Cauê Kaufmann Ribeiro, L. Mello, V. Martelli, D. Cornejo, M. B. Silva Neto, E. Fogh, H. Rønnow, Julio Antonio Larrea Jiménez
{"title":"Investigation of role of antisite disorder in pristine cage compound FeGa$_3$","authors":"Cauê Kaufmann Ribeiro, L. Mello, V. Martelli, D. Cornejo, M. B. Silva Neto, E. Fogh, H. Rønnow, Julio Antonio Larrea Jiménez","doi":"10.21468/scipostphysproc.11.023","DOIUrl":null,"url":null,"abstract":"The role of controlled Fe antisite disorder in the narrow gap semiconductor FeGa_33 has been investigated. Polycrystalline samples were synthesized by the combination of arc-melting furnace and successive annealing processes. Deviations from occupation numbers of Fe and Ga sites expected in the pristine compound were obtained from X-ray data using Rietveld refinement analysis. Besides that, electrical transport and magnetization measurements reveal that hierarchy in Fe and Ga site disorder tunes the ground state of FeGa_33 from paramagnetic semiconductor to a magnetic metal. These findings are discussed inside the framework of Anderson localization in the vicinity of metal-semiconductor transitions and spin fluctuations.","PeriodicalId":355998,"journal":{"name":"SciPost Physics Proceedings","volume":"30 1","pages":"0"},"PeriodicalIF":0.0000,"publicationDate":"2023-09-05","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":null,"platform":"Semanticscholar","paperid":null,"PeriodicalName":"SciPost Physics Proceedings","FirstCategoryId":"1085","ListUrlMain":"https://doi.org/10.21468/scipostphysproc.11.023","RegionNum":0,"RegionCategory":null,"ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"","JCRName":"","Score":null,"Total":0}
引用次数: 0
Abstract
The role of controlled Fe antisite disorder in the narrow gap semiconductor FeGa_33 has been investigated. Polycrystalline samples were synthesized by the combination of arc-melting furnace and successive annealing processes. Deviations from occupation numbers of Fe and Ga sites expected in the pristine compound were obtained from X-ray data using Rietveld refinement analysis. Besides that, electrical transport and magnetization measurements reveal that hierarchy in Fe and Ga site disorder tunes the ground state of FeGa_33 from paramagnetic semiconductor to a magnetic metal. These findings are discussed inside the framework of Anderson localization in the vicinity of metal-semiconductor transitions and spin fluctuations.
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