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Semi-empirical determination of radiative parameters for atomic lutetium 原子镥辐射参数的半经验测定
IF 4.1 3区 物理与天体物理 Q2 PHYSICS, ATOMIC, MOLECULAR & CHEMICAL Pub Date : 2026-01-09 DOI: 10.1016/j.adt.2025.101785
M. Klempka , J. Ruczkowski , M. Elantkowska
The values of the radiative parameters for atomic lutetium (Lu I) were determined using a semi-empirical method. The eigenvector amplitudes determined in our previously published research were adopted. In most cases, the calculated values of the oscillator strengths and radiative lifetimes agree well with the experimental data. Predictions of the values of the radiative parameters are also provided.
用半经验方法测定了原子镥(Lu I)的辐射参数。采用我们之前发表的研究中确定的特征向量振幅。在大多数情况下,振子强度和辐射寿命的计算值与实验数据吻合较好。还提供了辐射参数值的预测。
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引用次数: 0
Low-energy phase shifts and scattering length of strontium from Dirac-Coulomb and polarization potential modeling 狄拉克-库仑和极化势模型研究锶的低能相移和散射长度
IF 4.1 3区 物理与天体物理 Q2 PHYSICS, ATOMIC, MOLECULAR & CHEMICAL Pub Date : 2026-01-08 DOI: 10.1016/j.adt.2025.101783
P. Syty , M.P. Piłat , J.E. Sienkiewicz
We present a calculation of the low-energy phase shift and scattering length for the strontium atom, using the Dirac-Coulomb Hamiltonian augmented with a model polarization potential. The scattering length is extracted from the asymptotic behavior of the wave function in the zero-energy limit. To evaluate the reliability of our results, we compare them with existing experimental data and previous theoretical predictions. Bound-state properties are obtained using a multiconfigurational approach with the GRASP2018 package, while continuum states are computed with a modified version of the GRASP code, known as GRASPC, recently published in Computer Physics Communications.
我们提出了一个计算锶原子的低能相移和散射长度,使用狄拉克-库仑哈密顿增广模型极化势。从波函数在零能量极限下的渐近特性提取散射长度。为了评估我们的结果的可靠性,我们将它们与现有的实验数据和先前的理论预测进行了比较。绑定状态属性是使用GRASP2018包的多配置方法获得的,而连续状态是使用最近发表在《计算机物理通信》上的修改版本的GRASP代码(称为GRASPC)计算的。
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引用次数: 0
Stevens multiplicative factors α, β, γ for 3dn and 4fn ions in spin–orbital space 自旋轨道空间中3dn和4fn离子的Stevens乘法因子α, β, γ
IF 4.1 3区 物理与天体物理 Q2 PHYSICS, ATOMIC, MOLECULAR & CHEMICAL Pub Date : 2026-01-06 DOI: 10.1016/j.adt.2025.101784
D.M. Nalecz
This study presents new tables for Stevens’ multiplicative factors LβL and LγL for ions with a 4fn configuration. The tables, denoted as Table 4 and Table 5, provide values for these factors that were calculated for 4fn ions in the |L,Lz,S,Sz basis, which distinguishes them from typically used tables expressed in the |J,Jz basis and commonly truncated for 4fn ions. These values are crucial for describing the magnetic and electric properties of compounds containing lanthanide ions. To the best of our knowledge, these values have not been explicitly tabulated in any previous publication. The tables may help in the analysis of experimental data and the modeling of magnetic and electric properties for ions with a 4fn configuration.
本研究提出了史蒂文斯的乘法因子< L‖β‖L >和< L‖γ‖L >与4fn配置离子的新表。表4和表5给出了这些因子的值,这些因子是在|L、Lz、S、Sz >基下为4fn离子计算的,这与通常使用|J、Jz >基表示的表和通常截断的4fn离子表不同。这些值对于描述含有镧系离子的化合物的磁性和电学性质是至关重要的。据我们所知,这些值在以前的任何出版物中都没有明确列出。这些表有助于对实验数据的分析和对具有4fn结构的离子的磁性和电学性质的建模。
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引用次数: 0
Revised level energies of Nb I Nb I的修正能级能
IF 4.1 3区 物理与天体物理 Q2 PHYSICS, ATOMIC, MOLECULAR & CHEMICAL Pub Date : 2025-12-31 DOI: 10.1016/j.adt.2025.101771
L. Windholz , S. Kröger
With the use of wave number calibrated Fourier transform spectra spanning from the IR to the UV wavelength range, the values of energy levels of the atomic niobium (Nb I) have been revised. Due to recently published work (JQSRT 332 (2024) 109285) now the magnetic dipole hyperfine structure constants are available for all known Nb I levels. This allows to find the center of gravity wave numbers of the observed spectral lines with high accuracy. Revised level energies of all 399 known fine structure levels are determined using a global fit of altogether 1756 spectral lines, based on a least squares procedure. A comparison between our new results and available literature values is given and discussed.
利用从红外到紫外波长范围的波数校准傅立叶变换光谱,修正了铌原子(Nb I)的能级值。由于最近发表的工作(JQSRT 332(2024) 109285),现在磁偶极子超精细结构常数可用于所有已知的铌I能级。这样可以高精度地求出观测光谱线的重心波数。所有399个已知精细结构能级的修正能级能量是基于最小二乘程序,使用总共1756条谱线的全局拟合来确定的。我们的新结果与现有文献值进行了比较,并进行了讨论。
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引用次数: 0
Erratum to “Nuclear β−-decay with statistical de-excitation” [At. Data Nucl. Data Tables 165 (2025) 1–81] “核β−衰变与统计去激发”的勘误[a]。数据诊断。数据表165 (2025)1-81]
IF 4.1 3区 物理与天体物理 Q2 PHYSICS, ATOMIC, MOLECULAR & CHEMICAL Pub Date : 2025-12-15 DOI: 10.1016/j.adt.2025.101782
M.R. Mumpower , T. Kawano , O. Korobkin , G.W. Misch , T.M. Sprouse
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引用次数: 0
Measurement of the cross sections of prompt γ-ray production in the 14.1 MeV neutron induced reactions for 16 elements with atomic numbers between 3 and 50 原子序数在3 ~ 50之间的16种元素在14.1 MeV中子诱导反应中激发γ射线产生截面的测量
IF 4.1 3区 物理与天体物理 Q2 PHYSICS, ATOMIC, MOLECULAR & CHEMICAL Pub Date : 2025-12-10 DOI: 10.1016/j.adt.2025.101781
P.S. Prusachenko , N.A. Fedorov , D.N. Grozdanov , Yu.N. Kopatch , P.I. Kharlamov , C. Hramco , V.R. Skoy , T.Yu. Tretyakova , А.V. Andreev , P.G. Filonchik , I.N. Ruskov , TANGRA collaboration
This paper presents an overview of the latest results of measuring differential and integrated γ-ray emission cross sections in reactions induced by 14.1 MeV neutrons for 16 elements (Li, B, N, F, Na, Mg, S, Cl, K, V, Mn, Co, Ni, Cu, Zn, Sn) carried out within the framework of the TANGRA (TAgged Neutrons and Gamma RAys) project. The experiments were performed using high-resolution γ-ray detectors based on LaBr3(Ce) crystals and high-purity germanium (HPGe) detectors. A distinctive feature of this work was the use of the tagged neutron method to determine the number of neutrons hitting the sample and background rejection by time of flight. Differential cross sections were obtained in the angular range of 12–89°, with subsequent expansion into Legendre polynomials of even degree to obtain the integrated cross sections.
本文概述了在TANGRA(标记中子和伽马射线)项目框架内进行的14.1 MeV中子诱导16种元素(Li, B, N, F, Na, Mg, S, Cl, K, V, Mn, Co, Ni, Cu, Zn, Sn)反应的微分和积分γ射线发射截面测量的最新结果。实验采用基于LaBr3(Ce)晶体和高纯锗(HPGe)探测器的高分辨率γ射线探测器进行。这项工作的一个显著特点是使用标记中子方法来确定击中样品的中子数和飞行时间的背景排斥。在12-89°角范围内得到微分截面,然后展开为偶次的勒让德多项式得到积分截面。
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引用次数: 0
Systematic photoabsorption cross sections studied within the axially deformed relativistic quasiparticle finite amplitude framework 轴向变形相对论准粒子有限振幅框架内系统光吸收截面的研究
IF 4.1 3区 物理与天体物理 Q2 PHYSICS, ATOMIC, MOLECULAR & CHEMICAL Pub Date : 2025-12-01 DOI: 10.1016/j.adt.2025.101770
C. Chen (陈晨) , Y.F. Niu (牛一斐) , R. Xu (续瑞瑞) , Y. Tian (田源)
Photoabsorption cross sections for 235 stable nuclei, ranging from 40Ca to 209Bi, were investigated by the quasiparticle finite amplitude method (QFAM) based on the axially deformed relativistic Hartree–Bogoliubov (RHB) approach using relativistic point-coupling interaction DD-PC1, with extensions to odd-A nuclei. The microscopic description of odd-A nuclei makes it possible to capture abrupt changes in the photoabsorption cross sections due to the shape transitions between odd-A nuclei and their even–even neighbors. GDR parameters based on the standard Lorentzian (SLO) model were extracted from QFAM results and compared with those from experimental data recommended by IAEA. Good agreement was achieved for giant dipole resonance (GDR) peak energies, while resonance widths were underestimated and hence peak cross sections were overestimated due to the lack of higher-order many-body correlations. These discrepancies were much improved in deformed nuclei. The effects of deformation on photoabsorption cross sections were examined systematically. The comparison of photoabsorption cross sections among QFAM results and discrepant experimental data revealed the potential of QFAM calculations in the evaluation of photonuclear data.
利用相对论点耦合相互作用DD-PC1,采用准粒子有限振幅法(QFAM)研究了235个40Ca ~ 209Bi稳定原子核的光吸收截面,并扩展到奇a核。通过对奇a核的微观描述,可以捕捉到由于奇a核与其偶偶相邻核之间的形状转变而引起的光吸收截面的突变。从QFAM结果中提取基于标准洛伦兹(SLO)模型的GDR参数,并与IAEA推荐的实验数据进行比较。巨偶极子共振(GDR)峰值能量得到了很好的一致性,而共振宽度被低估了,因此由于缺乏高阶多体相关,峰值截面被高估了。这些差异在畸形核中得到改善。系统地考察了变形对光吸收截面的影响。比较了QFAM计算结果与不同实验数据的光吸收截面,揭示了QFAM计算在评价光核数据中的潜力。
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引用次数: 0
Ionisation potentials and energy levels of ions of heavy and superheavy elements Te, I, Po, At, Lv and Ts 重、超重元素Te、I、Po、At、Lv和Ts离子的电离势和能级
IF 4.1 3区 物理与天体物理 Q2 PHYSICS, ATOMIC, MOLECULAR & CHEMICAL Pub Date : 2025-11-01 DOI: 10.1016/j.adt.2025.101769
G.K. Vong, V.A. Dzuba, V.V. Flambaum
We calculate the energy levels and successive ionisation potentials (IPs) of ions of the three heaviest known Group 16 and 17 elements using a theoretical approach that combines the linearised coupled-cluster method, configuration interaction, and perturbation theory. Our calculations address critical gaps in the available data on the electronic structure of the superheavy elements livermorium (Lv) and tennessine (Ts), as well as their lighter homologues polonium (Po) and astatine (At). To assess the accuracy of our methods, we perform analogous calculations for the lighter homologues tellurium (Te) and iodine (I), for which both experimental and reliable theoretical data are available for comparison.
我们使用结合线性耦合簇方法、构型相互作用和摄动理论的理论方法计算了已知的3个最重的16族和17族元素的离子能级和连续电离势(IPs)。我们的计算解决了超重元素livermorium (Lv)和tennessine (Ts)以及它们较轻的同系物polonium (Po)和astatine (At)电子结构现有数据中的关键空白。为了评估我们的方法的准确性,我们对较轻的同系物碲(Te)和碘(I)进行了类似的计算,实验和可靠的理论数据可供比较。
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引用次数: 0
Discovery of nuclear isomers 发现核异构体
IF 4.1 3区 物理与天体物理 Q2 PHYSICS, ATOMIC, MOLECULAR & CHEMICAL Pub Date : 2025-10-30 DOI: 10.1016/j.adt.2025.101767
M. Thoennessen, J. Chen
Currently, 1917 nuclear isomers with half-lives longer than 100 ns have been discovered in 1310 different nuclides and 103 different elements. While the physical properties of isomers have been compiled before, this is the first compilation of the isomer discoveries. For each isomer the reference, year, laboratory and country are documented.
目前,在1310种不同的核素和103种不同的元素中发现了1917种半衰期超过100纳秒的核异构体。虽然同分异构体的物理性质以前已经汇编,但这是第一次汇编同分异构体的发现。每种异构体的参考文献、年份、实验室和国家都有记录。
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引用次数: 0
Effects of the Breit and QED corrections on the splittings between the fine-structure 1s22s22p2P1/2,3/2 levels for the boron isoelectronic sequence Breit和QED修正对硼等电子层序1s22s22p2P1/2和3/2精细结构劈裂的影响
IF 4.1 3区 物理与天体物理 Q2 PHYSICS, ATOMIC, MOLECULAR & CHEMICAL Pub Date : 2025-10-24 DOI: 10.1016/j.adt.2025.101766
Jian-Jie Wan, Qin Ma, Bin Bai, Jiao Li
Multiconfiguration Dirac–Hartree–Fock (MCDHF) and relativistic configuration interaction (RCI) methods have been used to calculate the energies of 1s22s22p2P1/2,3/2 levels for the boron isoelectronic sequence with Z=592. It is found that the fine-structure splitting can be corrected by adding the frequency-dependent part of the Breit correction, which can result in a significant improvement of up to about 0.2% especially for high-Z B-like ions. We suggest that the fine-structure 1s22s22p2P3/22P1/2 splittings in the boron isoelectronic sequence could be used to accurately test current theoretical methods to calculate the corrections of Breit and quantum electrodynamic (QED) effects. As far as the QED effects are concerned, the self-energy correction dominates for the low- and mid-Z range (Z=579), but then decreases to change sign for Z=87 and meanwhile after Z=80 the vacuum polarization is the leading term. It is also found that the frequency-dependent part of Breit correction strongly cancel out the SE and the total QED effects for Z=56 and 60, respectively. This allows us to accurately test VP and Breit correlation for these ions. The uncertainties of the frequency-independent Breit correction and Coulomb correlation are expected to be at least 2 orders of magnitude smaller than the QED and frequency-dependent part of Breit corrections for intermediate- and high-Z B-like ions. Finally, the present M1 and E2 transition probabilities between the fine-structure levels are calculated and they are in good agreement with other theoretical and experimental results, especially for the mid- and high-Z ions.
用多组态dirac - harree - fock (MCDHF)和相对论组态相互作用(RCI)方法计算了Z=5−92的硼等电子序列的1s22s22p2P1/2和3/2能级的能量。研究发现,通过增加Breit校正的频率相关部分,可以对精细结构的分裂进行校正,特别是对于高z类b离子,可以显著改善约0.2%。我们认为硼等电子序列中的1s22s22p2P3/2−2P1/2的精细结构可以用来精确测试当前计算Breit和量子电动力学(QED)效应修正的理论方法。在QED效应中,自能修正在Z=5 ~ 79的低、中Z范围内占主导地位,但在Z=87时减小到变化符号,而在Z=80之后,真空极化是主导项。还发现,Breit修正的频率相关部分强烈地抵消了SE和总QED效应,分别为Z=56和60。这使我们能够准确地测试这些离子的VP和Breit相关性。对于中z和高z类b离子,与频率无关的Breit校正和库仑相关的不确定性预计至少比Breit校正的QED和频率相关部分小2个数量级。最后,计算了精细结构能级间的M1和E2跃迁概率,它们与其他理论和实验结果吻合得很好,特别是对于中、高z离子。
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引用次数: 0
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Atomic Data and Nuclear Data Tables
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