具有电子和空穴准粒子的光致奇异金属

N. Dasari, Jiajun Li, P. Werner, M. Eckstein
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引用次数: 2

摘要

莫特绝缘体或相关金属的光掺杂可以产生一种不寻常的金属态,同时容纳类空穴和类电子粒子。我们研究这种状态的动力学长达很长时间,因为它将动能传递给环境。当系统冷却下来时,它从坏金属过渡到有弹性的准粒子状态,在这种状态下,准粒子带形成了电子和空穴的独立费米能级,但准粒子还不满足费米液体范式。随后,能量向环境的传递明显减慢,即使在皮秒的时间尺度上,系统也没有达到费米液态。瞬态光掺杂奇异金属表现出与超快电荷和热输运相关的不同寻常的特性:特别是,电子和空穴的特性可能存在不对称性,并且电子和空穴之间存在强相关性,如光谱特性所示。
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Photoinduced strange metal with electron and hole quasiparticles
Photo-doping of Mott insulators or correlated metals can create an unusual metallic state which simultaneously hosts hole-like and electron-like particles. We study the dynamics of this state up to long times, as it passes its kinetic energy to the environment. When the system cools down, it crosses over from a bad metal into a resilient quasiparticle regime, in which quasiparticle bands are formed with separate Fermi levels for electrons and holes, but quasiparticles do not yet satisfy the Fermi liquid paradigm. Subsequently, the transfer of energy to the environment slows down significantly, and the system does not reach the Fermi liquid state even on the timescale of picoseconds. The transient photo-doped strange metal exhibits unusual properties of relevance for ultrafast charge and heat transport: In particular, there can be an asymmetry in the properties of electrons and holes, and strong correlations between electrons and holes, as seen in the spectral properties.
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