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Assessment of health implications of PM2.5, NO2, and SO2 exposure in Türkiye: A metropolitan and demographic-based approach (2020–2024) <s:1>基耶耶PM2.5、NO2和SO2暴露对健康影响的评估:基于大都市和人口统计学的方法(2020-2024)
IF 2.9 4区 环境科学与生态学 Q3 ENVIRONMENTAL SCIENCES Pub Date : 2026-01-30 DOI: 10.1007/s11869-026-01887-9
Kemal Ulusoy, S. Levent Kuzu, Neslihan Dogan-Saglamtimur

Air pollution causes various adverse health effects on millions of people every year. This study focused on provinces that house 65% of Türkiye’s population to analyze the trends and potential health impacts of PM2.5, NO2, and SO2. Furthermore, a 2025 health impact forecast was developed based on observed pollutant trends. The health impact assessment was structured around two key variables: population size and population density. Concurrently, trend analysis was differentiated based on the provinces’ metropolitan status. The AirQ + assessment tool identified Hatay and Düzce provinces as having the most significant health impacts. Conversely, SO2 trend analysis demonstrated higher average concentration values within non-metropolitan provinces. Over the five-year study period (2020–2024), specific mortality findings were documented. The highest PM2.5-attributed mortality was due to stroke in the 25–29 age group. In contrast, the highest NO2-attributed mortality was observed for Acute Lower Respiratory Tract Infections (ALRI) in adults aged 30 and over. Analysis revealed that the peak number of pollutant-attributed deaths occurred in 2022. The 2025 forecast offers valuable insights for future pollutant-based health impact assessments, with the outputs presented on a pollutant-oriented basis. The study concludes with various recommendations, ranging from individual protection measures to national-level investment priorities.

空气污染每年对数百万人的健康造成各种不良影响。本研究以占日本人口65%的省份为重点,分析PM2.5、二氧化氮和二氧化硫的趋势和潜在健康影响。此外,根据观察到的污染物趋势,制定了2025年健康影响预测。健康影响评估围绕两个关键变量进行:人口规模和人口密度。同时,根据各省的都市地位进行趋势分析。AirQ +评估工具确定哈塔伊省和省 zce省对健康的影响最为显著。相反,SO2趋势分析显示,非大城市省份的平均浓度较高。在五年的研究期间(2020-2024年),记录了具体的死亡率发现。在25-29岁年龄组中,pm2.5导致的死亡率最高的是中风。相比之下,在30岁及以上的成年人中,急性下呼吸道感染(ALRI)的二氧化氮死亡率最高。分析显示,污染导致的死亡人数高峰出现在2022年。2025年预测为未来基于污染物的健康影响评估提供了宝贵的见解,其产出以污染物为导向。该研究最后提出了各种建议,从个人保护措施到国家一级的投资重点。
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引用次数: 0
Spatial clustering in air quality data accuracy: assessment of low-cost sensors in Lisbon using a novel correlation-distance index 空间聚类在空气质量数据的准确性:评估低成本传感器在里斯本使用一个新的相关距离指数
IF 2.9 4区 环境科学与生态学 Q3 ENVIRONMENTAL SCIENCES Pub Date : 2026-01-29 DOI: 10.1007/s11869-026-01882-0
Sina Ataee, Myriam Lopes, Maria Isabel Nunes, Sónia Gouveia, Mohammad Vahidi Borji, Helder Relvas

Effective air quality monitoring is essential for ensuring urban environmental comfort and protecting public health, especially within smart-city frameworks. In Lisbon, the performance of low-cost NO₂ and PM10 sensors was assessed using a novel Correlation-Distance Index (CDI) coupled with Principal Component Analysis (PCA) weighting, alongside a demographic-weighted spatial association technique, benchmarked against reference monitoring stations. The analysis began by quantifying the inverse relationship between sensor–sensor correlation and Euclidean distance. This metric was then refined through the integration of PCA-derived weights and local population density, resulting in a composite CDI-PCA score assigned to each sensor. Spatial clustering of these scores identified zones of underperforming sensors, particularly in densely populated downtown and western neighborhoods. When these clusters were compared with census-block population data, there was a statistically significant association between CDI patterns and population density (χ²=406.5, p < 0.001). High-performing sensors were 22.5% more enriched in densely populated areas, indicating that demographic context provides meaningful spatial structure for network optimization, even though the modest effect size suggests the influence of multiple underlying factors. Robustness was verified through seasonal subsampling and leave-one-out cross-validation, confirming that distance-decay patterns and cluster boundaries remain consistent across environmental conditions and are not driven by individual outliers. The results demonstrate that coupling multivariate spatial statistics with demographic context supports targeted sensor calibration and redeployment strategies. Prioritizing high-population areas and dynamically adjusting sensor densities can improve real-time data accuracy and promote more equitable air quality monitoring.

有效的空气质量监测对于确保城市环境舒适和保护公众健康至关重要,特别是在智慧城市框架内。在里斯本,低成本的NO₂和PM10传感器的性能评估使用了一种新的相关距离指数(CDI),结合主成分分析(PCA)加权,以及人口加权空间关联技术,以参考监测站为基准。分析开始于量化传感器-传感器相关和欧几里得距离之间的反比关系。然后,通过整合pca衍生的权重和当地人口密度来改进该指标,从而为每个传感器分配复合CDI-PCA评分。这些分数的空间聚类确定了传感器表现不佳的区域,特别是在人口稠密的市中心和西部社区。当将这些聚类与普查块人口数据进行比较时,CDI模式与人口密度之间存在统计学上显著的关联(χ 2 =406.5, p < 0.001)。在人口密集地区,高性能传感器的丰度高出22.5%,这表明人口背景为网络优化提供了有意义的空间结构,尽管适度的效应大小表明多重潜在因素的影响。鲁棒性通过季节性子抽样和留一交叉验证验证,确认距离衰减模式和集群边界在各种环境条件下保持一致,而不是由个别异常值驱动。结果表明,将多元空间统计与人口背景相结合,可以支持有针对性的传感器校准和重新部署策略。优先考虑人口密集地区和动态调整传感器密度可以提高实时数据的准确性,促进更公平的空气质量监测。
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引用次数: 0
Research on the coordinated development of regional energy-economy-environment-carbon coupling systems 区域能源-经济-环境-碳耦合系统协调发展研究
IF 2.9 4区 环境科学与生态学 Q3 ENVIRONMENTAL SCIENCES Pub Date : 2026-01-28 DOI: 10.1007/s11869-026-01895-9
Yang Wei, Han Zhang, Yumin Chen, Zhengwei Chang, Jie Zhang

With the accelerated pace of industrialization, energy demand continues to increase, exacerbating the contradictions between economic development and environmental protection. Rising carbon emissions have posed serious challenges to ecosystems. Achieving coordinated development among energy, economy, environment, and carbon emissions is therefore essential for regional sustainable development. Accordingly, this study investigates the coordinated development within the regional energy-economy-environment-carbon (EEEC) coupling system. Firstly, this research integrates energy consumption, economic industrial structure, ecological environmental quality, and carbon emission levels into a unified analytical framework, thereby developing an EEEC coupling system. Secondly, a coupling coordination model is employed to quantitatively assess the level of coordinated development within the regional EEEC system. Then, an optimization model aiming at maximizing the coupling coordination degree is established. This model comprehensively considers multiple constraints, such as economic and energy factors, facilitating the optimization of industrial structures and exploration of sustainable development pathways. Lastly, the developed model is empirically applied to Southwest China to verify its effectiveness. The main findings of this study are as follows: (1) Energy carbon emissions in the Southwest region show an overall upward trend. Electricity is the largest contributor to energy carbon emissions in the region, followed by raw coal, with carbon emission volumes of 76100.59 (({10^8}kgC{O_2}eq)) and 31942.16 (({10^8}kgC{O_2}eq)), respectively. (2) The coupling coordination degree of the Energy-Economy-Environment-Carbon system presents a gradually rising trend. In 2022, the coupling coordination degree across various regions was approximately 0.7; however, it remains in the intermediate coordination stage, indicating that the overall synergy level of the system still has room for further optimization. (3) Industry still holds a relatively large proportion in the industrial structure of various regions. The structures of agriculture, the construction industry, and other industries have improved, with average increases of 0.08%, 0.12%, and 9.88%, respectively.

随着工业化步伐的加快,能源需求不断增加,加剧了经济发展与环境保护之间的矛盾。不断上升的碳排放对生态系统构成了严重挑战。实现能源、经济、环境、碳排放协调发展,是区域可持续发展的必然要求。据此,本研究对区域能源-经济-环境-碳耦合系统内的协调发展进行了研究。首先,本研究将能源消耗、经济产业结构、生态环境质量、碳排放水平整合到一个统一的分析框架中,构建EEEC耦合体系。其次,采用耦合协调模型定量评价区域经济共同体系统内的协调发展水平。然后,建立了以耦合协调度最大化为目标的优化模型。该模型综合考虑了经济、能源等多重约束因素,有利于优化产业结构,探索可持续发展路径。最后,以西南地区为例,验证了模型的有效性。研究结果表明:①西南地区能源碳排放总体呈上升趋势;电力是该地区能源碳排放的最大贡献者,其次是原煤,碳排放量分别为76100.59 (({10^8}kgC{O_2}eq))和31942.16 (({10^8}kgC{O_2}eq))。(2)能源-经济-环境-碳系统的耦合协调度呈逐渐上升的趋势。2022年,各区域间的耦合协调度约为0.7;但仍处于中间协调阶段,说明系统整体协同水平仍有进一步优化的空间。(3)工业在各地区产业结构中的比重仍然较大。农业、建筑业等行业结构优化,平均增长0.08个百分点%, 0.12%, and 9.88%, respectively.
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引用次数: 0
Urban morphology and air quality: microclimatic simulation of PM2.5 and NO₂ dispersion in urban canyons scale 城市形态与空气质量:城市峡谷尺度下PM2.5和NO 2弥散的小气候模拟
IF 2.9 4区 环境科学与生态学 Q3 ENVIRONMENTAL SCIENCES Pub Date : 2026-01-28 DOI: 10.1007/s11869-026-01884-y
Carolina Girotti, Alessandra R. Prata Shimomura, António Lopes

Air pollution in megacities such as São Paulo is one of the major public health challenges, with fine particulate matter (PM2.5) and nitrogen dioxide (NO₂) among the most critical air pollutants due to their respiratory and cardiovascular effects. Intensified land use along the Urban Structuring Axes (EETU), a strategy within transit-oriented development, has promoted densification and verticalization, altering the urban microclimate and pollutant dispersion. This study analyzed how different urban morphological configurations influence the dispersion of PM2.5 and NO₂ in street canyons along the EETU in São Paulo city, considering the interaction between built form and street trees. The ENVI-met microclimatic model, based on Computational Fluid Dynamics (CFD), was used to simulate pollutant concentration and dispersion in five street canyons representative of distinct urban morphologies. Indicators such as urban density, verticality (average building height), H/W ratio, occupation, directionality (building orientation relative to prevailing winds), and Normalized Difference Vegetation Index (NDVI) were applied to characterize each area. Results show that compact and highly occupied urban forms exhibit substantially higher NO₂ concentrations at pedestrian level, with differences of up to ~ 80% between contrasting urban morphologies. In contrast, PM2.5 concentrations vary only modestly between canyons (< 5% variation), remaining close to urban background levels. PM2.5 deposition mass, however, shows pronounced sensitivity to urban form and vegetation, varying by over 60% between canyons, indicating that deposition responds differently from pollutant concentration. Urban form therefore plays a key role in shaping ventilation efficiency and air quality in dense areas of São Paulo. Strategies that combine building height variation, transversal block openings, orientation relative to prevailing winds, and context-sensitive street-tree management are essential to reduce population exposure to air pollution in compact urban environments.

圣保罗这样的大城市的空气污染是主要的公共卫生挑战之一,细颗粒物(PM2.5)和二氧化氮(NO₂)是最重要的空气污染物,因为它们对呼吸和心血管有影响。城市结构轴(EETU)沿线的集约化土地利用是交通导向发展的一种战略,促进了高密度化和垂直化,改变了城市小气候和污染物的扩散。考虑建筑形态与行道树之间的相互作用,本研究分析了圣保罗市EETU沿线街道峡谷中不同的城市形态配置对PM2.5和NO₂扩散的影响。采用基于计算流体动力学(CFD)的ENVI-met微气候模型,模拟了五个具有不同城市形态代表的街道峡谷的污染物浓度和扩散。利用城市密度、垂直度(建筑平均高度)、H/W比、占用、方向性(建筑相对于盛行风的朝向)和归一化植被指数(NDVI)等指标来描述每个地区。结果表明,紧凑和高度占用的城市形态在行人水平上表现出更高的NO₂浓度,不同城市形态之间的差异高达80%。相比之下,PM2.5浓度在峡谷之间的差异很小(5%的差异),仍然接近城市背景水平。然而,PM2.5沉积质量对城市形态和植被表现出明显的敏感性,峡谷之间的差异超过60%,表明沉积响应与污染物浓度不同。因此,城市形态在塑造圣保罗人口密集地区的通风效率和空气质量方面起着关键作用。结合建筑高度变化、横向街区开口、相对于盛行风的朝向和上下文敏感的街道树木管理的策略对于减少人口暴露于紧凑城市环境中的空气污染至关重要。
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引用次数: 0
How does artificial intelligence influence infant mortality?: a cross-country analysis (2000–2023) 人工智能如何影响婴儿死亡率?:跨国分析(2000-2023)
IF 2.9 4区 环境科学与生态学 Q3 ENVIRONMENTAL SCIENCES Pub Date : 2026-01-28 DOI: 10.1007/s11869-026-01896-8
Partha Acharjee, Debasis Neogi, Sauvik Chakraborty

This study examines the effect of Artificial Intelligence (AI) on infant mortality rates (IMR) across 102 countries from 2000 to 2023, considering the moderating roles of governance quality (GQI), digital infrastructure (DII), and medical infrastructure (MII). Grounded in the Health Production Function, Institutional, Technological Systems and Absorptive Capacity theories, the study explores how institutional, technological and healthcare readiness influence AI’s effectiveness in improving healthcare outcomes. Multiple estimation techniques, such as Pooled Ordinary Least Squares (POLS), Fully Modified Ordinary Least Squares (FMOLS), Driscoll–Kraay Standard Errors (DKSE), Two-Stage Least Squares (2SLS), and Method of Moments Quantile Regression (MMQR), were employed to address heterogeneity and endogeneity concerns. Results across all estimators are consistent and show that AI significantly reduces IMR by enhancing diagnostic precision, healthcare resource allocation, and data-driven decision-making. The moderating effects of GQI, DII, and MII are negative and significant, suggesting that strong governance, robust digital networks, and advanced medical systems amplify the effectiveness of AI. Quantile regression results indicate heterogeneous effects, with stronger impacts in technologically advanced and low-mortality contexts, and weaker impacts where structural constraints exist. Subsample analysis reveals that AI reduces IMR in both developing and developed economies, but the effect is greater in the latter due to institutional maturity. Overall, the study highlights that AI’s transformative potential in reducing infant mortality depends critically on governance capacity, digital readiness, and healthcare system strength.

本研究考察了2000年至2023年102个国家的人工智能(AI)对婴儿死亡率(IMR)的影响,并考虑了治理质量(GQI)、数字基础设施(DII)和医疗基础设施(MII)的调节作用。该研究以卫生生产函数、制度、技术系统和吸收能力理论为基础,探讨了制度、技术和卫生保健准备如何影响人工智能在改善卫生保健结果方面的有效性。多重估计技术,如池普通最小二乘法(POLS)、完全修正普通最小二乘法(FMOLS)、Driscoll-Kraay标准误差(DKSE)、两阶段最小二乘法(2SLS)和矩分位数回归法(MMQR),被用来解决异质性和内质性问题。所有估算器的结果都是一致的,并且表明人工智能通过提高诊断精度、医疗保健资源分配和数据驱动的决策,显著降低了IMR。GQI、DII和MII的调节作用是负面且显著的,这表明强有力的治理、稳健的数字网络和先进的医疗系统放大了人工智能的有效性。分位数回归结果显示了异质性效应,在技术先进和死亡率低的情况下,影响更大,而在存在结构限制的情况下,影响更弱。子样本分析显示,人工智能降低了发展中经济体和发达经济体的综合综合税收,但由于制度成熟度的原因,后者的影响更大。总体而言,该研究强调,人工智能在降低婴儿死亡率方面的变革潜力在很大程度上取决于治理能力、数字化准备程度和医疗保健系统的实力。
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引用次数: 0
Impact of forest fire on surface black carbon concentration over Mizoram, North-east India 印度东北部米佐拉姆邦森林火灾对地表黑碳浓度的影响
IF 2.9 4区 环境科学与生态学 Q3 ENVIRONMENTAL SCIENCES Pub Date : 2026-01-26 DOI: 10.1007/s11869-026-01889-7
Arundhati Kundu, Shyam S. Kundu, Arup Borgohain, Arban S. Youroi, Rahul Mahanta, Mukunda M. Gogoi, S. Suresh Babu, Kasturi Chakraborty

In order to understand the influence of forest fires on one of the critical pollutants impacting air quality over a hilly station, this study was undertaken utilizing integrated observation from in-situ station, satellites and reanalysis data. Black Carbon (BC) surface mass concentration was measured over Mizoram, the southernmost state of North east India (NEI) for the first time during 4th March − 3rd April 2022 under a campaign mode. Mean BC during the study period was 6.18 ± 3.1 µg/m3 that varied between a daily mean of 2.43 ± 0.41 µg/m3 to 12.87 ± 2.12 µg/m3. Reanalysis data is found as not sufficiently representative for this region as MERRA-2 reanalysis significantly overestimated BC (~ 4 times than the observed mean) over Mizoram during the fire active period while underestimated during other times. The possibilities of long range transport increasing the BC load over Mizoram was found limited during the study period. An average absorption Ångström exponent (AAE) of 1.22 ± 0.1 suggests dominant influence of biomass burning, consistent with flaming combustion of local and regional wood sources. Higher forest fire activity within 250 km of the station coincided with increased BC levels and implicated forest fire as dominant BC emission source during this season. CALIPSO Lidar observations detected an elevated smoke layer at 4.5–5 km AMSL, indicating fire induced convective activities, which was gradually replaced by dust and polluted dust as the season advanced. This study highlights the importance of long-term in-situ measurements of aerosols over fragile ecosystems like the NEI.

为了了解森林火灾对影响山地站点空气质量的关键污染物之一的影响,本研究利用了原位站、卫星和再分析数据的综合观测。在2022年3月4日至4月3日期间,首次在印度东北部(NEI)最南端的米佐拉姆邦(Mizoram)进行了黑碳(BC)表面质量浓度的测量。研究期间的平均BC为6.18±3.1µg/m3,每日平均值为2.43±0.41µg/m3至12.87±2.12µg/m3。再分析数据不能充分代表该地区,因为MERRA-2再分析在火灾活跃期显著高估了米佐拉姆邦的BC(约为观测平均值的4倍),而在其他时间则低估了BC。在研究期间,发现长距离运输增加米佐拉姆邦BC负荷的可能性有限。平均吸收Ångström指数(AAE)为1.22±0.1,表明生物质燃烧的影响占主导地位,与当地和区域木材源的火焰燃烧一致。该站250公里范围内的森林火灾活动增加与BC水平增加相吻合,表明森林火灾是本季节主要的BC排放源。CALIPSO激光雷达观测到4.5 ~ 5 km AMSL处有升高的烟雾层,表明火引起的对流活动,随着季节的推进,逐渐被沙尘和污染沙尘所取代。这项研究强调了在像NEI这样脆弱的生态系统上对气溶胶进行长期原位测量的重要性。
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引用次数: 0
An overview of CO2 level as an infection risk proxy for different indoor environments in Istanbul 伊斯坦布尔不同室内环境中二氧化碳水平作为感染风险指标的概述
IF 2.9 4区 环境科学与生态学 Q3 ENVIRONMENTAL SCIENCES Pub Date : 2026-01-24 DOI: 10.1007/s11869-026-01903-y
Coşkun Ayvaz, Ülkü Alver Şahin, Ecem Yıldız, Şule Demirci, Kezban Özcan, Burcu Uzun Ayvaz, Dila Aydın Aytekin, Burcu Onat, Nüket Sivri

Indoor CO₂ concentration is widely recognized as an effective proxy for infection risk and ventilation efficiency. In addition to improving indoor air quality, the necessity of performing indoor ventilation correctly, effectively, and efficiently to prevent or minimize the spread of SARS-CoV-2 has gained even more importance during the COVID-19 pandemic. In this study, carbon dioxide (CO2), fine particulate matter (PM2.5,) temperature, and humidity were monitored in sixteen different indoor environments belonging to four categories: markets, restaurants, public transportation (Metrobus), and shopping centers in Istanbul, Türkiye, during March and April 2021. Measurements were conducted using calibrated low-cost sensors (± 30 ppm accuracy for CO2) that recorded data every 20 s for 15 min on four different days. The lowest variation in CO2 measurements was observed in shopping centers (533–663 ppm), while the highest was in restaurants (532–974 ppm). Humidity, temperature, and PM2.5 values were also recorded and discussed. Results indicate that restaurants exhibited the highest CO2 based infection risk due to limited or natural ventilation, whereas shopping centers with central mechanical ventilation maintained CO2 concentrations below 650 ppm, indicating low risk. Ventilation management through continuous CO2 monitoring is emphasized as a crucial strategy for controlling epidemic risks indoors. Recommendations include improving ventilation efficiency, using portable air cleaners with HEPA/UV filters, and visually displaying CO2 levels via a “traffic-light” system to inform occupants about indoor safety. This study provides the first quantitative comparison of CO2-based infection risk across multiple indoor environments in Istanbul, providing baseline data for future research and public health policies.

室内CO₂浓度被广泛认为是感染风险和通风效率的有效指标。除了改善室内空气质量外,正确、有效和高效地进行室内通风以防止或尽量减少SARS-CoV-2的传播的必要性在COVID-19大流行期间变得更加重要。在这项研究中,二氧化碳(CO2)、细颗粒物(PM2.5)、温度和湿度在16个不同的室内环境中进行了监测,这些环境属于4类:市场、餐馆、公共交通(地铁)和购物中心,时间为2021年3月和4月。测量使用校准过的低成本传感器(CO2精度为±30 ppm),在4个不同的日子里每20秒记录15分钟的数据。二氧化碳测量值变化最小的是购物中心(533-663 ppm),而最高的是餐馆(532-974 ppm)。还记录和讨论了湿度、温度和PM2.5值。结果表明,由于有限通风或自然通风,餐馆的CO2感染风险最高,而中央机械通风的购物中心的CO2浓度维持在650 ppm以下,表明风险较低。强调通过持续监测CO2进行通风管理是控制室内疫情风险的关键策略。建议包括提高通风效率,使用带有HEPA/UV过滤器的便携式空气净化器,以及通过“红绿灯”系统直观显示二氧化碳水平,以告知居住者室内安全。该研究首次对伊斯坦布尔多个室内环境中基于二氧化碳的感染风险进行了定量比较,为未来的研究和公共卫生政策提供了基线数据。
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引用次数: 0
The associations of maternal exposure to black carbon and foetal growth risks in Southern Sweden 瑞典南部产妇接触黑碳与胎儿生长风险的关系
IF 2.9 4区 环境科学与生态学 Q3 ENVIRONMENTAL SCIENCES Pub Date : 2026-01-23 DOI: 10.1007/s11869-026-01890-0
Kajsa Pira, Cale Lawlor, Tanya Andersson Nystedt, Anna Oudin, Ralf Rittner, Jiawei Zhang, Rina So, Marie Bergmann, Youn-Hee Lim, Zorana J. Andersen, Ebba Malmqvist

Black carbon (BC) is an air pollutant of emerging concern, and further evidence is needed to understand its health effects. This study investigates the association between gestational BC exposure and birth outcomes, and whether these effects are independent of particulate matter with an aerodynamic diameter of ≤ 2.5 μm (PM2.5) exposure. We used data from the population-based birth cohort, Maternal Air Pollution in Southern Sweden (MAPSS) for the years 2000–2009, including 43,676 mother-child pairs. Maternal exposure to air pollution at residential address was estimated using a high-resolution dispersion model. We used logistic and linear regressions to examine association of air pollution with birth outcomes adjusting for maternal age, Body Mass Index, smoking, education, maternal country of birth, sex of the child, parity, household income, and birth year. We found that BC exposure during pregnancy was associated with birth weight (decrease of 69 g per 1 µg/m³ (95% Confidence Interval (CI): -96, -42) and small for gestational age (SGA) (odds ratio (OR) of 1.29 (95% CI: 1.05, 1.59; p = 0.015) per 1 µg/m³ increase in BC). BC exposure during the second trimester (OR of 1.79 (95% CI: 1.03, 3.09) and PM2.5 during pregnancy (OR of 1.06 (95% CI: 1.01,1.12) were associated with Low Birth Weight (LBW). Associations with BC remained after adjustment for PM2.5. Our study contributes to further evidence of birth weight impact from BC exposure to an emerging pollutant of concern, even in a low-exposure environment. Further, we demonstrate effects of PM2.5, but also differentiate independent effects of these two correlated pollutants.

黑碳(BC)是一种日益受到关注的空气污染物,需要进一步的证据来了解其对健康的影响。本研究探讨了妊娠期BC暴露与出生结局之间的关系,以及这些影响是否与空气动力学直径≤2.5 μm (PM2.5)暴露的颗粒物无关。我们使用了2000-2009年瑞典南部孕产妇空气污染(MAPSS)基于人口的出生队列数据,包括43,676对母子。使用高分辨率弥散模型估计孕产妇在居住地址的空气污染暴露。我们使用逻辑回归和线性回归来检验空气污染与出生结果的关系,调整了产妇年龄、体重指数、吸烟、教育程度、产妇出生国家、儿童性别、胎次、家庭收入和出生年份。我们发现妊娠期接触BC与出生体重相关(每1 μ g/m³减少69 g(95%可信区间(CI): -96, -42),胎龄较小(SGA)(优势比(OR)为1.29 (95% CI: 1.05, 1.59; p = 0.015))。妊娠中期暴露于BC (OR为1.79 (95% CI: 1.03, 3.09)和妊娠期间暴露于PM2.5 (OR为1.06 (95% CI: 1.01,1.12)与低出生体重(LBW)相关。在调整PM2.5后,与BC的相关性仍然存在。我们的研究进一步证明,即使在低暴露环境中,BC暴露于一种新兴的污染物也会影响出生体重。此外,我们论证了PM2.5的影响,但也区分了这两种相关污染物的独立影响。
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引用次数: 0
Spatiotemporal characteristics and driving factors of air pollution islands in Urumqi of China during heating and non-heating periods 乌鲁木齐采暖期与非采暖期空气污染岛时空特征及驱动因素分析
IF 2.9 4区 环境科学与生态学 Q3 ENVIRONMENTAL SCIENCES Pub Date : 2026-01-23 DOI: 10.1007/s11869-026-01900-1
Yi Han, Xuegang Chen, Yunyao Feng, Siqi Xie

This study investigates the spatiotemporal patterns and driving mechanisms of urban pollution islands (UPI) in Urumqi, a representative arid city in northwestern China, during heating and non-heating periods. Using PM₂.₅ monitoring data (2017–2023) from national control stations in urban and suburban areas combined with meteorological and pollution factors, we developed the Urban Pollution Island Intensity (UPII) and applied Pearson correlation analysis and principal component analysis (PCA) to systematically examine the spatiotemporal evolution and dominant drivers of UPI. Results reveal significant temporal differences in UPII intensity, with the heating period average (105 µg/m³) being 4.2 times higher than the non-heating period (25 µg/m³), highlighting the synergistic effect of coal-fired heating and unfavorable diffusion conditions. Spatially, a “northern rural > urban > southern rural” gradient was observed. During heating periods, UPIIN was more prominent due to industrial agglomeration and topographic blocking, while higher UPIIS during non-heating periods suggested regional transport. A “temporal shift” in pollution formation mechanisms was identified: non-heating periods were meteorologically dominated (e.g., temperature showed significant negative correlation with UPIIS, r = -0.480, p < 0.01), while heating periods exhibited strong emission-driven patterns, with PCA indicating the first principal component explained 41.2% of variance, mainly loaded by coal-combustion pollutants including SO2, CO, and PM10. The UPII index effectively distinguished between local emissions and regional transport contributions, further validated by the sharp UPII decline during COVID-19 lockdowns. This study proposes a “period-subarea-category” precision governance strategy to inform air pollution control in arid northwestern cities.

以乌鲁木齐市为例,研究了采暖期和非采暖期城市污染岛(UPI)的时空格局及其驱动机制。使用点₂。根据2017-2023年城市和郊区国家控制站的监测数据,结合气象和污染因素,我们开发了城市污染岛强度(UPII),并应用Pearson相关分析和主成分分析(PCA)系统地研究了UPI的时空演变和主导驱动因素。结果显示,UPII强度在时间上存在显著差异,供热期平均值(105µg/m³)是非供热期平均值(25µg/m³)的4.2倍,凸显了燃煤供热的协同效应和不利的扩散条件。空间上呈现“北部农村&城市&南部农村”梯度。在采暖期,由于产业集聚和地形阻塞,UPIIS更为突出,而在非采暖期,UPIIS较高表明区域运输。发现了污染形成机制的“时间转移”:非供暖期以气象因素为主(例如,温度与UPIIS呈显著负相关,r = -0.480, p < 0.01),而供暖期则表现出强烈的排放驱动模式,主成分分析表明,第一主成分解释了41.2%的方差,主要是燃煤污染物,包括SO2、CO和PM10。UPII指数有效区分了地方排放和区域运输贡献,这一点在COVID-19封城期间的UPII急剧下降进一步得到了验证。本研究提出了“时期-分区-分类”的精准治理策略,为西北干旱城市大气污染治理提供参考。
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引用次数: 0
Seasonal and meteorological influences on atmospheric piperazine and its nitrosated derivatives in fine and coarse particulate matter in an urban-industrial environment 城市-工业环境中大气细、粗颗粒物中哌嗪及其亚硝化衍生物的季节和气象影响
IF 2.9 4区 环境科学与生态学 Q3 ENVIRONMENTAL SCIENCES Pub Date : 2026-01-23 DOI: 10.1007/s11869-026-01891-z
Berrin Gürler Akyüz, Mehmet Akyüz

This study investigates the seasonal occurrence, sources and transformation mechanisms of piperazine and its nitrosated derivatives, mononitrosopiperazine and dinitrosopiperazine, alongside nitrate and nitrite in fine and coarse particulate matter in order to evaluate the influence of emissions and meteorological conditions. All target compounds exhibited significantly higher concentrations during the heating season, reflecting increased combustion activities as well as atmospheric conditions conducive to pollutant accumulation and secondary formation. The concentrations of fine and coarse particulates exhibited a highly significant correlation, suggesting the presence of shared sources, particularly residential and industrial heating, during the winter months. The secondary formation of mononitrosopiperazine and dinitrosopiperazine was a consequence of the atmospheric nitrosation of piperazine in the presence of nitrite. The formation of these compounds was found to be favoured by the following conditions: cold weather, stagnant conditions and low solar radiation. The dinitrosopiperazine exhibited a significant correlation with nitrite and nitrate, while demonstrating an inverse relationship with temperature and insolation, thereby supporting its secondary formation. However, a negative correlation was observed between relative humidity and mononitrosopiperazine, dinitrosopiperazine, nitrite, and nitrate, indicating enhanced scavenging or dilution processes. Principal component analysis (PCA) differentiated primary piperazine emissions from secondary nitrosamine formation, thereby reinforcing the role of NOx-related chemistry. ANOVA analysis was also performed to back up the findings from seasonal concentration trends, correlation analysis and PCA, and to provide a consistent understanding of their behavior, sources and atmospheric dynamics. The findings under consideration demonstrate the combined effects of precursor availability, emission strength, and meteorology on reactive nitrogen compounds and nitrosamines.

本研究考察了哌嗪及其亚硝化衍生物单硝基哌嗪和二硝基哌嗪,以及硝酸盐和亚硝酸盐在细颗粒物和粗颗粒物中的季节分布、来源和转化机制,以评价排放和气象条件的影响。在采暖季,所有目标化合物的浓度都显著升高,反映了燃烧活动的增加以及有利于污染物积累和二次形成的大气条件。细颗粒物和粗颗粒物的浓度表现出高度显著的相关性,表明在冬季存在共同的来源,特别是住宅和工业供暖。单硝基哌嗪和二硝基哌嗪的二次生成是哌嗪在亚硝酸盐存在下大气亚硝化的结果。这些化合物的形成被发现在以下条件下是有利的:寒冷的天气,停滞的条件和低太阳辐射。二硝基哌嗪与亚硝酸盐和硝酸盐呈显著相关,而与温度和日照呈反比关系,从而支持其二次生成。然而,相对湿度与单硝基哌嗪、二硝基哌嗪、亚硝酸盐和硝酸盐之间呈负相关,表明清除或稀释过程增强。主成分分析(PCA)将一次哌嗪排放与二次亚硝胺形成区分开来,从而加强了nox相关化学的作用。还进行了方差分析,以支持季节性浓度趋势、相关分析和主成分分析的发现,并提供对其行为、来源和大气动力学的一致理解。正在考虑的研究结果表明,前体可利用性、排放强度和气象学对活性氮化合物和亚硝胺的综合影响。
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引用次数: 0
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Air Quality Atmosphere and Health
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