Enhanced Visible Light Photocatalytic Activity of g-C3N4/SiO2@TiO2 Heterojunction Fabricated by Hydrothermal Synthesis

Q4 Physics and Astronomy Defect and Diffusion Forum Pub Date : 2023-08-22 DOI:10.4028/p-b5m89a
Shota Yuge, Dang Trang Nguyen, Kozo Taguchi
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Abstract

Photocatalysts that can utilize sunlight energy have attracted attention. In this study, g-C 3 N 4 and mesoporous SiO 2 @TiO 2 particles were mixed by hydrothermal synthesis. g-C 3 N 4 was made by a simple method of directly heating melamine. Mesoporous SiO 2 @TiO 2 was prepared using the stover method. These two types of particles were then mixed by hydrothermal synthesis. Hydrothermal synthesis reduced the size of the g-C 3 N 4 particles, and they bound more closely with the TiO 2 particles. The degradation of methylene blue dye by visible light was performed to evaluate the organic degradation of the mixed particles. In addition, the mixed particles were formed into a thin film by the spin-coating method. The film's methylene blue degradation performance and the film's power generation performance in a battery were evaluated. The film showed high convenience in the practical application of photocatalytic degradation of organic pollutants because it can be easily separated from the treated liquid after organic matter degradation.
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水热合成g-C3N4/SiO2@TiO2异质结增强可见光催化活性
利用太阳光的光催化剂引起了人们的广泛关注。本研究采用水热合成法将g- c3n4与介孔sio2 @ tio2颗粒混合。采用直接加热三聚氰胺的简单方法制备了g- c3n4。采用秸秆法制备了介孔sio2 @ tio2。然后通过水热合成将这两种类型的颗粒混合。水热合成减小了g- c3n4颗粒的尺寸,使其与tio2颗粒结合更紧密。通过可见光降解亚甲基蓝染料,考察混合颗粒的有机降解效果。此外,通过旋涂法将混合颗粒形成薄膜。对膜的亚甲基蓝降解性能和膜在电池中的发电性能进行了评价。由于该膜在有机物降解后可以很容易地从处理液中分离出来,在光催化降解有机污染物的实际应用中具有很高的便利性。
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Defect and Diffusion Forum
Defect and Diffusion Forum Physics and Astronomy-Radiation
CiteScore
1.20
自引率
0.00%
发文量
127
期刊介绍: Defect and Diffusion Forum (formerly Part A of ''''Diffusion and Defect Data'''') is designed for publication of up-to-date scientific research and applied aspects in the area of formation and dissemination of defects in solid materials, including the phenomena of diffusion. In addition to the traditional topic of mass diffusion, the journal is open to papers from the area of heat transfer in solids, liquids and gases, materials and substances. All papers are peer-reviewed and edited. Members of Editorial Boards and Associate Editors are invited to submit papers for publication in “Defect and Diffusion Forum” . Authors retain the right to publish an extended and significantly updated version in another periodical.
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