Qinglan Zhao , Yan Zhang , Dapeng Cao , Minhua Shao
{"title":"The prospects of urea manufacturing via electrochemical co-reduction of CO2 and nitrates","authors":"Qinglan Zhao , Yan Zhang , Dapeng Cao , Minhua Shao","doi":"10.1016/j.coelec.2024.101479","DOIUrl":null,"url":null,"abstract":"<div><p>Electrochemical co-reduction of CO<sub>2</sub> and nitrates presents a promising alternative for urea production. However, the current electrochemical synthesis of urea faces challenges related to low selectivity and production rates. The development of high-efficiency electrocatalysts is the key to performance improvement of urea electrosynthesis. This minireview primarily focuses on the rational design of catalysts, starting with a mechanistic overview. In addition, the advancement of electrolyzers for urea electrochemical synthesis is also discussed aiming to articulate guiding principles of achieving high-rate production reaching industrial relevant level in the future.</p></div>","PeriodicalId":11028,"journal":{"name":"Current Opinion in Electrochemistry","volume":"45 ","pages":"Article 101479"},"PeriodicalIF":7.9000,"publicationDate":"2024-03-13","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":null,"platform":"Semanticscholar","paperid":null,"PeriodicalName":"Current Opinion in Electrochemistry","FirstCategoryId":"92","ListUrlMain":"https://www.sciencedirect.com/science/article/pii/S2451910324000401","RegionNum":2,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"CHEMISTRY, PHYSICAL","Score":null,"Total":0}
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Abstract
Electrochemical co-reduction of CO2 and nitrates presents a promising alternative for urea production. However, the current electrochemical synthesis of urea faces challenges related to low selectivity and production rates. The development of high-efficiency electrocatalysts is the key to performance improvement of urea electrosynthesis. This minireview primarily focuses on the rational design of catalysts, starting with a mechanistic overview. In addition, the advancement of electrolyzers for urea electrochemical synthesis is also discussed aiming to articulate guiding principles of achieving high-rate production reaching industrial relevant level in the future.
期刊介绍：
The development of the Current Opinion journals stemmed from the acknowledgment of the growing challenge for specialists to stay abreast of the expanding volume of information within their field. In Current Opinion in Electrochemistry, they help the reader by providing in a systematic manner:
1.The views of experts on current advances in electrochemistry in a clear and readable form.
2.Evaluations of the most interesting papers, annotated by experts, from the great wealth of original publications.
In the realm of electrochemistry, the subject is divided into 12 themed sections, with each section undergoing an annual review cycle:
• Bioelectrochemistry • Electrocatalysis • Electrochemical Materials and Engineering • Energy Storage: Batteries and Supercapacitors • Energy Transformation • Environmental Electrochemistry • Fundamental & Theoretical Electrochemistry • Innovative Methods in Electrochemistry • Organic & Molecular Electrochemistry • Physical & Nano-Electrochemistry • Sensors & Bio-sensors •
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