Experimental measurements of X-rays emission cross sections induced by photons

IF 1.4 3区 化学 Q4 CHEMISTRY, INORGANIC & NUCLEAR Radiochimica Acta Pub Date : 2023-09-21 DOI:10.1515/ract-2023-0179
Nabila Taïbouni, Arezki Amokrane, Tarek Azli, Ben Amor Mohammed Larbi, Naima Belouadah, Khelifa Boukeffoussa, Camelia Yasmine Medour, Hamza Zouad, Mohammed Messaoudi
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Abstract

Abstract The energy-dispersive X-ray fluorescence (ED-XRF) technique has been used for measurements of K α , K β , and total K X-rays emission cross sections induced by photons, as well as K-shell fluorescence yields for pure elements with 22 ⩽ Z ⩽ 49. These metals have been irradiated at 59.54 KeV excitation energy from an 241 Am annular radioactive source. The characteristic K X-rays emitted by the targets have been detected with a Silicon drift detector (SDD); the net areas of the K α and K β spectral peaks have been determined using the fitting process of PYMCA software. The obtained experimental values of the K X-ray fluorescence cross sections and the K-shell fluorescence yields were compared to the theoretical calculated ones and also to the experimental results obtained from a different experimental setup using a point source. The obtained values were between (6.84 ± 0.55 b/at.) and (891.0 ± 67.5 b/at.) for pure metals form Scandium to Indium. Experimental values were in good agreement with theoretical values within limits of uncertainty, as well as with the data reported in the literature. Moreover, the experimental determination of K X-ray fluorescence cross-section of scandium (Sc) at 59.54 KeV has not been preceded as far as we know. The value obtained is (6.84 ± 0.55 b/at). This new result obtained maybe contribute to the enrichment of the available databases.
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光子诱导的x射线发射截面的实验测量
利用能量色散x射线荧光(ED-XRF)技术测量了光子诱导的K α、K β和总K x射线发射截面,以及纯元素的K壳层荧光产率(22≤Z≤49)。这些金属以59.54 KeV的激发能从241 Am环形放射源照射。用硅漂移检测器(SDD)检测了目标发射的特征K x射线;利用PYMCA软件对K α和K β光谱峰的净面积进行了拟合。将得到的K- x射线荧光截面和K-壳层荧光产率的实验值与理论计算值进行了比较,并与使用点源的不同实验装置获得的实验结果进行了比较。从纯金属钪到铟,得到的值在(6.84±0.55 b/at.)和(891.0±67.5 b/at.)之间。在不确定度范围内,实验值与理论值以及文献中报道的数据一致。此外,据我们所知,在59.54 KeV下钪(Sc)的K x射线荧光截面的实验测定还没有先例。得到的值为(6.84±0.55 b/at)。这一新结果可能有助于丰富现有数据库。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
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来源期刊
Radiochimica Acta
Radiochimica Acta 化学-核科学技术
CiteScore
2.90
自引率
16.70%
发文量
78
审稿时长
6 months
期刊介绍: Radiochimica Acta publishes manuscripts encompassing chemical aspects of nuclear science and technology.
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