TiO2/SAPO-5复合沸石的制备及其光催化降解苯酚的性能

Xiuhong Xu, R. Jiang, Hong-kai Shi, Kejuan Qiang, Peng Wang, Jing Wang
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引用次数: 2

摘要

采用水热法合成了具有AFI拓扑结构的SAPO-5微孔;采用溶胶-凝胶法制备了TiO2/SAPO-5复合沸石。采用多种分析技术对SAPO-5分子筛和TiO2/SAPO-5复合分子筛的结构进行了表征。XRD谱图表明,SAPO-5分子筛结晶度高,纯度高。通过SEM和BET分析了小粒径(500 ~ 600 nm)和大比表面积。以光催化降解苯酚为模型反应,评价了TiO2/SAPO-5复合沸石的光催化活性。与纯TiO2相比,TiO2/SAPO-5对苯酚具有更高的降解活性。
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Preparation of TiO2/SAPO-5 Composite Zeolite and its Photocatalytic Properties for the Degradation of Phenol
Abstract Microporous SAPO-5 with an AFI topology has been synthesized by hydrothermal method; using this material, TiO2/SAPO-5 composite zeolites were prepared using sol-gel technique. The structures of SAPO-5 molecular sieves and TiO2/SAPO-5 composite zeolites were characterized by several analytical techniques. XRD patterns show the high crystallinity and purity of SAPO-5 molecular sieves. The small particle size (500-600 nm) and the large specific surface area have been analyzed by SEM and BET. The photocatalytic activity of TiO2/SAPO-5 composite zeolite was evaluated by photocatalytic degradation of phenol as model reaction. TiO2/SAPO-5 exhibits a higher activity for the degradation of phenol in comparison with pure TiO2.
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来源期刊
CiteScore
0.88
自引率
0.00%
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审稿时长
1 months
期刊介绍: The Journal of advanced oxidation technologies (AOTs) has been providing an international forum that accepts papers describing basic research and practical applications of these technologies. The Journal has been publishing articles in the form of critical reviews and research papers focused on the science and engineering of AOTs for water, air and soil treatment. Due to the enormous progress in the applications of various chemical and bio-oxidation and reduction processes, the scope of the Journal is now expanded to include submission in these areas so that high quality submission from industry would also be considered for publication. Specifically, the Journal is soliciting submission in the following areas (alphabetical order): -Advanced Oxidation Nanotechnologies -Bio-Oxidation and Reduction Processes -Catalytic Oxidation -Chemical Oxidation and Reduction Processes -Electrochemical Oxidation -Electrohydraulic Discharge, Cavitation & Sonolysis -Electron Beam & Gamma Irradiation -New Photocatalytic Materials and processes -Non-Thermal Plasma -Ozone-based AOTs -Photochemical Degradation Processes -Sub- and Supercritical Water Oxidation -TiO2 Photocatalytic Redox Processes -UV- and Solar Light-based AOTs -Water-Energy (and Food) Nexus of AOTs
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