Ultra-stability and high output performance of a sliding mode triboelectric nanogenerator achieved by an asymmetric electrode structure design†

IF 32.4 1区 材料科学 Q1 CHEMISTRY, MULTIDISCIPLINARY Energy & Environmental Science Pub Date : 2024-02-29 DOI:10.1039/D3EE04253G
Gui Li, Jian Wang, Yue He, Shuyan Xu, Shaoke Fu, Chuncai Shan, Huiyuan Wu, Shanshan An, Kaixian Li, Wen Li, Ping Wang and Chenguo Hu
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Abstract

The sliding mode triboelectric nanogenerator (S-TENG) is a highly efficient technology for harvesting environmental mechanical energy due to its advantages of sustainable energy output and simple structure design. However, boosting the output performance of the S-TENG remains a challenge because of the bottleneck of air breakdown. Herein, a new type of an asymmetric electrode structure S-TENG (AE-S-TENG) is proposed by designing asymmetric top and bottom electrodes, which is quite different from the previous symmetric electrode structure. The electrostatic shielding mechanism and quantified charge transfer analysis are presented. The ultra-stability and high output performance of the AE-S-TENG are achieved by balancing the electrostatic shielding to inhabit the air breakdown and the charge supplement to enhance the charge density through the asymmetric electrodes and non-electrode shielding areas. The output charge of the AE-S-TENG with equal size is 1.89-fold higher than that of the normal S-TENG. The output charge, current and average power of rotation AE-S-TENG at 60 rpm maintain 3.01 μC, 120 μA and 48.64 mW after more than 72 000 cycles, respectively. This work provides insights into the electrostatic shielding and charge transfer mechanism of the asymmetric electrode structure, which provides a new idea for designing high-output and superdurability TENGs.

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通过非对称电极结构设计实现滑动模式三电纳米发电机的超稳定性和高输出性能
滑动模式三电纳米发电机(S-TENG)具有可持续输出能量、结构设计简单等优点,是一种高效的环境机械能采集技术。然而,由于空气击穿的瓶颈,提高 S-TENG 的输出性能仍是一项挑战。本文提出了一种新型非对称电极结构 S-TENG(AE-S-TENG),通过设计非对称的顶部和底部电极,与以往的对称电极结构截然不同。文中介绍了静电屏蔽机理和电荷转移量化分析。AE-S-TENG 的超稳定性和高输出性能是通过非对称电极和非电极屏蔽区的静电屏蔽和电荷补充平衡实现的。同等尺寸的 AE-S-TENG 输出电荷是普通 S-TENG 的 1.89 倍。在 60 rpm 转速下旋转 AE-S-TENG 的输出电荷、电流和平均功率在超过 72 000 次循环后仍保持在 3.01 μC、120 μA 和 48.64 mW。这项研究深入探讨了非对称电极结构的静电屏蔽和电荷转移机制,为设计高输出和超耐用的 TENG 提供了新思路。
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来源期刊
Energy & Environmental Science
Energy & Environmental Science 化学-工程:化工
CiteScore
50.50
自引率
2.20%
发文量
349
审稿时长
2.2 months
期刊介绍: Energy & Environmental Science, a peer-reviewed scientific journal, publishes original research and review articles covering interdisciplinary topics in the (bio)chemical and (bio)physical sciences, as well as chemical engineering disciplines. Published monthly by the Royal Society of Chemistry (RSC), a not-for-profit publisher, Energy & Environmental Science is recognized as a leading journal. It boasts an impressive impact factor of 8.500 as of 2009, ranking 8th among 140 journals in the category "Chemistry, Multidisciplinary," second among 71 journals in "Energy & Fuels," second among 128 journals in "Engineering, Chemical," and first among 181 scientific journals in "Environmental Sciences." Energy & Environmental Science publishes various types of articles, including Research Papers (original scientific work), Review Articles, Perspectives, and Minireviews (feature review-type articles of broad interest), Communications (original scientific work of an urgent nature), Opinions (personal, often speculative viewpoints or hypotheses on current topics), and Analysis Articles (in-depth examination of energy-related issues).
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