Hydrocarbon Transformations in Bottom Sediments after an Emergency Spill of Diesel Fuel in Norilsk

IF 0.9 4区 环境科学与生态学 Q4 WATER RESOURCES Water Resources Pub Date : 2024-03-05 DOI:10.1134/s0097807823700240
Yu. S. Glyaznetsova, I. A. Nemirovskaya
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Abstract

One year after an emergency spill of diesel fuel in Norilsk, hydrocarbon concentrations in bottom sediments of the Norilo-Pyasinskaya Water System decreased, but, on the average over the regions, they decreased in the surface layer in the same order as in 2020: Ambarnaya River mouth (835 µg/g, σ = 1788) > Bezymyannyi Creek—Daldykan River—Ambarnaya River (306 µg/g, σ = 273) > Pyasina River (23 µg/g, σ = 20) > Pyasino Lake (12 µg/g, σ = 8). The decrease in the concentrations was due to the degradation of low-molecular hydrocarbons. The concentration of polycyclic aromatic hydrocarbons in 2021 also varied within a narrower interval (0–1027 ng/g) than in 2020 (0–3865 ng/g). The oil origin of the hydrocarbons in the sediments of the Bezymyannyi Creek and the rivers of Daldykan and Ambarnaya is confirmed by their high content of alkylied naphthalene homologues. The accumulation of hydrocarbons in some horizons of the sedimentary stratum is due not only to the seepage of diesel fuel, but also to the input of organic matter from swampy areas and floodplain lakes, as well as to the burial of the surface layer by the flood of 2021.

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诺里尔斯克柴油紧急泄漏后海底沉积物中的碳氢化合物转化
摘要 在诺里尔斯克发生柴油紧急泄漏事件一年后,诺里尔斯克-皮亚辛斯卡娅水系底层沉积物中的碳氢化合物浓度有所下降,但从各地区的平均水平来看,表层的碳氢化合物浓度下降顺序与 2020 年相同:安巴尔纳亚河口(835 微克/克,σ = 1788)> Bezymyannyi 溪-Daldykan 河-安巴尔纳亚河(306 微克/克,σ = 273)> Pyasina 河(23 微克/克,σ = 20)> Pyasino 湖(12 微克/克,σ = 8)。浓度下降的原因是低分子碳氢化合物的降解。2021 年的多环芳烃浓度变化区间(0-1027 纳克/克)也比 2020 年(0-3865 纳克/克)窄。Bezymyannyi 河、Daldykan 河和 Ambarnaya 河沉积物中烷基萘同系物的高含量证实了碳氢化合物的石油来源。沉积层某些地层中碳氢化合物的积累不仅是由于柴油的渗出,也是由于沼泽地区和洪泛平原湖泊有机物的输入,以及 2021 年洪水对表层的掩埋。
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来源期刊
Water Resources
Water Resources 环境科学-水资源
CiteScore
1.60
自引率
20.00%
发文量
86
审稿时长
6-12 weeks
期刊介绍: Water Resources is a journal that publishes articles on the assessment of water resources, integrated water resource use, water quality, and environmental protection. The journal covers many areas of research, including prediction of variations in continental water resources and regime; hydrophysical, hydrodynamic, hydrochemical and hydrobiological processes, environmental aspects of water quality and protection; economic, social, and legal aspects of water-resource development; and experimental methods of studies.
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