Ultrafast pulse generation via magnetic topological insulator MnBi2Te4 nanosheets

Haiqin Deng, Qiang Yu, Zixin Yang, Jian Wu, Pu Zhou
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Abstract

Recently, 2D layered MnBi2Te4 has been a promising candidate for discovering the exotic topological quantum phenomena for the coexisting topology and magnetism. In particular, the layered structure of MnBi2Te4 with a small bandgap possesses excellent ultrafast nonlinear response and broadband saturable absorption, which indicates that they can be applied in the field of ultrafast photonics. Despite tremendous research on magnetism and topology, the nonlinear optical properties of MnBi2Te4 have been underexplored. Herein, we have successfully synthesized the high-quality MnBi2Te4 by the self-flux method. By using MnBi2Te4 nanosheets as a saturable absorber (SA), a passive mode-locking erbium-doped fiber (EDF) laser centered at 1560 nm was obtained with a pulse duration of 331 fs. This work suggests that magnetic topological insulators possess great potential for ultrafast photonics.
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通过磁性拓扑绝缘体 MnBi2Te4 纳米片生成超快脉冲
最近,二维层状 MnBi2Te4 已成为发现拓扑与磁性共存的奇异拓扑量子现象的有望候选材料。尤其是具有小带隙的层状 MnBi2Te4 结构具有优异的超快非线性响应和宽带可饱和吸收,这表明它们可以应用于超快光子学领域。尽管在磁学和拓扑学方面有大量研究,但对锰铋碲 4 的非线性光学特性的探索还很不够。在此,我们采用自流变方法成功合成了高质量的 MnBi2Te4。通过使用 MnBi2Te4 纳米片作为可饱和吸收体(SA),我们获得了中心波长为 1560 nm、脉冲持续时间为 331 fs 的无源锁模掺铒光纤(EDF)激光器。这项工作表明,磁性拓扑绝缘体在超快光子学方面具有巨大潜力。
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