Radiative decay rates for electric dipole transitions in doubly-, trebly- and quadruply-charged rhenium ions (Re III – V) of interest to nuclear fusion research and astrophysical spectra analyses
Maxime Brasseur , Sébastien Gamrath , Pascal Quinet
{"title":"Radiative decay rates for electric dipole transitions in doubly-, trebly- and quadruply-charged rhenium ions (Re III – V) of interest to nuclear fusion research and astrophysical spectra analyses","authors":"Maxime Brasseur , Sébastien Gamrath , Pascal Quinet","doi":"10.1016/j.adt.2024.101636","DOIUrl":null,"url":null,"abstract":"<div><p>A new set of radiative parameters (oscillator strengths and transition probabilities) was obtained for the most intense spectral lines in Re III, Re IV and Re V ions. These parameters were calculated using two independent methods, namely the pseudo-relativistic Hartree–Fock approach including core-polarization effects (HFR+CPOL) and the fully relativistic multiconfiguration Dirac–Hartree–Fock (MCDHF) approach. Detailed comparisons between the results obtained from these two methods as well as with the few data available in the literature allowed us to estimate the precision of the calculations carried out. The radiative parameters reported in the present paper concern a total of 368 electric dipole (E1) transitions in Re III, Re IV and Re V covering the ultraviolet spectral region from 655 to 2135 Å. These are of great interest for the analysis of spectra emitted by plasmas in nuclear fusion reactors, such as ITER where rhenium can be produced by neutron bombardment of the tungsten divertor wall, as well as for the investigation of astrophysical spectra observed from chemically peculiar stars or from kilonovae where rhenium can be produced by the nucleosynthesis r-process.</p></div>","PeriodicalId":55580,"journal":{"name":"Atomic Data and Nuclear Data Tables","volume":"157 ","pages":"Article 101636"},"PeriodicalIF":2.7000,"publicationDate":"2024-02-13","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":null,"platform":"Semanticscholar","paperid":null,"PeriodicalName":"Atomic Data and Nuclear Data Tables","FirstCategoryId":"101","ListUrlMain":"https://www.sciencedirect.com/science/article/pii/S0092640X24000019","RegionNum":3,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q2","JCRName":"PHYSICS, ATOMIC, MOLECULAR & CHEMICAL","Score":null,"Total":0}
引用次数: 0
Abstract
A new set of radiative parameters (oscillator strengths and transition probabilities) was obtained for the most intense spectral lines in Re III, Re IV and Re V ions. These parameters were calculated using two independent methods, namely the pseudo-relativistic Hartree–Fock approach including core-polarization effects (HFR+CPOL) and the fully relativistic multiconfiguration Dirac–Hartree–Fock (MCDHF) approach. Detailed comparisons between the results obtained from these two methods as well as with the few data available in the literature allowed us to estimate the precision of the calculations carried out. The radiative parameters reported in the present paper concern a total of 368 electric dipole (E1) transitions in Re III, Re IV and Re V covering the ultraviolet spectral region from 655 to 2135 Å. These are of great interest for the analysis of spectra emitted by plasmas in nuclear fusion reactors, such as ITER where rhenium can be produced by neutron bombardment of the tungsten divertor wall, as well as for the investigation of astrophysical spectra observed from chemically peculiar stars or from kilonovae where rhenium can be produced by the nucleosynthesis r-process.
与核聚变研究和天体物理光谱分析有关的双电荷、三电荷和四电荷铼离子(Re III - V)电偶极子转换的辐射衰变率
针对 Re III、Re IV 和 Re V 离子中最强烈的光谱线,获得了一组新的辐射参数(振荡器强度和跃迁概率)。这些参数的计算采用了两种独立的方法,即包括核极化效应的伪相对论哈特里-福克方法(HFR+CPOL)和完全相对论多构型狄拉克-哈特里-福克方法(MCDHF)。通过对这两种方法得出的结果以及文献中的少量数据进行详细比较,我们估算出了计算的精确度。本文报告的辐射参数涉及 Re III、Re IV 和 Re V 中总共 368 个电偶极子 (E1) 转变,涵盖 655 至 2135 Å 的紫外光谱区。这些参数对于分析核聚变反应堆(如国际热核聚变实验堆,其中铼可通过中子轰击钨偏转器壁产生)中等离子体发射的光谱以及研究从化学性质奇特的恒星或千新星(其中铼可通过核合成 r 过程产生)中观测到的天体物理光谱具有重要意义。
期刊介绍:
Atomic Data and Nuclear Data Tables presents compilations of experimental and theoretical information in atomic physics, nuclear physics, and closely related fields. The journal is devoted to the publication of tables and graphs of general usefulness to researchers in both basic and applied areas. Extensive ... click here for full Aims & Scope
Atomic Data and Nuclear Data Tables presents compilations of experimental and theoretical information in atomic physics, nuclear physics, and closely related fields. The journal is devoted to the publication of tables and graphs of general usefulness to researchers in both basic and applied areas. Extensive and comprehensive compilations of experimental and theoretical results are featured.