Porous electrocatalysts modified electrodes in organic electrocatalysis

IF 7.9 2区 化学 Q1 CHEMISTRY, PHYSICAL Current Opinion in Electrochemistry Pub Date : 2024-03-11 DOI:10.1016/j.coelec.2024.101478
Xinglei He, Hong Yan, Ke-Yin Ye
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Abstract

Porous materials are emerging recyclable electrocatalysts that exhibit many advantages such as rich pore environments, tunable structures and functionalities, and large specific surface areas. However, the research of these materials in organic electrocatalysis is promising but only emerged recently. In this review, we summarized the latest research progress of porous carbon materials, metal-organic frameworks (MOFs), and covalent-organic frameworks (COFs) in organic electrocatalysis, focusing on their structural optimization, electrochemical performance, and reaction mechanisms. In addition, the main challenges and future directions in this field were also discussed. We hope that this review can inspire more research interest of synthetic organic chemists in the development of porous electrocatalysts in organic electrocatalysis.

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有机电催化中的多孔电催化剂改性电极
多孔材料是新兴的可回收电催化剂,具有许多优点,如丰富的孔隙环境、可调的结构和功能以及较大的比表面积。然而,这些材料在有机电催化方面的研究前景广阔,但最近才刚刚兴起。在这篇综述中,我们总结了多孔碳材料、金属有机框架(MOFs)和共价有机框架(COFs)在有机电催化中的最新研究进展,重点介绍了它们的结构优化、电化学性能和反应机理。此外,还讨论了该领域的主要挑战和未来发展方向。希望这篇综述能激发更多有机合成化学家对有机电催化中多孔电催化剂开发的研究兴趣。
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来源期刊
Current Opinion in Electrochemistry
Current Opinion in Electrochemistry Chemistry-Analytical Chemistry
CiteScore
14.00
自引率
5.90%
发文量
272
审稿时长
73 days
期刊介绍: The development of the Current Opinion journals stemmed from the acknowledgment of the growing challenge for specialists to stay abreast of the expanding volume of information within their field. In Current Opinion in Electrochemistry, they help the reader by providing in a systematic manner: 1.The views of experts on current advances in electrochemistry in a clear and readable form. 2.Evaluations of the most interesting papers, annotated by experts, from the great wealth of original publications. In the realm of electrochemistry, the subject is divided into 12 themed sections, with each section undergoing an annual review cycle: • Bioelectrochemistry • Electrocatalysis • Electrochemical Materials and Engineering • Energy Storage: Batteries and Supercapacitors • Energy Transformation • Environmental Electrochemistry • Fundamental & Theoretical Electrochemistry • Innovative Methods in Electrochemistry • Organic & Molecular Electrochemistry • Physical & Nano-Electrochemistry • Sensors & Bio-sensors •
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