Spontaneous Small Biskyrmions in a Centrosymmetric Rare-Earth Kagome Ferrimagnet

IF 8.6 2区 材料科学 Q1 MATERIALS SCIENCE, MULTIDISCIPLINARY Npg Asia Materials Pub Date : 2024-03-15 DOI:10.1038/s41427-024-00534-y
Shulan Zuo, Kaiming Qiao, Zhan Wang, Ying Zhang, Chengbao Jiang, Baogen Shen
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Abstract

Magnetic skyrmions with nontrivial topologies have great potential to serve as memory cells in novel spintronic devices. Small skyrmions were theoretically and experimentally confirmed to be generated under the influence of external fields in ferrimagnetic films via Dzyaloshinskii–Moriya interactions (DMIs). However, this topological state has yet to be verified in ferrimagnetic crystals, especially in the absence of external fields and DMIs. Here, spontaneous biskyrmions were directly observed in the Tb0.2Gd0.8Co2 ferrimagnetic crystal with a Kagome lattice using Lorentz transmission electron microscopy. The high-density biskyrmions exhibited a small size (approximately 50 nm) over a wide temperature range, were closely related to subtle magnetic interaction competition, and coexisted with some broken stripes that could be easily converted into zero-field biskyrmions by utilizing proper field-cooling manipulation. These results can be used to establish a platform for investigating functional sub-50-nm skyrmions in ferrimagnetic crystals and to facilitate advanced applications in magnetic devices. Scientists have found a new method to control small skyrmions, which are tiny magnetic patterns, in ferrimagnetic materials (materials that have a net magnetic moment even without an external magnetic field arising from the two opposite magnetic sublattices). The research, led by S.L. Zuo and K.M. Qiao, revealed that these skyrmions can be maintained in ferrimagnetic materials without requiring an external magnetic field. The researchers used a technique called Lorentz transmission electron microscopy to observe the skyrmions in a specific ferrimagnetic crystal, Tb0.2Gd0.8Co2. They discovered that the skyrmions remained stable across a broad temperature range and could be easily controlled by altering the temperature or applying a minor magnetic field. This finding could be crucial for the creation of future spintronic devices, devices that use the rotation of electrons to store and process data. This summary was initially drafted using artificial intelligence, then revised and fact-checked by the author.

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中心对称稀土卡戈梅铁磁体中的自发小比斯基米尔离子
具有非复杂拓扑结构的磁天线具有在新型自旋电子器件中用作存储单元的巨大潜力。理论和实验证实,在铁磁性薄膜的外部磁场影响下,可以通过 Dzyaloshinskii-Moriya 相互作用(DMIs)产生小型天幕。然而,这种拓扑状态尚未在铁磁晶体中得到验证,尤其是在没有外场和 DMI 的情况下。在这里,我们利用洛伦兹透射电子显微镜直接观察到了具有 Kagome 晶格的 Tb0.2Gd0.8Co2 铁磁晶体中的自发双yrmions。在很宽的温度范围内,高密度双yrmions 的尺寸很小(约 50 nm),与微妙的磁相互作用竞争密切相关,并与一些断裂的条纹共存,通过适当的场冷却操作,这些断裂的条纹可以很容易地转化为零场双yrmions。这些结果可用于建立一个平台,以研究铁磁晶体中 50 纳米以下的功能性天戎,并促进磁性器件的先进应用。
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来源期刊
Npg Asia Materials
Npg Asia Materials MATERIALS SCIENCE, MULTIDISCIPLINARY-
CiteScore
15.40
自引率
1.00%
发文量
87
审稿时长
2 months
期刊介绍: NPG Asia Materials is an open access, international journal that publishes peer-reviewed review and primary research articles in the field of materials sciences. The journal has a global outlook and reach, with a base in the Asia-Pacific region to reflect the significant and growing output of materials research from this area. The target audience for NPG Asia Materials is scientists and researchers involved in materials research, covering a wide range of disciplines including physical and chemical sciences, biotechnology, and nanotechnology. The journal particularly welcomes high-quality articles from rapidly advancing areas that bridge the gap between materials science and engineering, as well as the classical disciplines of physics, chemistry, and biology. NPG Asia Materials is abstracted/indexed in Journal Citation Reports/Science Edition Web of Knowledge, Google Scholar, Chemical Abstract Services, Scopus, Ulrichsweb (ProQuest), and Scirus.
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