Selective detection of Fe3+ by Ag2S QDs and construction of the IMPLICATION gate

IF 5.4 Q1 CHEMISTRY, ANALYTICAL Sensing and Bio-Sensing Research Pub Date : 2024-02-01 DOI:10.1016/j.sbsr.2024.100624
Lijun Liu , Lu Ga , Jun Ai
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Abstract

Several studies have demonstrated that Ag2S QDs are promising near-infrared II-emitting nanoprobes. They Ag2S QDs can be used in the fields of bio-imaging, fluorescence detection and photodetectors. In this work, we achieved the first successful construction of a dual-input logic gate IMPLICATION gate based on the specific detection of Fe3+ by silver sulfide quantum dots and the reduction of Fe3+ by ascorbic acid. The Ag2S QDs were successfully prepared from glutathione and silver nitrate and characterized by fluorescence spectroscopy analysis, XPS analysis, and transmission electron microscopy TEM analysis. The prepared Ag2S QDs can achieve selective detection of Fe3+ with a detection limit of LOD of 0.15 mM. This work provides a new method for the detection of Fe3+.

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Ag2S QDs 对 Fe3+ 的选择性检测和 IMPLICATION 门的构建
多项研究表明,Ag2S QDs 是一种很有前途的近红外 II 发射纳米探针。Ag2S QDs 可用于生物成像、荧光检测和光电探测器等领域。在这项工作中,我们首次成功构建了基于硫化银量子点对 Fe3+ 的特异性检测和抗坏血酸对 Fe3+ 的还原的双输入逻辑门 IMPLICATION 门。利用谷胱甘肽和硝酸银成功制备了 Ag2S QDs,并通过荧光光谱分析、XPS 分析和透射电子显微镜 TEM 分析对其进行了表征。制备的 Ag2S QDs 可实现对 Fe3+ 的选择性检测,检测限为 0.15 mM。这项工作为检测 Fe3+ 提供了一种新方法。
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来源期刊
Sensing and Bio-Sensing Research
Sensing and Bio-Sensing Research Engineering-Electrical and Electronic Engineering
CiteScore
10.70
自引率
3.80%
发文量
68
审稿时长
87 days
期刊介绍: Sensing and Bio-Sensing Research is an open access journal dedicated to the research, design, development, and application of bio-sensing and sensing technologies. The editors will accept research papers, reviews, field trials, and validation studies that are of significant relevance. These submissions should describe new concepts, enhance understanding of the field, or offer insights into the practical application, manufacturing, and commercialization of bio-sensing and sensing technologies. The journal covers a wide range of topics, including sensing principles and mechanisms, new materials development for transducers and recognition components, fabrication technology, and various types of sensors such as optical, electrochemical, mass-sensitive, gas, biosensors, and more. It also includes environmental, process control, and biomedical applications, signal processing, chemometrics, optoelectronic, mechanical, thermal, and magnetic sensors, as well as interface electronics. Additionally, it covers sensor systems and applications, µTAS (Micro Total Analysis Systems), development of solid-state devices for transducing physical signals, and analytical devices incorporating biological materials.
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