A hybrid spatial-temporal deep learning prediction model of industrial methanol-to-olefins process

IF 4.3 3区 工程技术 Q2 ENGINEERING, CHEMICAL Frontiers of Chemical Science and Engineering Pub Date : 2024-03-15 DOI:10.1007/s11705-024-2403-7
Jibin Zhou, Xue Li, Duiping Liu, Feng Wang, Tao Zhang, Mao Ye, Zhongmin Liu
{"title":"A hybrid spatial-temporal deep learning prediction model of industrial methanol-to-olefins process","authors":"Jibin Zhou,&nbsp;Xue Li,&nbsp;Duiping Liu,&nbsp;Feng Wang,&nbsp;Tao Zhang,&nbsp;Mao Ye,&nbsp;Zhongmin Liu","doi":"10.1007/s11705-024-2403-7","DOIUrl":null,"url":null,"abstract":"<div><p>Methanol-to-olefins, as a promising non-oil pathway for the synthesis of light olefins, has been successfully industrialized. The accurate prediction of process variables can yield significant benefits for advanced process control and optimization. The challenge of this task is underscored by the failure of traditional methods in capturing the complex characteristics of industrial processes, such as high nonlinearities, dynamics, and data distribution shift caused by diverse operating conditions. In this paper, we propose a novel hybrid spatial-temporal deep learning prediction model to address these issues. Firstly, a unique data normalization technique called reversible instance normalization is employed to solve the problem of different data distributions. Subsequently, convolutional neural network integrated with the self-attention mechanism are utilized to extract the temporal patterns. Meanwhile, a multi-graph convolutional network is leveraged to model the spatial interactions. Afterward, the extracted temporal and spatial features are fused as input into a fully connected neural network to complete the prediction. Finally, the outputs are denormalized to obtain the ultimate results. The monitoring results of the dynamic trends of process variables in an actual industrial methanol-to-olefins process demonstrate that our model not only achieves superior prediction performance but also can reveal complex spatial-temporal relationships using the learned attention matrices and adjacency matrices, making the model more interpretable. Lastly, this model is deployed onto an end-to-end Industrial Internet Platform, which achieves effective practical results.\n</p><div><figure><div><div><picture><source><img></source></picture></div></div></figure></div></div>","PeriodicalId":571,"journal":{"name":"Frontiers of Chemical Science and Engineering","volume":"18 4","pages":""},"PeriodicalIF":4.3000,"publicationDate":"2024-03-15","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":null,"platform":"Semanticscholar","paperid":null,"PeriodicalName":"Frontiers of Chemical Science and Engineering","FirstCategoryId":"5","ListUrlMain":"https://link.springer.com/article/10.1007/s11705-024-2403-7","RegionNum":3,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q2","JCRName":"ENGINEERING, CHEMICAL","Score":null,"Total":0}
引用次数: 0

Abstract

Methanol-to-olefins, as a promising non-oil pathway for the synthesis of light olefins, has been successfully industrialized. The accurate prediction of process variables can yield significant benefits for advanced process control and optimization. The challenge of this task is underscored by the failure of traditional methods in capturing the complex characteristics of industrial processes, such as high nonlinearities, dynamics, and data distribution shift caused by diverse operating conditions. In this paper, we propose a novel hybrid spatial-temporal deep learning prediction model to address these issues. Firstly, a unique data normalization technique called reversible instance normalization is employed to solve the problem of different data distributions. Subsequently, convolutional neural network integrated with the self-attention mechanism are utilized to extract the temporal patterns. Meanwhile, a multi-graph convolutional network is leveraged to model the spatial interactions. Afterward, the extracted temporal and spatial features are fused as input into a fully connected neural network to complete the prediction. Finally, the outputs are denormalized to obtain the ultimate results. The monitoring results of the dynamic trends of process variables in an actual industrial methanol-to-olefins process demonstrate that our model not only achieves superior prediction performance but also can reveal complex spatial-temporal relationships using the learned attention matrices and adjacency matrices, making the model more interpretable. Lastly, this model is deployed onto an end-to-end Industrial Internet Platform, which achieves effective practical results.

查看原文
分享 分享
微信好友 朋友圈 QQ好友 复制链接
本刊更多论文
工业甲醇制烯烃过程的时空混合深度学习预测模型
摘要 甲醇制烯烃是合成轻质烯烃的一种前景广阔的非石油途径,已成功实现工业化。准确预测工艺变量可为先进的工艺控制和优化带来显著效益。传统方法无法捕捉工业过程的复杂特性,如高度非线性、动态性和由不同操作条件引起的数据分布偏移,这凸显了这项任务的挑战性。本文提出了一种新型时空混合深度学习预测模型来解决这些问题。首先,我们采用了一种名为可逆实例归一化的独特数据归一化技术来解决不同数据分布的问题。随后,利用卷积神经网络与自注意机制相结合来提取时态模式。同时,利用多图卷积网络建立空间交互模型。然后,将提取的时间和空间特征作为输入融合到全连接神经网络中,完成预测。最后,对输出进行去规范化处理,得出最终结果。对实际工业甲醇制烯烃过程中工艺变量动态趋势的监测结果表明,我们的模型不仅实现了卓越的预测性能,还能利用学习到的注意力矩阵和邻接矩阵揭示复杂的时空关系,使模型更具可解释性。最后,该模型被部署到端到端的工业互联网平台上,取得了有效的实际效果。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
求助全文
约1分钟内获得全文 去求助
来源期刊
CiteScore
7.60
自引率
6.70%
发文量
868
审稿时长
1 months
期刊介绍: Frontiers of Chemical Science and Engineering presents the latest developments in chemical science and engineering, emphasizing emerging and multidisciplinary fields and international trends in research and development. The journal promotes communication and exchange between scientists all over the world. The contents include original reviews, research papers and short communications. Coverage includes catalysis and reaction engineering, clean energy, functional material, nanotechnology and nanoscience, biomaterials and biotechnology, particle technology and multiphase processing, separation science and technology, sustainable technologies and green processing.
期刊最新文献
Effective lateral dispersion of momentum, heat and mass in bubbling fluidized beds Reversible heat-set four-phase transitions of gel1-to-sol1-to-gel2-to-sol2 in binary hydrogels Investigating CO2 electro-reduction mechanisms: DFT insight into earth-abundant Mn diimine catalysts for CO2 conversions over hydrogen evolution reaction, feasibility, and selectivity considerations DFT insights into oxygen vacancy formation and chemical looping dry reforming of methane on metal-substituted CeO2 (111) surface Chemical recycling of polyolefin waste: from the perspective of efficient pyrolysis reactors
×
引用
GB/T 7714-2015
复制
MLA
复制
APA
复制
导出至
BibTeX EndNote RefMan NoteFirst NoteExpress
×
×
提示
您的信息不完整,为了账户安全,请先补充。
现在去补充
×
提示
您因"违规操作"
具体请查看互助需知
我知道了
×
提示
现在去查看 取消
×
提示
确定
0
微信
客服QQ
Book学术公众号 扫码关注我们
反馈
×
意见反馈
请填写您的意见或建议
请填写您的手机或邮箱
已复制链接
已复制链接
快去分享给好友吧!
我知道了
×
扫码分享
扫码分享
Book学术官方微信
Book学术文献互助
Book学术文献互助群
群 号:481959085
Book学术
文献互助 智能选刊 最新文献 互助须知 联系我们:info@booksci.cn
Book学术提供免费学术资源搜索服务,方便国内外学者检索中英文文献。致力于提供最便捷和优质的服务体验。
Copyright © 2023 Book学术 All rights reserved.
ghs 京公网安备 11010802042870号 京ICP备2023020795号-1