Engineering the Device Performance of PLD Grown Tantalum Oxide based RRAM Devices

Alireza Moazzeni, Md. Tawsif Rahman Chowdhury, C. Rouleau, G. Tutuncuoglu
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Abstract

Resistive Switching Random Access Memory (RRAM) technology is critical for advancing beyond von Neumann computing applications like neuromorphic computing. Enhancing RRAM performances is contingent on carefully controlling the properties of the switching layer material, such as composition, stoichiometry, and crystal structure. This paper reports the use of a Pulsed Laser Deposition (PLD) and post-growth annealing process to create $TaO_{x}$ films with different crystal structures, and their comprehensive characterization, including structural analysis using XRD and XPS techniques, as well as electrical characterization through I-V measurements to assess switching performance. Bipolar resistive switching dynamics is demonstrated for RRAM device stacks fabricated from both as-grown and annealed TaOx films. Additionally, electroformation, set, and reset voltage device metrics of RRAM devices are reported to increase as a result of the annealing process, which enhances the crystallization of the PLD-grown $TaO_{x}$ films.
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基于氧化钽的可编程逻辑器件的性能设计
电阻开关随机存取存储器(RRAM)技术对于超越神经形态计算等冯·诺伊曼计算应用至关重要。提高RRAM性能取决于仔细控制开关层材料的性质,如组成、化学计量和晶体结构。本文报道了使用脉冲激光沉积(PLD)和生长后退火工艺制备具有不同晶体结构的$TaO_{x}$薄膜,并对其进行了全面表征,包括使用XRD和XPS技术进行结构分析,以及通过I-V测量进行电学表征以评估开关性能。双极电阻开关动力学证明了由生长和退火的TaOx薄膜制造的RRAM器件堆栈。此外,据报道,由于退火过程,RRAM器件的电形成,设置和复位电压器件指标增加,这增强了pld生长的$TaO_{x}$薄膜的结晶性。
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