One-step liquid-phase synthesis of platinum nanocatalysts supported on carbon fiber substrates and their electrochemical characterization

IF 1.5 4区 物理与天体物理 Q3 PHYSICS, APPLIED Japanese Journal of Applied Physics Pub Date : 2024-01-04 DOI:10.35848/1347-4065/ad1006
Kiyofumi Yamagiwa, Kyohei Kamimura, Yuuri Kimura
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Abstract

Highly dispersed Pt nanoparticles supported on polyacrylonitrile-based carbon fiber substrates were prepared using a one-step liquid-phase process. Nanoparticles were grown on the fiber surface via electric resistance heating of the substrate in ethanol solutions containing a platinum-based organometallic complex as the nanoparticle precursor. After the synthesis, Pt nanoparticles were formed on the surface in highly dispersed states. Electrochemical characterization of the Pt nanoparticles was conducted using the substrates directly after synthesis. The Pt nanoparticles were electrochemically active and exhibited superior methanol oxidation properties.
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碳纤维基底上支持的铂纳米催化剂的一步液相合成及其电化学表征
采用一步液相法制备了支撑在聚丙烯腈基碳纤维基底上的高度分散铂纳米粒子。在含有铂基有机金属复合物作为纳米粒子前体的乙醇溶液中,通过电阻加热基底,在纤维表面生长出纳米粒子。合成完成后,铂纳米粒子以高度分散的状态在纤维表面形成。铂纳米粒子合成后直接使用基底进行了电化学表征。铂纳米粒子具有电化学活性,并表现出优异的甲醇氧化性能。
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来源期刊
Japanese Journal of Applied Physics
Japanese Journal of Applied Physics 物理-物理:应用
CiteScore
3.00
自引率
26.70%
发文量
818
审稿时长
3.5 months
期刊介绍: The Japanese Journal of Applied Physics (JJAP) is an international journal for the advancement and dissemination of knowledge in all fields of applied physics. JJAP is a sister journal of the Applied Physics Express (APEX) and is published by IOP Publishing Ltd on behalf of the Japan Society of Applied Physics (JSAP). JJAP publishes articles that significantly contribute to the advancements in the applications of physical principles as well as in the understanding of physics in view of particular applications in mind. Subjects covered by JJAP include the following fields: • Semiconductors, dielectrics, and organic materials • Photonics, quantum electronics, optics, and spectroscopy • Spintronics, superconductivity, and strongly correlated materials • Device physics including quantum information processing • Physics-based circuits and systems • Nanoscale science and technology • Crystal growth, surfaces, interfaces, thin films, and bulk materials • Plasmas, applied atomic and molecular physics, and applied nuclear physics • Device processing, fabrication and measurement technologies, and instrumentation • Cross-disciplinary areas such as bioelectronics/photonics, biosensing, environmental/energy technologies, and MEMS
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