Characteristics of air pollution variation and potential source contributions of typical megacities in the Sichuan Basin, Southwest China

IF 2.9 4区 环境科学与生态学 Q3 ENVIRONMENTAL SCIENCES Air Quality Atmosphere and Health Pub Date : 2023-11-30 DOI:10.1007/s11869-023-01466-2
Xiaoju Li, Luqman Chuah Abdullah, Shafreeza Sobri, Mohamad Syazarudin Md Said, Siti Aslina Hussain, Tan Poh Aun, Jinzhao Hu
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Abstract

Air pollution is a regional issue, influenced not only by local emission sources but also by regional transport. This study excavated the pollution variation of PM2.5 and O3 from 2014 to 2020 through statistical analysis in the megacity-Chengdu. Then, based on backward trajectory calculation and trajectory clustering, the long-term air mass transport pathways were explored, and the Potential Source Contribution Function (PSCF) model and Concentration Weighted Trajectory (CWT) analysis method were combined to further quantitatively identify the potential source areas affecting PM2.5 and O3 from an annual perspective. Finally, suggestions and measures for synergistic control of O3 and PM2.5 are put forward. The results showed that the CWT simulation results were basically consistent with the PSCF simulations, and there were significant inter-annual differences in the potential contributing source areas of pollutants. PM2.5 and O3 concentrations are not only affected by local source emissions, but regional transport (Chongqing, Lanzhou, Xi’an) is also an important source of contribution. In addition, the proportion of PM2.5 pollution trajectories decreased from 30% in 2015 to 12% in 2020, while the proportion of O3 pollution trajectories fluctuated. This study provides more detailed information on potential source regions of pollutants in typical megacities, better captures their spatial heterogeneity, and highlights the role of local sources and transboundary transport. More importantly, it also accumulated some experience for regional joint prevention and control air pollution in China’s megacities and other similar situations in the world.

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四川盆地典型特大城市大气污染变化特征及潜在污染源贡献
大气污染是一个区域性问题,不仅受到当地排放源的影响,还受到区域交通的影响。本研究通过统计分析,挖掘了2014 - 2020年特大城市成都PM2.5和O3的污染变化。然后,在反向轨迹计算和轨迹聚类的基础上,探索长期气团输送路径,并结合潜在源贡献函数(PSCF)模型和浓度加权轨迹(CWT)分析方法,进一步从年角度定量识别影响PM2.5和O3的潜在源区域。最后,提出了协同控制O3和PM2.5的建议和措施。结果表明,CWT模拟结果与PSCF模拟结果基本一致,污染物的潜在贡献源区年际差异显著。PM2.5和O3浓度不仅受局部源排放的影响,区域运输(重庆、兰州、西安)也是重要的贡献源。此外,PM2.5污染轨迹占比从2015年的30%下降到2020年的12%,而O3污染轨迹占比波动较大。本研究提供了典型特大城市潜在污染源区域的更详细信息,更好地捕捉了其空间异质性,并突出了当地污染源和跨界运输的作用。更重要的是,它也为中国特大城市大气污染区域联防联控以及世界其他类似情况积累了一些经验。图形抽象
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来源期刊
Air Quality Atmosphere and Health
Air Quality Atmosphere and Health ENVIRONMENTAL SCIENCES-
CiteScore
8.80
自引率
2.00%
发文量
146
审稿时长
>12 weeks
期刊介绍: Air Quality, Atmosphere, and Health is a multidisciplinary journal which, by its very name, illustrates the broad range of work it publishes and which focuses on atmospheric consequences of human activities and their implications for human and ecological health. It offers research papers, critical literature reviews and commentaries, as well as special issues devoted to topical subjects or themes. International in scope, the journal presents papers that inform and stimulate a global readership, as the topic addressed are global in their import. Consequently, we do not encourage submission of papers involving local data that relate to local problems. Unless they demonstrate wide applicability, these are better submitted to national or regional journals. Air Quality, Atmosphere & Health addresses such topics as acid precipitation; airborne particulate matter; air quality monitoring and management; exposure assessment; risk assessment; indoor air quality; atmospheric chemistry; atmospheric modeling and prediction; air pollution climatology; climate change and air quality; air pollution measurement; atmospheric impact assessment; forest-fire emissions; atmospheric science; greenhouse gases; health and ecological effects; clean air technology; regional and global change and satellite measurements. This journal benefits a diverse audience of researchers, public health officials and policy makers addressing problems that call for solutions based in evidence from atmospheric and exposure assessment scientists, epidemiologists, and risk assessors. Publication in the journal affords the opportunity to reach beyond defined disciplinary niches to this broader readership.
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