From electrolyte to electrode interface: Understanding impacts of electrolyte additives for aqueous zinc-ion batteries

IF 7.9 2区 化学 Q1 CHEMISTRY, PHYSICAL Current Opinion in Electrochemistry Pub Date : 2024-03-14 DOI:10.1016/j.coelec.2024.101483
Zeshen Deng, Liuzhang Ouyang, Longtao Ma, Lichun Yang, Min Zhu
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Abstract

Aqueous zinc-ion batteries (AZIBs) hold tremendous potential as next-generation large-scale energy storage devices, yet they face significant challenges. The reversibility of AZIBs is hindered by the unstable electrode/electrolyte interface caused by dendrite formation and parasitic side reactions. Electrolyte additives present a promising and straightforward approach to enhance the reversibility of AZIBs while maintaining overall energy density. In this short review, we systematically summarize the impacts of electrolyte additives based on the functional mechanisms. We provide a comprehensive analysis of the effects of additives on the bulk electrolyte and the electrode/electrolyte interface, as well as highlight the significance of multifunctional additives for achieving durable anodes and cathodes. To address the current research limitations, we offer perspectives on future research directions, guiding the exploration of novel additives and the realization of high-performance AZIBs.

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从电解质到电极界面:了解锌离子水电池电解质添加剂的影响
锌离子水电池(AZIBs)作为下一代大规模储能设备具有巨大潜力,但也面临着重大挑战。由于枝晶形成和寄生副反应导致电极/电解质界面不稳定,AZIBs 的可逆性受到阻碍。电解质添加剂为提高 AZIB 的可逆性同时保持整体能量密度提供了一种前景广阔的直接方法。在这篇简短的综述中,我们根据功能机制系统地总结了电解质添加剂的影响。我们全面分析了添加剂对体电解质和电极/电解质界面的影响,并强调了多功能添加剂对实现耐用阳极和阴极的重要意义。针对目前研究的局限性,我们展望了未来的研究方向,为探索新型添加剂和实现高性能 AZIB 提供了指导。
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来源期刊
Current Opinion in Electrochemistry
Current Opinion in Electrochemistry Chemistry-Analytical Chemistry
CiteScore
14.00
自引率
5.90%
发文量
272
审稿时长
73 days
期刊介绍: The development of the Current Opinion journals stemmed from the acknowledgment of the growing challenge for specialists to stay abreast of the expanding volume of information within their field. In Current Opinion in Electrochemistry, they help the reader by providing in a systematic manner: 1.The views of experts on current advances in electrochemistry in a clear and readable form. 2.Evaluations of the most interesting papers, annotated by experts, from the great wealth of original publications. In the realm of electrochemistry, the subject is divided into 12 themed sections, with each section undergoing an annual review cycle: • Bioelectrochemistry • Electrocatalysis • Electrochemical Materials and Engineering • Energy Storage: Batteries and Supercapacitors • Energy Transformation • Environmental Electrochemistry • Fundamental & Theoretical Electrochemistry • Innovative Methods in Electrochemistry • Organic & Molecular Electrochemistry • Physical & Nano-Electrochemistry • Sensors & Bio-sensors •
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