Convective Drying of Porous Media: Comparison of Phase-Field Simulations with Microfluidic Experiments

IF 2.7 3区 工程技术 Q3 ENGINEERING, CHEMICAL Transport in Porous Media Pub Date : 2024-01-23 DOI:10.1007/s11242-023-02051-y
Lukas Maier, Sebastian Brosch, Magnus Gaehr, John Linkhorst, Matthias Wessling, Ulrich Nieken
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Abstract

Convective drying of porous media is central to many engineering applications, ranging from spray drying over water management in fuel cells to food drying. To improve these processes, a deep understanding of drying phenomena in porous media is crucial. Therefore, detailed simulation of multiphase flows with phase change is of great importance to investigate the complex processes involved in drying porous media. While many studies aim to access the phenomena solely by simulations, here we succeed to compare comprehensively simulations with an experimental methodology based on microfluidic multiphase flow studies in engineered porous media. In this contribution, we propose a Navier–Stokes Cahn–Hilliard model coupled with balance equations for heat and moisture to simulate the two-phase flow with phase change. The phase distribution of the two fluids air and water is modeled by the Phase-Field equation. Comparisons with experiments are rare in the literature and usually involve very simple cases. We compare our simulation with convective drying experiments of porous media. Experimentally, the interface propagation of the water–air interface was visualized in detail during drying in a structured microfluidic cell made from PDMS. The drying pattern and the drying time in the experiment are very well reproduced by our simulation. This validation will enable the application for the presented Navier–Stokes Cahn–Hilliard model in more complex cases focused more on applications, e.g., in the field of fibrous materials.

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多孔介质的对流干燥:相场模拟与微流控实验的比较
摘要 多孔介质的对流干燥是许多工程应用的核心,从燃料电池中水管理的喷雾干燥到食品干燥,不一而足。要改进这些过程,深入了解多孔介质中的干燥现象至关重要。因此,相变多相流的详细模拟对于研究多孔介质干燥的复杂过程非常重要。虽然许多研究的目的仅仅是通过模拟来了解这些现象,但在这里,我们成功地将模拟与基于工程多孔介质中微流体多相流研究的实验方法进行了全面比较。在这篇论文中,我们提出了一个纳维-斯托克斯-卡恩-希利亚德模型,并结合热量和水分平衡方程来模拟相变的两相流动。空气和水两种流体的相分布由相场方程建模。与实验的比较在文献中很少见,通常涉及非常简单的情况。我们将模拟结果与多孔介质的对流干燥实验进行了比较。实验中,我们详细观察了水-空气界面在由 PDMS 制成的结构化微流池内干燥过程中的界面传播。我们的模拟很好地再现了实验中的干燥模式和干燥时间。这一验证将使我们提出的 Navier-Stokes Cahn-Hilliard 模型能够应用于更复杂的情况,如纤维材料领域。
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来源期刊
Transport in Porous Media
Transport in Porous Media 工程技术-工程:化工
CiteScore
5.30
自引率
7.40%
发文量
155
审稿时长
4.2 months
期刊介绍: -Publishes original research on physical, chemical, and biological aspects of transport in porous media- Papers on porous media research may originate in various areas of physics, chemistry, biology, natural or materials science, and engineering (chemical, civil, agricultural, petroleum, environmental, electrical, and mechanical engineering)- Emphasizes theory, (numerical) modelling, laboratory work, and non-routine applications- Publishes work of a fundamental nature, of interest to a wide readership, that provides novel insight into porous media processes- Expanded in 2007 from 12 to 15 issues per year. Transport in Porous Media publishes original research on physical and chemical aspects of transport phenomena in rigid and deformable porous media. These phenomena, occurring in single and multiphase flow in porous domains, can be governed by extensive quantities such as mass of a fluid phase, mass of component of a phase, momentum, or energy. Moreover, porous medium deformations can be induced by the transport phenomena, by chemical and electro-chemical activities such as swelling, or by external loading through forces and displacements. These porous media phenomena may be studied by researchers from various areas of physics, chemistry, biology, natural or materials science, and engineering (chemical, civil, agricultural, petroleum, environmental, electrical, and mechanical engineering).
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