Effect of roughness on third-order nonlinear-optical susceptibility of rare earth doped zinc oxide thin films

M. Addoua, M. El Jouad, A.M. Lamrani, Z. Sofian, B. Sahraoui, A. Monteil, N. Gaumer, S. Dabos, T. El Habbani, N. Fellah, K. Bahedi, L. Dghoughi
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引用次数: 2

Abstract

Zinc oxide (ZnO) and erbium doped zinc oxide (ZnO:Er) thin films, were deposited on heated glass substrates using spray pyrolysis technique. Third-order nonlinear-optical properties of ZnO and ZnO:Er have been investigated by the third harmonic generation (THG) method at the wavelength of 1064 nm using nanosecond Nd3+:YAG laser radiation. The dependence of third order nonlinear susceptibility and transmission characteristics on the thin film roughness has been measured. Third order nonlinear optical susceptibility ( chi(3)) values of the studied materials were in the remarkable range of 10-12 esu. The deposited films have been analyzed using X-ray diffraction (XRD) and atomic force microscopy (AFM).
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粗糙度对稀土掺杂氧化锌薄膜三阶非线性光学磁化率的影响
采用喷雾热解技术在加热玻璃衬底上制备氧化锌(ZnO)和掺铒氧化锌(ZnO:Er)薄膜。利用纳米级Nd3+:YAG激光辐射,用三次谐波产生(THG)方法研究了ZnO和ZnO:Er在1064 nm波长下的三阶非线性光学性质。测量了三阶非线性磁化率和透射特性与薄膜粗糙度的关系。材料的三阶非线性光磁化率(chi(3))值在10 ~ 12 esu的显著范围内。用x射线衍射仪(XRD)和原子力显微镜(AFM)对沉积膜进行了分析。
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