Raman Scattering Spectroscopy and Photoluminescence of GaAs Nanowires

IF 0.5 Q4 PHYSICS, MULTIDISCIPLINARY Optoelectronics Instrumentation and Data Processing Pub Date : 2024-03-26 DOI:10.3103/s8756699023060055
I. V. Kalachev, I. A. Milekhin, E. A. Emel’yanov, V. V. Preobrazhenskii, V. S. Tumashev, A. G. Milekhin, A. V. Latyshev
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Abstract

Experimental data on studying the phonon and optical properties of GaAs nanowires with orientation (111) located on a gold substrate with the help of Raman scattering spectroscopy (RSS) and photoluminescence (PL) are presented. Structural parameters of nanowires are determined by the atomic-force microscopy (AFM) and scanning electron microscopy (SEM) methods. In the micro-RSS and micro-PL spectra of a single GaAs nanowire, the modes of optical phonons of GaAs and their overtones up to the third order and an exciton luminescence band are observed. In the micro-PL spectra, anisotropy of the PL intensity is observed; the maximum/minimum signal is observed at the polarization-vector direction along/across the wire. Mapping of nano-PL of a single GaAs nanowire is performed with a spatial resolution of 20 nm, which is significantly smaller than the diffraction limit. When passing to the nanometer scale, a plasmon amplification of the signal of the near-field exciton nano-PL conditioned by the metallized AFM-needle is revealed.

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砷化镓纳米线的拉曼散射光谱学和光致发光
摘要 介绍了借助拉曼散射光谱(RSS)和光致发光(PL)研究金基底上取向(111)的砷化镓纳米线的声子和光学特性的实验数据。纳米线的结构参数是通过原子力显微镜(AFM)和扫描电子显微镜(SEM)方法确定的。在单根砷化镓纳米线的微 RSS 和微光致发光光谱中,观察到了砷化镓的光学声子模式及其高达三阶的泛音和激子发光带。在微PL光谱中,可观察到PL强度的各向异性;在沿着/穿过导线的偏振矢量方向上可观察到最大/最小信号。绘制单根砷化镓纳米线的纳米光致发光图的空间分辨率为 20 纳米,明显小于衍射极限。当达到纳米尺度时,金属化原子力显微镜针对近场激子纳米光致发光信号的等离子放大作用显现出来。
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来源期刊
CiteScore
1.00
自引率
50.00%
发文量
16
期刊介绍: The scope of Optoelectronics, Instrumentation and Data Processing encompasses, but is not restricted to, the following areas: analysis and synthesis of signals and images; artificial intelligence methods; automated measurement systems; physicotechnical foundations of micro- and optoelectronics; optical information technologies; systems and components; modelling in physicotechnical research; laser physics applications; computer networks and data transmission systems. The journal publishes original papers, reviews, and short communications in order to provide the widest possible coverage of latest research and development in its chosen field.
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