. OMS-2 material synthesized by the refluxing method was used as the catalyst. To reduce the cost of the catalyst, various support materials were employed for supporting the OMS-2 catalyst. The effects of supports (i.e., bentonite, kaolinite, and alumina) and their contents on the catalytic activity of OMS-2 for the oxidation of toluene were investigated. Among the supports, bentonite with Al:Si ratio of 1:2 was the best material with the lowest temperature that reached 100% of toluene conversion at 260 oC. Therefore, 20%OMS-2/bentonite could be a suitable catalyst with high efficiency but low cost for catalytic oxidation of toluene and other organic compounds in the gas phase.\",\"PeriodicalId\":17641,\"journal\":{\"name\":\"JST: Engineering and Technology for Sustainable Development\",\"volume\":\"36 1\",\"pages\":\"\"},\"PeriodicalIF\":0.0000,\"publicationDate\":\"2022-07-15\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"JST: Engineering and Technology for Sustainable Development\",\"FirstCategoryId\":\"1085\",\"ListUrlMain\":\"https://doi.org/10.51316/jst.159.etsd.2022.32.3.2\",\"RegionNum\":0,\"RegionCategory\":null,\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"\",\"JCRName\":\"\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"JST: Engineering and Technology for Sustainable Development","FirstCategoryId":"1085","ListUrlMain":"https://doi.org/10.51316/jst.159.etsd.2022.32.3.2","RegionNum":0,"RegionCategory":null,"ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"","JCRName":"","Score":null,"Total":0}
A Study on the Effect of Support on the Catalytic Activity of OMS-2 for Oxidation of Toluene in Gas Phase
In this study, the complete oxidation of an aromatic hydrocarbon compound such as toluene into carbon dioxide and water was carried out in a continuous fixed bed reactor. OMS-2 material synthesized by the refluxing method was used as the catalyst. To reduce the cost of the catalyst, various support materials were employed for supporting the OMS-2 catalyst. The effects of supports (i.e., bentonite, kaolinite, and alumina) and their contents on the catalytic activity of OMS-2 for the oxidation of toluene were investigated. Among the supports, bentonite with Al:Si ratio of 1:2 was the best material with the lowest temperature that reached 100% of toluene conversion at 260 oC. Therefore, 20%OMS-2/bentonite could be a suitable catalyst with high efficiency but low cost for catalytic oxidation of toluene and other organic compounds in the gas phase.