Bloch-type magnetic skyrmions in two-dimensional lattices†

IF 10.7 2区 材料科学 Q1 CHEMISTRY, MULTIDISCIPLINARY Materials Horizons Pub Date : 2023-08-26 DOI:10.1039/D3MH00868A
Wenhui Du, Kaiying Dou, Zhonglin He, Ying Dai, Baibiao Huang and Yandong Ma
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Abstract

Magnetic skyrmions in two-dimensional lattices are a prominent topic of condensed matter physics and materials science. Current research efforts in this field are exclusively constrained to Néel-type and antiskyrmions, while Bloch-type magnetic skyrmions are rarely explored. Here, we report the discovery of Bloch-type magnetic skyrmions in a two-dimensional lattice of MnInP2Te6, using first-principles calculations and Monte-Carlo simulations. Arising from the joint effect of broken inversion symmetry and strong spin–orbit coupling, monolayer MnInP2Te6 presents large Dzyaloshinskii–Moriya interaction. This, along with ferromagnetic exchange interaction and out-of-plane magnetic anisotropy, gives rise to skyrmion physics in monolayer MnInP2Te6, in the absence of a magnetic field. Remarkably, different from all previous works on two-dimensional lattices, the resultant magnetic skyrmions feature Bloch-type magnetism, which is protected by D3 symmetry. Furthermore, Bloch-type magnetic bimerons are also identified in monolayer MnTlP2Te6. The phase diagrams of these Bloch-type topological magnetisms under a magnetic field, temperature and strain are mapped out. Our results greatly enrich the research on magnetic skyrmions in two-dimensional lattices.

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二维晶格中的Bloch型磁性skyrmions。
二维晶格中的磁性skyrmions是凝聚态物理学和材料科学的一个重要课题。目前该领域的研究工作仅限于Néel型和抗skyrmions,而Bloch型磁性skyrmions很少被探索。在这里,我们使用第一性原理计算和蒙特卡罗模拟,在MnInP2Te6的二维晶格中发现了Bloch型磁性skyrmions。由于破坏的反转对称性和强自旋轨道耦合的共同作用,单层MnInP2Te6呈现出大的Dzyaloshinskii-Moriya相互作用。这与铁磁交换相互作用和平面外磁各向异性一起,在没有磁场的情况下,在单层MnInP2Te6中产生了skyrmion物理。值得注意的是,与以往所有关于二维晶格的工作不同,所产生的磁性skyrmions具有Bloch型磁性,受到D3对称性的保护。此外,在单层MnTlP2Te6中还鉴定出Bloch型磁性双原子子。绘制了这些Bloch型拓扑磁在磁场、温度和应变作用下的相图。我们的研究结果极大地丰富了二维晶格中磁性skyrmions的研究。
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来源期刊
Materials Horizons
Materials Horizons CHEMISTRY, MULTIDISCIPLINARY-MATERIALS SCIENCE, MULTIDISCIPLINARY
CiteScore
18.90
自引率
2.30%
发文量
306
审稿时长
1.3 months
期刊介绍: Materials Horizons is a leading journal in materials science that focuses on publishing exceptionally high-quality and innovative research. The journal prioritizes original research that introduces new concepts or ways of thinking, rather than solely reporting technological advancements. However, groundbreaking articles featuring record-breaking material performance may also be published. To be considered for publication, the work must be of significant interest to our community-spanning readership. Starting from 2021, all articles published in Materials Horizons will be indexed in MEDLINE©. The journal publishes various types of articles, including Communications, Reviews, Opinion pieces, Focus articles, and Comments. It serves as a core journal for researchers from academia, government, and industry across all areas of materials research. Materials Horizons is a Transformative Journal and compliant with Plan S. It has an impact factor of 13.3 and is indexed in MEDLINE.
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