进化算法在合成SAPO-34催化剂上建模和优化超声相关参数的应用:结晶度和粒度

IF 2.1 4区 化学 Q3 CHEMISTRY, PHYSICAL Progress in Reaction Kinetics and Mechanism Pub Date : 2018-10-01 DOI:10.3184/146867818X15233705894446
M. Azarhoosh, R. Halladj, S. Askari
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引用次数: 6

摘要

首先,利用遗传编程(GP)方法模拟了超声相关变量对合成SAPO-34催化剂结晶度和粒径的影响。结果表明,GP具有较好的预测能力。其次,采用遗传算法对超声参数进行优化,得到了高结晶度、最小粒径的SAPO-34催化剂,使其在甲醇制轻烯烃工艺中具有最佳性能。将GP模型作为遗传算法内部的适应度函数。最后,对最优解进行了实验验证,实验结果与预测值吻合较好。
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Application of Evolutionary Algorithms for Modelling and Optimisation of Ultrasound-Related Parameters on Synthesised SAPO-34 Catalysts: Crystallinity and Particle Size
First, the effects of ultrasound-related variables on the crystallinity and particle size of synthesised SAPO-34 catalysts were modelled using a genetic programming (GP) method. The results confirm that GP has good predictive power. Secondly, optimisation of the ultrasound parameters was considered using a genetic algorithm (GA) to obtain SAPO-34 catalysts with high crystallinity and minimum particle size for the best performance in the methanol to light olefins process. The GP models were used as the fitness functions inside the GA. Finally, the optimum solution was validated experimentally and the results indicate that there is a good agreement between experimental and predicted values.
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来源期刊
CiteScore
2.10
自引率
0.00%
发文量
5
审稿时长
2.3 months
期刊介绍: The journal covers the fields of kinetics and mechanisms of chemical processes in the gas phase and solution of both simple and complex systems.
期刊最新文献
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