Use of pure-rotational Raman scattering in measurements with a mobile Mie-Raman lidar

Y. Balin, M. Klemasheva, S. Nasonov, M. Novoselov, S. Samoilova, I. É. Penner
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Abstract

Small-sized mobile lidars mainly use single-frequency sounding with registration of elastic backscattered radiation on aerosols. Mie-Raman lidars are used to correctly reconstruct the optical characteristics of an aerosol. The method most widely used in such lidar measurements for evaluating optical properties is the method of recording vibrational Raman scattering on nitrogen molecules. The disadvantages of this method are the low backscattering cross section and the significant frequency shift of the Raman vibrational component. These problems are solved by using purely rotational Raman scattering, which is characterized by a higher backscattering cross section, and a much smaller frequency shift, which practically eliminates the dependence on the Angstrom exponent. The paper presents the practical implementation of pure-rotational Raman measurements in the mobile lidar "LOSA-A2".
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使用纯旋转拉曼散射测量与移动米-拉曼激光雷达
小型移动激光雷达主要采用单频探测,并配准气溶胶的弹性后向散射辐射。米拉曼激光雷达用于正确地重建气溶胶的光学特性。在这种激光雷达测量中,最广泛用于评估光学性质的方法是记录氮分子上的振动拉曼散射的方法。该方法的缺点是后向散射截面小,拉曼振动分量频移明显。这些问题可以通过使用纯旋转拉曼散射来解决,它的特点是具有更高的后向散射截面和更小的频移,从而消除了对埃指数的依赖。本文介绍了“LOSA-A2”移动激光雷达纯旋转拉曼测量的实际实现。
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