Graphene-based CO2 reduction electrocatalysts: A review

IF 5.7 3区 材料科学 Q2 Materials Science New Carbon Materials Pub Date : 2024-02-01 DOI:10.1016/S1872-5805(24)60839-5
Ze-lin Wu , Cong-wei Wang , Xiao-xiang Zhang , Quan-gui Guo , Jun-ying Wang
{"title":"Graphene-based CO2 reduction electrocatalysts: A review","authors":"Ze-lin Wu ,&nbsp;Cong-wei Wang ,&nbsp;Xiao-xiang Zhang ,&nbsp;Quan-gui Guo ,&nbsp;Jun-ying Wang","doi":"10.1016/S1872-5805(24)60839-5","DOIUrl":null,"url":null,"abstract":"<div><p>The reduction of carbon dioxide (CO<sub>2</sub>) by electrochemical methods for the production of fuels and value-added chemicals is an effective strategy for overcoming the global warming problem. Due to the stable molecular structure of CO<sub>2</sub>, the design of highly selective, energy-efficient and cost-effective electrocatalysts is key. For this reason, graphene and its derivatives are competitive for CO<sub>2</sub> electroreduction with their unique and excellent physical, mechanical and electrical properties and relatively low cost. In addition, the surface of graphene-based materials can be modified using different methods, including doping, defect engineering, production of composite structures and wrapped shapes. We first review the fundamental concepts and criteria for evaluating electrochemical CO<sub>2</sub> reduction, as well as the catalytic principles and processes. Methods for preparing graphene-based catalysts are briefly introduced, and recent research on them is summarized according to the categories of the catalytic sites. Finally, the future development direction of CO<sub>2</sub> electroreduction technology is discussed.</p></div>","PeriodicalId":19719,"journal":{"name":"New Carbon Materials","volume":null,"pages":null},"PeriodicalIF":5.7000,"publicationDate":"2024-02-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.sciencedirect.com/science/article/pii/S1872580524608395/pdf?md5=14b5913d9a3497fecb7a75487977444f&pid=1-s2.0-S1872580524608395-main.pdf","citationCount":"0","resultStr":null,"platform":"Semanticscholar","paperid":null,"PeriodicalName":"New Carbon Materials","FirstCategoryId":"88","ListUrlMain":"https://www.sciencedirect.com/science/article/pii/S1872580524608395","RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q2","JCRName":"Materials Science","Score":null,"Total":0}
引用次数: 0

Abstract

The reduction of carbon dioxide (CO2) by electrochemical methods for the production of fuels and value-added chemicals is an effective strategy for overcoming the global warming problem. Due to the stable molecular structure of CO2, the design of highly selective, energy-efficient and cost-effective electrocatalysts is key. For this reason, graphene and its derivatives are competitive for CO2 electroreduction with their unique and excellent physical, mechanical and electrical properties and relatively low cost. In addition, the surface of graphene-based materials can be modified using different methods, including doping, defect engineering, production of composite structures and wrapped shapes. We first review the fundamental concepts and criteria for evaluating electrochemical CO2 reduction, as well as the catalytic principles and processes. Methods for preparing graphene-based catalysts are briefly introduced, and recent research on them is summarized according to the categories of the catalytic sites. Finally, the future development direction of CO2 electroreduction technology is discussed.

查看原文
分享 分享
微信好友 朋友圈 QQ好友 复制链接
本刊更多论文
石墨烯基二氧化碳还原电催化剂:综述
利用电化学方法还原二氧化碳(CO2)以生产燃料和高附加值化学品,是解决全球变暖问题的有效策略。由于二氧化碳分子结构稳定,因此设计高选择性、高能效和高成本效益的电催化剂至关重要。因此,石墨烯及其衍生物以其独特而优异的物理、机械和电气性能以及相对较低的成本,在二氧化碳电还原方面具有很强的竞争力。此外,石墨烯基材料的表面可以通过不同的方法进行改性,包括掺杂、缺陷工程、生产复合结构和包裹形状。我们首先回顾了评估电化学二氧化碳还原的基本概念和标准,以及催化原理和过程。简要介绍了制备石墨烯基催化剂的方法,并根据催化位点的类别总结了近期的相关研究。最后,讨论了二氧化碳电还原技术的未来发展方向。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
求助全文
约1分钟内获得全文 去求助
来源期刊
New Carbon Materials
New Carbon Materials MATERIALS SCIENCE, MULTIDISCIPLINARY-
CiteScore
6.10
自引率
8.80%
发文量
3245
审稿时长
5.5 months
期刊介绍: New Carbon Materials is a scholarly journal that publishes original research papers focusing on the physics, chemistry, and technology of organic substances that serve as precursors for creating carbonaceous solids with aromatic or tetrahedral bonding. The scope of materials covered by the journal extends from diamond and graphite to a variety of forms including chars, semicokes, mesophase substances, carbons, carbon fibers, carbynes, fullerenes, and carbon nanotubes. The journal's objective is to showcase the latest research findings and advancements in the areas of formation, structure, properties, behaviors, and technological applications of carbon materials. Additionally, the journal includes papers on the secondary production of new carbon and composite materials, such as carbon-carbon composites, derived from the aforementioned carbons. Research papers on organic substances will be considered for publication only if they have a direct relevance to the resulting carbon materials.
期刊最新文献
A review of hard carbon anodes for rechargeable sodium-ion batteries Recent advances in producing hollow carbon spheres for use in sodium−sulfur and potassium−sulfur batteries Design, progress and challenges of 3D carbon-based thermally conductive networks The application of metal–organic frameworks and their derivatives for lithium-ion capacitors A review of the carbon coating of the silicon anode in high-performance lithium-ion batteries
×
引用
GB/T 7714-2015
复制
MLA
复制
APA
复制
导出至
BibTeX EndNote RefMan NoteFirst NoteExpress
×
×
提示
您的信息不完整,为了账户安全,请先补充。
现在去补充
×
提示
您因"违规操作"
具体请查看互助需知
我知道了
×
提示
现在去查看 取消
×
提示
确定
0
微信
客服QQ
Book学术公众号 扫码关注我们
反馈
×
意见反馈
请填写您的意见或建议
请填写您的手机或邮箱
已复制链接
已复制链接
快去分享给好友吧!
我知道了
×
扫码分享
扫码分享
Book学术官方微信
Book学术文献互助
Book学术文献互助群
群 号:481959085
Book学术
文献互助 智能选刊 最新文献 互助须知 联系我们:info@booksci.cn
Book学术提供免费学术资源搜索服务,方便国内外学者检索中英文文献。致力于提供最便捷和优质的服务体验。
Copyright © 2023 Book学术 All rights reserved.
ghs 京公网安备 11010802042870号 京ICP备2023020795号-1